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Sandwich-like silicon/Ti3C2Tx MXene composite by electrostatic self-assembly for high performance lithium ion battery

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  • Zhang, Fan
  • Jia, Zirui
  • Wang, Chao
  • Feng, Ailing
  • Wang, Kuikui
  • Hou, Tianqi
  • Liu, Jiajia
  • Zhang, Yi
  • Wu, Guanglei

Abstract

Silicon has been regarded as a promising anode materials for lithium ion battery. However, large volume change during lithiation/delithiation process impedes its application for energy storage. Two-dimensional titanium carbide or carbonitride nanosheet, known as MXene, possesses layered-stacked structure and high electrical conductivity. So MXene has a great potential to improve the cycle life of silicon anode because its layered-stacked structure can accommodate the volume expansion of silicon. Herein, we present a facile process to prepare sandwich-like silicon/Ti3C2Tx MXene composite directed by electrostatic self-assembly. This unique architecture could accommodate silicon expansion during lithiation and enhance electronical conductivity. The silicon/Ti3C2Tx MXene composite delivers an initial reversible capacity of 1067.6 mAh g−1 at a current of 300 mA g−1. Moreover, it shows a steady cycling ability of 643.8 mAh g−1 at 300 mA g−1 after 100 cycles. This work may shed lights on the development of high energy density silicon-based anode materials for lithium ion battery.

Suggested Citation

  • Zhang, Fan & Jia, Zirui & Wang, Chao & Feng, Ailing & Wang, Kuikui & Hou, Tianqi & Liu, Jiajia & Zhang, Yi & Wu, Guanglei, 2020. "Sandwich-like silicon/Ti3C2Tx MXene composite by electrostatic self-assembly for high performance lithium ion battery," Energy, Elsevier, vol. 195(C).
    • Handle: RePEc:eee:energy:v:195:y:2020:i:c:s0360544220301547
    DOI: 10.1016/j.energy.2020.117047
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    References listed on IDEAS

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    1. Eddahech, Akram & Briat, Olivier & Vinassa, Jean-Michel, 2013. "Thermal characterization of a high-power lithium-ion battery: Potentiometric and calorimetric measurement of entropy changes," Energy, Elsevier, vol. 61(C), pages 432-439.
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    1. Chen, Jiasheng & Wang, Xuan Liang & Jin, En Mei & Moon, Seung-Guen & Jeong, Sang Mun, 2021. "Optimization of B2O3 coating process for NCA cathodes to achieve long-term stability for application in lithium ion batteries," Energy, Elsevier, vol. 222(C).
    2. Jin, En Mei & Kim, Min Soo & Kim, Tae Yun & Shin, Beom-Ju & Moon, Jong-Ho & Jeong, Sang Mun, 2023. "Upcycling of silicon scrap collected from photovoltaic cell manufacturing process for lithium-ion batteries via transferred arc thermal plasma," Energy, Elsevier, vol. 262(PB).
    3. Tang, Hong & Jiang, Mengjin & Ren, Erhui & Zhang, Yue & Lai, Xiaoxu & Cui, Ce & Jiang, Shouxiang & Zhou, Mi & Qin, Qin & Guo, Ronghui, 2020. "Integrate electrical conductivity and Li+ ion mobility into hierarchical heterostructure Ti3C2@CoO/ZnO composites toward high-performance lithium ion storage," Energy, Elsevier, vol. 212(C).

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