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Impregnation of microporous SDC scaffold as stable solid oxide cell BSCF-based air electrode

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  • Asensio, Antonio Maria
  • Clematis, Davide
  • Viviani, Massimo
  • Carpanese, M. Paola
  • Presto, Sabrina
  • Cademartori, Davide
  • Cabot, Pere L.
  • Barbucci, Antonio

Abstract

Barium strontium cobaltite-ferrite (Ba1-xSrxCoyFe1-yO3-δ, BSCF) is a widely studied mixed ionic-electronic conductor material for air electrode in solid oxide cells (SOC). Despite having excellent features, due to fast oxygen surface exchange and oxygen bulk diffusion, it lacks long-term stability. Electrode/electrolyte thermal expansion coefficient (TEC) mismatch and structural instability at temperature lower than 900 °C are responsible for the increase of electrode polarization which becomes a crucial issue for the long-term stability.

Suggested Citation

  • Asensio, Antonio Maria & Clematis, Davide & Viviani, Massimo & Carpanese, M. Paola & Presto, Sabrina & Cademartori, Davide & Cabot, Pere L. & Barbucci, Antonio, 2021. "Impregnation of microporous SDC scaffold as stable solid oxide cell BSCF-based air electrode," Energy, Elsevier, vol. 237(C).
    • Handle: RePEc:eee:energy:v:237:y:2021:i:c:s036054422101762x
    DOI: 10.1016/j.energy.2021.121514
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    References listed on IDEAS

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    1. Xavier Majnoni d’Intignano & Davide Cademartori & Davide Clematis & Sabrina Presto & Massimo Viviani & Rodolfo Botter & Antonio Barbucci & Giacomo Cerisola & Gilles Caboche & M. Paola Carpanese, 2020. "Infiltrated Ba 0.5 Sr 0.5 Co 0.8 Fe 0.2 O 3-δ -Based Electrodes as Anodes in Solid Oxide Electrolysis Cells," Energies, MDPI, vol. 13(14), pages 1-10, July.
    2. Heleen L. Soest & Michel G. J. Elzen & Detlef P. Vuuren, 2021. "Net-zero emission targets for major emitting countries consistent with the Paris Agreement," Nature Communications, Nature, vol. 12(1), pages 1-9, December.
    3. Nicole Glanemann & Sven N. Willner & Anders Levermann, 2020. "Paris Climate Agreement passes the cost-benefit test," Nature Communications, Nature, vol. 11(1), pages 1-11, December.
    4. Mahmood, Asif & Bano, Saira & Yu, Ji Haeng & Lee, Kew-Ho, 2015. "High-performance solid oxide electrolysis cell based on ScSZ/GDC (scandia-stabilized zirconia/gadolinium-doped ceria) bi-layered electrolyte and LSCF (lanthanum strontium cobalt ferrite) oxygen electr," Energy, Elsevier, vol. 90(P1), pages 344-350.
    5. Chen, Guihua & Wang, Yong & Sunarso, Jaka & Liang, Fengli & Wang, Huanping, 2016. "A new scandium and niobium co-doped cobalt-free perovskite cathode for intermediate-temperature solid oxide fuel cells," Energy, Elsevier, vol. 95(C), pages 137-143.
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    1. Gao, Juntao & Ma, Dan & Zhao, Hui & Li, Qiang & Lü, Zhe & Wei, Bo, 2022. "Synergistically improving electrocatalytic performance and CO2 tolerance of Fe-based cathode catalysts for solid oxide fuel cells," Energy, Elsevier, vol. 252(C).

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