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Free-standing bimetallic CoNiTe2 nanosheets as efficient catalysts with high stability at large current density for oxygen evolution reaction

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Listed:
  • Qian, Guangfu
  • Mo, Yanshan
  • Yu, Chen
  • Zhang, Hao
  • Yu, Tianqi
  • Luo, Lin
  • Yin, Shibin

Abstract

The oxygen evolution reaction (OER) step for water splitting requires highly efficient, low-cost and stable catalysts. As efficient catalytic materials for OER, bimetallic telluride (CoNiTe2/NF) nanosheets are prepared by the combination of hydrothermal and calcination method in this work. The physicochemical characterizations confirm that the surface of CoNiTe2/NF is covered by bimetallic telluride compounds (CoNiTe2) with 3D morphology composed of thin and defective nanosheets that are well-distributed on nickel foam (NF). Notably, it shows very low overpotential at 10 (181 mV), 500 (230 mV) and 1000 (270 mV) mA cm−2 and low Tafel slope (44 mV dec−1). Besides, it also exhibits excellent durability lasting 24 h at 100, 500 and 1000 mA cm−2, respectively, without distinct deactivation. This outstanding performance could be due to the bimetallic telluride and the strong covalency around the CoNi center caused by Te that plays a crucial role for enhancing the activity of catalyst. The unique morphology could provide large electrochemical active area and exposure higher amounts of active sites. Meanwhile, the self-supported structure, without binders, could also enhance the performance for OER. This work thus provides a promising strategy to synthesize multi-metal telluride materials as highly efficient and stable catalyst for OER at large current density.

Suggested Citation

  • Qian, Guangfu & Mo, Yanshan & Yu, Chen & Zhang, Hao & Yu, Tianqi & Luo, Lin & Yin, Shibin, 2020. "Free-standing bimetallic CoNiTe2 nanosheets as efficient catalysts with high stability at large current density for oxygen evolution reaction," Renewable Energy, Elsevier, vol. 162(C), pages 2190-2196.
  • Handle: RePEc:eee:renene:v:162:y:2020:i:c:p:2190-2196
    DOI: 10.1016/j.renene.2020.10.028
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