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Energy consumption estimation for greenhouse gas separation processes by clathrate hydrate formation

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  • Tajima, Hideo
  • Yamasaki, Akihiro
  • Kiyono, Fumio

Abstract

The process energy consumption was estimated for gas separation processes by the formation of clathrate hydrates. The separation process is based on the equilibrium partition of the components between the gaseous phase and the hydrate phase. The separation and capturing processes of greenhouse gases were examined in this study. The target components were hydrofluorocarbon (HFC-134a) from air, sulfur hexafluoride (SF6) from nitrogen, and CO2 from flue gas. Since these greenhouse gases would form hydrates under much lower pressure and higher temperature conditions than the accompanying components, the effective capturing of the greenhouse gases could be achieved by using hydrate formation. A model separation process for each gaseous mixture was designed from the basis of thermodynamics, and the process energy consumption was estimated. The obtained results were then compared with those for conventional separation processes such as liquefaction separation processes. For the recovery of SF6, the hydrate process is preferable to liquefaction process in terms of energy consumption. On the other hand, the liquefaction process consumes less energy than the hydrate process for the recovery of HFC-134a. The capturing of CO2 by the hydrate process from a flue gas will consume a considerable amount of energy; mainly due to the extremely high pressure conditions required for hydrate formation. The influences of the operation conditions on the heat of hydrate formation were elucidated by sensitivity analysis. The hydrate processes for separating these greenhouse gases were evaluated in terms of reduction of global warming potential (GWP).

Suggested Citation

  • Tajima, Hideo & Yamasaki, Akihiro & Kiyono, Fumio, 2004. "Energy consumption estimation for greenhouse gas separation processes by clathrate hydrate formation," Energy, Elsevier, vol. 29(11), pages 1713-1729.
  • Handle: RePEc:eee:energy:v:29:y:2004:i:11:p:1713-1729
    DOI: 10.1016/j.energy.2004.03.003
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    1. Ge, Bin-Bin & Li, Xi-Yue & Zhong, Dong-Liang & Lu, Yi-Yu, 2022. "Investigation of natural gas storage and transportation by gas hydrate formation in the presence of bio-surfactant sulfonated lignin," Energy, Elsevier, vol. 244(PA).
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    3. Remi-Erempagamo Tariyemienyo Meindinyo & Thor Martin Svartaas, 2016. "Gas Hydrate Growth Kinetics: A Parametric Study," Energies, MDPI, vol. 9(12), pages 1-29, December.
    4. Sun, Qie & Li, Hailong & Yan, Jinying & Liu, Longcheng & Yu, Zhixin & Yu, Xinhai, 2015. "Selection of appropriate biogas upgrading technology-a review of biogas cleaning, upgrading and utilisation," Renewable and Sustainable Energy Reviews, Elsevier, vol. 51(C), pages 521-532.
    5. Wang, Xiaolin & Zhang, Fengyuan & LipiƄski, Wojciech, 2020. "Research progress and challenges in hydrate-based carbon dioxide capture applications," Applied Energy, Elsevier, vol. 269(C).
    6. Lee, Yohan & Lee, Dongyoung & Lee, Jong-Won & Seo, Yongwon, 2016. "Enclathration of CO2 as a co-guest of structure H hydrates and its implications for CO2 capture and sequestration," Applied Energy, Elsevier, vol. 163(C), pages 51-59.
    7. Sa, Jeong-Hoon & Sum, Amadeu K., 2019. "Promoting gas hydrate formation with ice-nucleating additives for hydrate-based applications," Applied Energy, Elsevier, vol. 251(C), pages 1-1.
    8. Yang, Mingjun & Jing, Wen & Zhao, Jiafei & Ling, Zheng & Song, Yongchen, 2016. "Promotion of hydrate-based CO2 capture from flue gas by additive mixtures (THF (tetrahydrofuran) + TBAB (tetra-n-butyl ammonium bromide))," Energy, Elsevier, vol. 106(C), pages 546-553.
    9. Foroutan, Shima & Mohsenzade, Hanie & Dashti, Ali & Roosta, Hadi, 2021. "New insights into the evaluation of kinetic hydrate inhibitors and energy consumption in rocking and stirred cells," Energy, Elsevier, vol. 218(C).
    10. Babu, Ponnivalavan & Linga, Praveen & Kumar, Rajnish & Englezos, Peter, 2015. "A review of the hydrate based gas separation (HBGS) process for carbon dioxide pre-combustion capture," Energy, Elsevier, vol. 85(C), pages 261-279.
    11. Zhao, Ruikai & Deng, Shuai & Liu, Yinan & Zhao, Qing & He, Junnan & Zhao, Li, 2017. "Carbon pump: Fundamental theory and applications," Energy, Elsevier, vol. 119(C), pages 1131-1143.
    12. Kim, Soyoung & Seo, Yongwon, 2015. "Semiclathrate-based CO2 capture from flue gas mixtures: An experimental approach with thermodynamic and Raman spectroscopic analyses," Applied Energy, Elsevier, vol. 154(C), pages 987-994.
    13. Zhang, Yingying & Ji, Xiaoyan & Lu, Xiaohua, 2014. "Energy consumption analysis for CO2 separation from gas mixtures," Applied Energy, Elsevier, vol. 130(C), pages 237-243.
    14. Babu, Ponnivalavan & Kumar, Rajnish & Linga, Praveen, 2013. "Pre-combustion capture of carbon dioxide in a fixed bed reactor using the clathrate hydrate process," Energy, Elsevier, vol. 50(C), pages 364-373.
    15. Liu, Fa-Ping & Li, Ai-Rong & Qing, Sheng-Lan & Luo, Ze-Dong & Ma, Yu-Ling, 2022. "Formation kinetics, mechanism of CO2 hydrate and its applications," Renewable and Sustainable Energy Reviews, Elsevier, vol. 159(C).
    16. Liu, Yinan & Deng, Shuai & Zhao, Ruikai & He, Junnan & Zhao, Li, 2017. "Energy-saving pathway exploration of CCS integrated with solar energy: A review of innovative concepts," Renewable and Sustainable Energy Reviews, Elsevier, vol. 77(C), pages 652-669.
    17. Xu, Chun-Gang & Xie, Wen-Jun & Chen, Guo-Shu & Yan, Xiao-Xue & Cai, Jing & Chen, Zhao-Yang & Li, Xiao-Sen, 2020. "Study on the influencing factors of gas consumption in hydrate-based CO2 separation in the presence of CP by Raman analysis," Energy, Elsevier, vol. 198(C).
    18. Veluswamy, Hari Prakash & Kumar, Rajnish & Linga, Praveen, 2014. "Hydrogen storage in clathrate hydrates: Current state of the art and future directions," Applied Energy, Elsevier, vol. 122(C), pages 112-132.
    19. Babu, Ponnivalavan & Ho, Chie Yin & Kumar, Rajnish & Linga, Praveen, 2014. "Enhanced kinetics for the clathrate process in a fixed bed reactor in the presence of liquid promoters for pre-combustion carbon dioxide capture," Energy, Elsevier, vol. 70(C), pages 664-673.
    20. Tooba Qureshi & Majeda Khraisheh & Fares Almomani, 2023. "Cost and Heat Integration Analysis for CO 2 Removal Using Imidazolium-Based Ionic Liquid-ASPEN PLUS Modelling Study," Sustainability, MDPI, vol. 15(4), pages 1-23, February.

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