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Co-liquefaction of sewage sludge and rice straw/wood sawdust: The effect of process parameters on the yields/properties of bio-oil and biochar products

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  • Huang, Hua-jun
  • Chang, Yan-chao
  • Lai, Fa-ying
  • Zhou, Chun-fei
  • Pan, Zi-qian
  • Xiao, Xiao-feng
  • Wang, Jia-xin
  • Zhou, Chun-huo

Abstract

Liquefaction is a promising technology for the preparation of bio-oil and biochar products from sewage sludge (SS). Co-liquefaction of SS and agricultural/forestry biomass is likely a potential method for obtaining high yield/quality of bio-oil and biochar. In this work, rice straw (RS) and wood sawdust (WS) were selected as representatives of agricultural/forestry biomass and the effects of main process parameters during the co-liquefaction of SS-RS/WS on the yields/properties of bio-oil and biochar were explored in details. The proper reaction temperature, solid-liquid ratio and reaction time for the co-liquefaction of SS-RS/WS were suggested to be 280–300 °C, 0.1 g/mL and 10–30 min, respectively. Potassium/sodium salt (-OH and -CO3) catalysts could efficiently enhanced the co-liquefaction of SS-RS/WS. The introduction of RS/WS into the liquefaction of SS would reduce the contents of nitrogen and sulfur in bio-oil and enhance the formation of phenolic compounds. In addition, co-liquefaction of SS-RS could promote the percentage of lower-boil-point compounds in bio-oil. Although the thermal stability, surface area and pore volume of biochars slightly decreased, the contents of organic matters in biochars were obviously improved, suggesting higher potential in land application.

Suggested Citation

  • Huang, Hua-jun & Chang, Yan-chao & Lai, Fa-ying & Zhou, Chun-fei & Pan, Zi-qian & Xiao, Xiao-feng & Wang, Jia-xin & Zhou, Chun-huo, 2019. "Co-liquefaction of sewage sludge and rice straw/wood sawdust: The effect of process parameters on the yields/properties of bio-oil and biochar products," Energy, Elsevier, vol. 173(C), pages 140-150.
    • Handle: RePEc:eee:energy:v:173:y:2019:i:c:p:140-150
    DOI: 10.1016/j.energy.2019.02.071
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    3. Kim, Jung-Hun & Oh, Jeong-Ik & Lee, Jechan & Kwon, Eilhann E., 2019. "Valorization of sewage sludge via a pyrolytic platform using carbon dioxide as a reactive gas medium," Energy, Elsevier, vol. 179(C), pages 163-172.
    4. Liu, Yali & Zhai, Yunbo & Li, Shanhong & Liu, Xiangmin & Liu, Xiaoping & Wang, Bei & Qiu, Zhenzi & Li, Caiting, 2020. "Production of bio-oil with low oxygen and nitrogen contents by combined hydrothermal pretreatment and pyrolysis of sewage sludge," Energy, Elsevier, vol. 203(C).
    5. Guanyu Zhang & Kejie Wang & Quan Liu & Lujia Han & Xuesong Zhang, 2022. "A Comprehensive Hydrothermal Co-Liquefaction of Diverse Biowastes for Energy-Dense Biocrude Production: Synergistic and Antagonistic Effects," IJERPH, MDPI, vol. 19(17), pages 1-17, August.
    6. Yuan, Zhilong & Jia, Guangchao & Cui, Xin & Song, Xueping & Wang, Cuiping & Zhao, Peitao & Ragauskas, Art J., 2022. "Effects of temperature and time on supercritical methanol Co-Liquefaction of rice straw and linear low-density polyethylene wastes," Energy, Elsevier, vol. 245(C).

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