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Economic evaluation for four different solid sorbent processes with heat integration for energy-efficient CO2 capture based on PEI-silica sorbent

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  • Jung, Wonho
  • Lee, Jinwon

Abstract

An amine-functionalized solid sorbent-based process with heat integration is considered an energy-efficient method for large-scale CO2 capture. Herein, we propose a techno-economic analysis (TEA) of four different solid sorbent processes for post-combustion CO2 capture with internal heat integration as an alternative to the conventional amine scrubbing process. Our proposed processes are fluidized bed adsorption, fixed bed adsorption, moving bed adsorption, and rapid thermal swing adsorption and involve continuous adsorption, heating, desorption, and cooling. In addition, the four processes use an amine-functionalized solid sorbent, SiO2/0.37 EB-PEI, which was transformed into powder, pellet, and hollow fiber to reflect the characteristics of each process. The proposed processes enable internal heat integration by recovering sensible heat from the cooling process and further enhance the CO2 cyclic capacity of amine-functionalized solid sorbents with high CO2 recovery by performing adsorption heat removal. Most importantly, our TEA based on rigorous mathematical modeling revealed that the CO2 capture cost of the four solid sorbent-based processes was approximately 48.1–75.2 $/t-CO2, with a 45%–58% sensible heat recovery. Such a low CO2 capture cost is comparable to that of the most mature amine-based absorption process (62.8 $/t-CO2), owing to a combination of internal heat integration and enhanced CO2 cyclic capacity. The results support the feasibility of four solid sorbent-based processes for post-combustion CO2 capture.

Suggested Citation

  • Jung, Wonho & Lee, Jinwon, 2022. "Economic evaluation for four different solid sorbent processes with heat integration for energy-efficient CO2 capture based on PEI-silica sorbent," Energy, Elsevier, vol. 238(PC).
  • Handle: RePEc:eee:energy:v:238:y:2022:i:pc:s0360544221021125
    DOI: 10.1016/j.energy.2021.121864
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    References listed on IDEAS

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    1. Jung, Wonho & Park, Junhyung & Won, Wangyun & Lee, Kwang Soon, 2018. "Simulated moving bed adsorption process based on a polyethylenimine-silica sorbent for CO2 capture with sensible heat recovery," Energy, Elsevier, vol. 150(C), pages 950-964.
    2. Yun, Seokwon & Oh, Se-Young & Kim, Jin-Kuk, 2020. "Techno-economic assessment of absorption-based CO2 capture process based on novel solvent for coal-fired power plant," Applied Energy, Elsevier, vol. 268(C).
    3. Woosung Choi & Kyungmin Min & Chaehoon Kim & Young Soo Ko & Jae Wan Jeon & Hwimin Seo & Yong-Ki Park & Minkee Choi, 2016. "Epoxide-functionalization of polyethyleneimine for synthesis of stable carbon dioxide adsorbent in temperature swing adsorption," Nature Communications, Nature, vol. 7(1), pages 1-8, November.
    4. Park, Junhyung & Won, Wangyun & Jung, Wonho & Lee, Kwang Soon, 2019. "One-dimensional modeling of a turbulent fluidized bed for a sorbent-based CO2 capture process with solid–solid sensible heat exchange," Energy, Elsevier, vol. 168(C), pages 1168-1180.
    5. Lee, Sunghoon & Kim, Jin-Kuk, 2020. "Process-integrated design of a sub-ambient membrane process for CO2 removal from natural gas power plants," Applied Energy, Elsevier, vol. 260(C).
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    1. Akinola, Toluleke E. & Bonilla Prado, Phebe L. & Wang, Meihong, 2022. "Experimental studies, molecular simulation and process modelling\simulation of adsorption-based post-combustion carbon capture for power plants: A state-of-the-art review," Applied Energy, Elsevier, vol. 317(C).
    2. A. G. Olabi & Tabbi Wilberforce & Enas Taha Sayed & Nabila Shehata & Abdul Hai Alami & Hussein M. Maghrabie & Mohammad Ali Abdelkareem, 2022. "Prospect of Post-Combustion Carbon Capture Technology and Its Impact on the Circular Economy," Energies, MDPI, vol. 15(22), pages 1-38, November.

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