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Engineering iron phosphide-on-plasmonic Ag/Au-nanoshells as an efficient cathode catalyst in water splitting for hydrogen production

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  • Zhao, Zhenlu
  • Wu, Haoxi
  • Li, Chuanping

Abstract

Constructing highly active electrocatalysts for hydrogen evolution reaction (HER) have drawn considerable attention recently. However, how to design nanostructured electrocatalysts with enhanced catalytic performances is still a challenge. Herein, plasmonic Ag/Au hollow porous nanoshells decorated with porous Fe2P thin layers (denoted as Ag/Au-HPNSs@PFP) are fabricated, in which porous Fe2P (PFP) thin layers are derived from pyrolysis and phosphidation of MIL-100(Fe) coated on plasmonic Ag/Au hollow porous nanoshells (Ag/Au-HPNSs) and the high porosity of the HER-active Fe2P, along with plasmonic enhancement of the Ag/Au hollow porous nanoshells, facilitates hydrogen evolution and electron transport, and accordingly boosts the electrocatalytic HER performance. When applied as a HER electrode, the hybrid electrocatalyst displays an onset overpotential of only 108 mV, satisfactory stability, and enhanced performance for hydrogen evolution under visible light, ascribing to electron interactions between Fe and P and synergistic effects of porous Fe2P and plasmonic Au/Ag hollow porous nanoshells.

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  • Zhao, Zhenlu & Wu, Haoxi & Li, Chuanping, 2021. "Engineering iron phosphide-on-plasmonic Ag/Au-nanoshells as an efficient cathode catalyst in water splitting for hydrogen production," Energy, Elsevier, vol. 218(C).
    • Handle: RePEc:eee:energy:v:218:y:2021:i:c:s036054422032627x
    DOI: 10.1016/j.energy.2020.119520
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    References listed on IDEAS

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    1. Yao Zheng & Yan Jiao & Yihan Zhu & Lu Hua Li & Yu Han & Ying Chen & Aijun Du & Mietek Jaroniec & Shi Zhang Qiao, 2014. "Hydrogen evolution by a metal-free electrocatalyst," Nature Communications, Nature, vol. 5(1), pages 1-8, September.
    2. Yongdong Jin & Congxian Jia & Sheng-Wen Huang & Matthew O'Donnell & Xiaohu Gao, 2010. "Multifunctional nanoparticles as coupled contrast agents," Nature Communications, Nature, vol. 1(1), pages 1-8, December.
    3. Zhang, Yuanyuan & Sun, Haohao & Qiu, Yunfeng & Zhang, Enhao & Ma, Tiange & Gao, Guang-gang & Cao, Changyan & Ma, Zhuo & Hu, PingAn, 2018. "Bifunctional hydrogen evolution and oxygen evolution catalysis using CoP-embedded N-doped nanoporous carbon synthesized via TEOS-assisted method," Energy, Elsevier, vol. 165(PB), pages 537-548.
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    Cited by:

    1. Liu, Wei & Tan, Wenyu & He, Hanwei & Peng, Yizhi & Chen, Yuxiang & Yang, Yang, 2022. "One–step electrodeposition of Ni–Ce–Pr–Ho/NF as an efficient electrocatalyst for hydrogen evolution reaction in alkaline medium," Energy, Elsevier, vol. 250(C).
    2. Guo, Junyan & Gao, Ruihong & Tong, Zhaoming & Zhang, Haijun & Duan, Hongjuan & Huang, Liang & Lu, Lilin & Jia, Quanli & Zhang, Shaowei, 2023. "Three eagles with one arrow: Simultaneous production of hydrogen, aluminum ethoxide, and supported metal catalysts via efficient and facile reaction between aluminum and ethanol," Energy, Elsevier, vol. 263(PD).

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