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Facile fabrication and nanostructure control of mesoporous iridium oxide films for efficient electrocatalytic water oxidation

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  • Chandra, Debraj
  • Sato, Tetsuya
  • Tanahashi, Yuki
  • Takeuchi, Ryouchi
  • Yagi, Masayuki

Abstract

The development of efficient catalyst materials for water oxidation is bottleneck to construct artificial photosynthesis that is a promising future energy-providing system. We review the recent progress on development of IrOx electrocatalyst films for water oxidation based on our latest research works. A controlled fabrication approach of an efficient IrOx electrocatalyst films is introduced by a facile spin-coating of a homogenous solution of Ir precursor complexes followed by simple annealing at different temperature. The composition and crystallinity of the IrOx film are tunable by a simple annealing treatment. The electrocatalytic properties of the IrOx film dramatically depended on annealing temperature are characterized to give the noticeably high performance at 300 °C annealing. A soft-template-assisted technique using different polymer surfactants as structure directing agents (SDAs) is illustrated in the spin-coating procedure to reveal impacts of SDAs on nanostructures and electrocatalytic water oxidation performances of the IrOx films. The characterization of the first accessible channel-like open pore architecture of the ordered 2D-hexagonal mesoporous IrOx film is described by a facile one-pot strategy using Pluronic F127 as SDA. The novel controlled nanostructures including mesoporous architecture of IrOx improves electrocatalytic performance for water oxidation relative to a conventional nanoparticulate structure of IrOx coating.

Suggested Citation

  • Chandra, Debraj & Sato, Tetsuya & Tanahashi, Yuki & Takeuchi, Ryouchi & Yagi, Masayuki, 2019. "Facile fabrication and nanostructure control of mesoporous iridium oxide films for efficient electrocatalytic water oxidation," Energy, Elsevier, vol. 173(C), pages 278-289.
    • Handle: RePEc:eee:energy:v:173:y:2019:i:c:p:278-289
    DOI: 10.1016/j.energy.2019.02.072
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    References listed on IDEAS

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    1. Marshall, A. & Børresen, B. & Hagen, G. & Tsypkin, M. & Tunold, R., 2007. "Hydrogen production by advanced proton exchange membrane (PEM) water electrolysers—Reduced energy consumption by improved electrocatalysis," Energy, Elsevier, vol. 32(4), pages 431-436.
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