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Enhancing hydrogen-rich syngas production and energy recovery efficiency by integrating hydrothermal carbonization pretreatment with steam gasification

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  • Peng, Nana
  • Gai, Chao
  • Peng, Chao

Abstract

Steam gasification behavior and kinetics of hydrothermally treated low-lipid microalgae Nannochloropsis sp. were probed in this work. The roles of hydrothermal carbonization (HTC) parameters (HTC temperature, HTC reaction time) as well as gasification conditions (gasification temperature, S/B mass ratio) in modulating the properties of hydrothermal carbons (HCs) as well as gasification performance were elucidated. Experimental results indicated that the aromaticity of the HCs derived from Nannochloropsis sp. was promoted, whereas the polarity was lowered by the increased HTC temperature and reaction time. At optimum HTC conditions (HTC temperature of 180 °C, residence time of 12 h) and gasification conditions (gasification temperature of 900 °C, S/B mass ratio of 2), the total maximum energy recovery efficiency was as high as 1.59. Kinetic parameters for the major gaseous products during the steam gasification of raw microalgae and the two typical HCs (HC–180C-12 h and HC-220C-12 h) were further determined. Kinetic results verified that the gasification reactivity of HC-180C-12 h was greatly higher than other two feedstock, and H2 formation was greatly promoted compared to the other two gaseous products. Overall, combining hydrothermal pretreatment and steam gasification in one step is a promising technology that could greatly promote hydrogen-rich syngas production and energy recovery efficiency from low-lipid microalgae.

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  • Peng, Nana & Gai, Chao & Peng, Chao, 2020. "Enhancing hydrogen-rich syngas production and energy recovery efficiency by integrating hydrothermal carbonization pretreatment with steam gasification," Energy, Elsevier, vol. 210(C).
    • Handle: RePEc:eee:energy:v:210:y:2020:i:c:s0360544220317631
    DOI: 10.1016/j.energy.2020.118655
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    References listed on IDEAS

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    3. Jia, Yongsheng & Wang, Yingjie & Jiang, Cong & Wang, Xun & Hu, Zhiquan & Xiao, Bo & Liu, Shiming, 2022. "Simultaneous enhancement of the H2 yield and HCl removal efficiency from pyrolysis of infusion tube under novel mayenite-based mesoporous catalytic sorbents," Energy, Elsevier, vol. 244(PB).
    4. Krishnamoorthy, Amarnath & Rodriguez, Cristina & Durrant, Andy, 2023. "Optimisation of ultrasonication pretreatment on microalgae Chlorella Vulgaris & Nannochloropsis Oculata for lipid extraction in biodiesel production," Energy, Elsevier, vol. 278(PB).
    5. Amira Alazmi & Sabina A. Nicolae & Pierpaolo Modugno & Bashir E. Hasanov & Maria M. Titirici & Pedro M. F. J. Costa, 2021. "Activated Carbon from Palm Date Seeds for CO 2 Capture," IJERPH, MDPI, vol. 18(22), pages 1-11, November.
    6. Xie, Xiaodi & Peng, Chao & Song, Xinyu & Peng, Nana & Gai, Chao, 2022. "Pyrolysis kinetics of the hydrothermal carbons derived from microwave-assisted hydrothermal carbonization of food waste digestate," Energy, Elsevier, vol. 245(C).

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