IDEAS home Printed from https://ideas.repec.org/a/eee/energy/v161y2018icp104-117.html
   My bibliography  Save this article

Transport phenomena of convergent and divergent serpentine flow fields for PEMFC

Author

Listed:
  • Chowdhury, Mohammad Ziauddin
  • Timurkutluk, Bora

Abstract

Reactive species and water transport are crucial for the proton exchange membrane fuel cell operation and performance, and for this, effective flow field design can facilitate the desired transport characteristics of species. From this motivation, the conventional single serpentine flow field pattern is modified by convergent and divergent design concepts and the complex transport phenomena of the newly developed flow field designs are investigated by a numerical approach. For the numerical analyses, an experimentally validated mathematical model is developed to predict the current density, oxygen mass transport, water concentration and pressure distribution. The different configurations of modified convergent and divergent serpentine flow fields are then numerically solved and the results are compared with the conventional serpentine flow field pattern. The transport of reactive species and water concentration are analyzed from the different perspectives including cathode domains and surfaces with a quantitative formulation of the transport species. The numerical results reveals that the modified convergent serpentine flow fields yield to a uniform current density due to the lower mass fraction of water concentration over the reaction zone facilitating better oxygen mass transport and also higher channel pressure distribution along the flow field comparing the conventional and divergent type serpentine flow fields.

Suggested Citation

  • Chowdhury, Mohammad Ziauddin & Timurkutluk, Bora, 2018. "Transport phenomena of convergent and divergent serpentine flow fields for PEMFC," Energy, Elsevier, vol. 161(C), pages 104-117.
  • Handle: RePEc:eee:energy:v:161:y:2018:i:c:p:104-117
    DOI: 10.1016/j.energy.2018.07.143
    as

    Download full text from publisher

    File URL: http://www.sciencedirect.com/science/article/pii/S0360544218314403
    Download Restriction: Full text for ScienceDirect subscribers only

    File URL: https://libkey.io/10.1016/j.energy.2018.07.143?utm_source=ideas
    LibKey link: if access is restricted and if your library uses this service, LibKey will redirect you to where you can use your library subscription to access this item
    ---><---

    As the access to this document is restricted, you may want to search for a different version of it.

    References listed on IDEAS

    as
    1. Arun Saco, S. & Thundil Karuppa Raj, R. & Karthikeyan, P., 2016. "A study on scaled up proton exchange membrane fuel cell with various flow channels for optimizing power output by effective water management using numerical technique," Energy, Elsevier, vol. 113(C), pages 558-573.
    2. khazaee, I. & Sabadbafan, H., 2016. "Effect of humidity content and direction of the flow of reactant gases on water management in the 4-serpentine and 1-serpentine flow channel in a PEM (proton exchange membrane) fuel cell," Energy, Elsevier, vol. 101(C), pages 252-265.
    3. Wu, Horng-Wen, 2016. "A review of recent development: Transport and performance modeling of PEM fuel cells," Applied Energy, Elsevier, vol. 165(C), pages 81-106.
    4. Siegel, C., 2008. "Review of computational heat and mass transfer modeling in polymer-electrolyte-membrane (PEM) fuel cells," Energy, Elsevier, vol. 33(9), pages 1331-1352.
    5. Chen, Ben & Wang, Jun & Yang, Tianqi & Cai, Yonghua & Zhang, Caizhi & Chan, Siew Hwa & Yu, Yi & Tu, Zhengkai, 2016. "Carbon corrosion and performance degradation mechanism in a proton exchange membrane fuel cell with dead-ended anode and cathode," Energy, Elsevier, vol. 106(C), pages 54-62.
    6. Thomas, Sobi & Bates, Alex & Park, Sam & Sahu, A.K. & Lee, Sang C. & Son, Byung Rak & Kim, Joo Gon & Lee, Dong-Ha, 2016. "An experimental and simulation study of novel channel designs for open-cathode high-temperature polymer electrolyte membrane fuel cells," Applied Energy, Elsevier, vol. 165(C), pages 765-776.
    7. Rostami, Leila & Mohamad Gholy Nejad, Puriya & Vatani, Ali, 2016. "A numerical investigation of serpentine flow channel with different bend sizes in polymer electrolyte membrane fuel cells," Energy, Elsevier, vol. 97(C), pages 400-410.
    8. Abdollahzadeh, M. & Pascoa, J.C. & Ranjbar, A.A. & Esmaili, Q., 2014. "Analysis of PEM (Polymer Electrolyte Membrane) fuel cell cathode two-dimensional modeling," Energy, Elsevier, vol. 68(C), pages 478-494.
    9. Karvelas, E.G. & Koubogiannis, D.G. & Hatziapostolou, A. & Sarris, I.E., 2016. "The effect of anode bed geometry on the hydraulic behaviour of PEM fuel cells," Renewable Energy, Elsevier, vol. 93(C), pages 269-279.
    10. Salva, J. Antonio & Iranzo, Alfredo & Rosa, Felipe & Tapia, Elvira, 2016. "Validation of cell voltage and water content in a PEM (polymer electrolyte membrane) fuel cell model using neutron imaging for different operating conditions," Energy, Elsevier, vol. 101(C), pages 100-112.
    11. Unknown, 2004. "End Materials," Choices: The Magazine of Food, Farm, and Resource Issues, Agricultural and Applied Economics Association, vol. 19(4), pages 1-1.
    12. Iranzo, Alfredo & Boillat, Pierre & Biesdorf, Johannes & Salva, Antonio, 2015. "Investigation of the liquid water distributions in a 50 cm2 PEM fuel cell: Effects of reactants relative humidity, current density, and cathode stoichiometry," Energy, Elsevier, vol. 82(C), pages 914-921.
    13. Damian-Ascencio, Cesar E. & Saldaña-Robles, Adriana & Hernandez-Guerrero, Abel & Cano-Andrade, Sergio, 2017. "Numerical modeling of a proton exchange membrane fuel cell with tree-like flow field channels based on an entropy generation analysis," Energy, Elsevier, vol. 133(C), pages 306-316.
    14. Andersson, M. & Beale, S.B. & Espinoza, M. & Wu, Z. & Lehnert, W., 2016. "A review of cell-scale multiphase flow modeling, including water management, in polymer electrolyte fuel cells," Applied Energy, Elsevier, vol. 180(C), pages 757-778.
    15. Hong, Po & Xu, Liangfei & Li, Jianqiu & Ouyang, Minggao, 2017. "Modeling of membrane electrode assembly of PEM fuel cell to analyze voltage losses inside," Energy, Elsevier, vol. 139(C), pages 277-288.
    16. Xing, Lei & Liu, Xiaoteng & Alaje, Taiwo & Kumar, Ravi & Mamlouk, Mohamed & Scott, Keith, 2014. "A two-phase flow and non-isothermal agglomerate model for a proton exchange membrane (PEM) fuel cell," Energy, Elsevier, vol. 73(C), pages 618-634.
    17. Carton, J.G. & Olabi, A.G., 2017. "Three-dimensional proton exchange membrane fuel cell model: Comparison of double channel and open pore cellular foam flow plates," Energy, Elsevier, vol. 136(C), pages 185-195.
    18. Lin, R. & Ren, Y.S. & Lin, X.W. & Jiang, Z.H. & Yang, Z. & Chang, Y.T., 2017. "Investigation of the internal behavior in segmented PEMFCs of different flow fields during cold start process," Energy, Elsevier, vol. 123(C), pages 367-377.
    19. Carton, J.G. & Lawlor, V. & Olabi, A.G. & Hochenauer, C. & Zauner, G., 2012. "Water droplet accumulation and motion in PEM (Proton Exchange Membrane) fuel cell mini-channels," Energy, Elsevier, vol. 39(1), pages 63-73.
    20. Wang, Junye, 2015. "Theory and practice of flow field designs for fuel cell scaling-up: A critical review," Applied Energy, Elsevier, vol. 157(C), pages 640-663.
    21. Mortazavi, Mehdi & Tajiri, Kazuya, 2015. "Two-phase flow pressure drop in flow channels of proton exchange membrane fuel cells: Review of experimental approaches," Renewable and Sustainable Energy Reviews, Elsevier, vol. 45(C), pages 296-317.
    22. Afshari, E. & Mosharaf-Dehkordi, M. & Rajabian, H., 2017. "An investigation of the PEM fuel cells performance with partially restricted cathode flow channels and metal foam as a flow distributor," Energy, Elsevier, vol. 118(C), pages 705-715.
    23. Xing, Lei & Du, Shangfeng & Chen, Rui & Mamlouk, Mohamed & Scott, Keith, 2016. "Anode partial flooding modelling of proton exchange membrane fuel cells: Model development and validation," Energy, Elsevier, vol. 96(C), pages 80-95.
    24. Ramiar, A. & Mahmoudi, A.H. & Esmaili, Q. & Abdollahzadeh, M., 2016. "Influence of cathode flow pulsation on performance of proton exchange membrane fuel cell with interdigitated gas distributors," Energy, Elsevier, vol. 94(C), pages 206-217.
    25. Xing, Lei & Cai, Qiong & Xu, Chenxi & Liu, Chunbo & Scott, Keith & Yan, Yongsheng, 2016. "Numerical study of the effect of relative humidity and stoichiometric flow ratio on PEM (proton exchange membrane) fuel cell performance with various channel lengths: An anode partial flooding modelli," Energy, Elsevier, vol. 106(C), pages 631-645.
    26. Li, Wenkai & Zhang, Qinglei & Wang, Chao & Yan, Xiaohui & Shen, Shuiyun & Xia, Guofeng & Zhu, Fengjuan & Zhang, Junliang, 2017. "Experimental and numerical analysis of a three-dimensional flow field for PEMFCs," Applied Energy, Elsevier, vol. 195(C), pages 278-288.
    Full references (including those not matched with items on IDEAS)

    Citations

    Citations are extracted by the CitEc Project, subscribe to its RSS feed for this item.
    as


    Cited by:

    1. Hwang, Jenn-Jiang & Dlamini, Mangaliso Menzi & Weng, Fang-Bor & Chang, Tseng & Lin, Chih-Hong & Weng, Shih-Cheng, 2022. "Simulation of fine mesh implementation on the cathode for proton exchange membrane fuel cell (PEMFC)," Energy, Elsevier, vol. 244(PA).
    2. Jiang, Ke & Zhao, Taotao & Fan, Wenxuan & Liu, Zhenning & Lu, Guolong, 2023. "Ramped step flow field to enhance mass transfer capacity and performance for PEMFC," Renewable Energy, Elsevier, vol. 219(P2).
    3. Yin, Yan & Wu, Shiyu & Qin, Yanzhou & Otoo, Obed Nenyi & Zhang, Junfeng, 2020. "Quantitative analysis of trapezoid baffle block sloping angles on oxygen transport and performance of proton exchange membrane fuel cell," Applied Energy, Elsevier, vol. 271(C).
    4. Liao, Shuxin & Qiu, Diankai & Yi, Peiyun & Peng, Linfa & Lai, Xinmin, 2022. "Modeling of a novel cathode flow field design with optimized sub-channels to improve drainage for proton exchange membrane fuel cells," Energy, Elsevier, vol. 261(PB).
    5. Najmi, Aezid-Ul-Hassan & Anyanwu, Ikechukwu S. & Xie, Xu & Liu, Zhi & Jiao, Kui, 2021. "Experimental investigation and optimization of proton exchange membrane fuel cell using different flow fields," Energy, Elsevier, vol. 217(C).
    6. Xiong, Kangning & Wu, Wei & Wang, Shuangfeng & Zhang, Lin, 2021. "Modeling, design, materials and fabrication of bipolar plates for proton exchange membrane fuel cell: A review," Applied Energy, Elsevier, vol. 301(C).
    7. Perng, Shiang-Wuu & Wu, Horng-Wen, 2022. "Influence of inlet-nozzle and outlet-diffuser mounted in the plate-shape reactor on PEMFC net power output and methanol steam reforming performance," Applied Energy, Elsevier, vol. 323(C).
    8. Zhou, Yu & Chen, Ben, 2023. "Investigation of optimization and evaluation criteria for flow field in proton exchange membrane fuel cell: A critical review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 185(C).
    9. Suprava Chakraborty & Devaraj Elangovan & Karthikeyan Palaniswamy & Ashley Fly & Dineshkumar Ravi & Denis Ashok Sathia Seelan & Thundil Karuppa Raj Rajagopal, 2022. "A Review on the Numerical Studies on the Performance of Proton Exchange Membrane Fuel Cell (PEMFC) Flow Channel Designs for Automotive Applications," Energies, MDPI, vol. 15(24), pages 1-21, December.

    Most related items

    These are the items that most often cite the same works as this one and are cited by the same works as this one.
    1. Xu, Liangfei & Fang, Chuan & Hu, Junming & Cheng, Siliang & Li, Jianqiu & Ouyang, Minggao & Lehnert, Werner, 2017. "Parameter extraction of polymer electrolyte membrane fuel cell based on quasi-dynamic model and periphery signals," Energy, Elsevier, vol. 122(C), pages 675-690.
    2. Abdollahzadeh, M. & Ribeirinha, P. & Boaventura, M. & Mendes, A., 2018. "Three-dimensional modeling of PEMFC with contaminated anode fuel," Energy, Elsevier, vol. 152(C), pages 939-959.
    3. Hu, Junming & Li, Jianqiu & Xu, Liangfei & Huang, Fusen & Ouyang, Minggao, 2016. "Analytical calculation and evaluation of water transport through a proton exchange membrane fuel cell based on a one-dimensional model," Energy, Elsevier, vol. 111(C), pages 869-883.
    4. Xiong, Kangning & Wu, Wei & Wang, Shuangfeng & Zhang, Lin, 2021. "Modeling, design, materials and fabrication of bipolar plates for proton exchange membrane fuel cell: A review," Applied Energy, Elsevier, vol. 301(C).
    5. Suprava Chakraborty & Devaraj Elangovan & Karthikeyan Palaniswamy & Ashley Fly & Dineshkumar Ravi & Denis Ashok Sathia Seelan & Thundil Karuppa Raj Rajagopal, 2022. "A Review on the Numerical Studies on the Performance of Proton Exchange Membrane Fuel Cell (PEMFC) Flow Channel Designs for Automotive Applications," Energies, MDPI, vol. 15(24), pages 1-21, December.
    6. Ashrafi, Moosa & Kanani, Homayoon & Shams, Mehrzad, 2018. "Numerical and experimental study of two-phase flow uniformity in channels of parallel PEM fuel cells with modified Z-type flow-fields," Energy, Elsevier, vol. 147(C), pages 317-328.
    7. Yin, Cong & Gao, Jianlong & Wen, Xuhui & Xie, Guangyou & Yang, Chunhua & Fang, Honglin & Tang, Hao, 2016. "In situ investigation of proton exchange membrane fuel cell performance with novel segmented cell design and a two-phase flow model," Energy, Elsevier, vol. 113(C), pages 1071-1089.
    8. Abdin, Z. & Webb, C.J. & Gray, E.MacA., 2016. "PEM fuel cell model and simulation in Matlab–Simulink based on physical parameters," Energy, Elsevier, vol. 116(P1), pages 1131-1144.
    9. Salva, J. Antonio & Iranzo, Alfredo & Rosa, Felipe & Tapia, Elvira, 2016. "Validation of cell voltage and water content in a PEM (polymer electrolyte membrane) fuel cell model using neutron imaging for different operating conditions," Energy, Elsevier, vol. 101(C), pages 100-112.
    10. Xing, Lei & Cai, Qiong & Xu, Chenxi & Liu, Chunbo & Scott, Keith & Yan, Yongsheng, 2016. "Numerical study of the effect of relative humidity and stoichiometric flow ratio on PEM (proton exchange membrane) fuel cell performance with various channel lengths: An anode partial flooding modelli," Energy, Elsevier, vol. 106(C), pages 631-645.
    11. Afshari, E. & Mosharaf-Dehkordi, M. & Rajabian, H., 2017. "An investigation of the PEM fuel cells performance with partially restricted cathode flow channels and metal foam as a flow distributor," Energy, Elsevier, vol. 118(C), pages 705-715.
    12. Ijaodola, O.S. & El- Hassan, Zaki & Ogungbemi, E. & Khatib, F.N. & Wilberforce, Tabbi & Thompson, James & Olabi, A.G., 2019. "Energy efficiency improvements by investigating the water flooding management on proton exchange membrane fuel cell (PEMFC)," Energy, Elsevier, vol. 179(C), pages 246-267.
    13. Atyabi, Seyed Ali & Afshari, Ebrahim & Wongwises, Somchai & Yan, Wen-Mon & Hadjadj, Abdellah & Shadloo, Mostafa Safdari, 2019. "Effects of assembly pressure on PEM fuel cell performance by taking into accounts electrical and thermal contact resistances," Energy, Elsevier, vol. 179(C), pages 490-501.
    14. Liu, Yongfeng & Wang, Na & Pei, Pucheng & Yao, Shengzhuo & Wang, Fang, 2018. "Asymptotic analysis of anode relative humidity effects on the fastest voltage decay single cell in a stack," Energy, Elsevier, vol. 151(C), pages 490-500.
    15. Ismail, M.S. & Ingham, D.B. & Ma, L. & Hughes, K.J. & Pourkashanian, M., 2017. "Effects of catalyst agglomerate shape in polymer electrolyte fuel cells investigated by a multi-scale modelling framework," Energy, Elsevier, vol. 122(C), pages 420-430.
    16. Tzelepis, Stefanos & Kavadias, Kosmas A. & Marnellos, George E. & Xydis, George, 2021. "A review study on proton exchange membrane fuel cell electrochemical performance focusing on anode and cathode catalyst layer modelling at macroscopic level," Renewable and Sustainable Energy Reviews, Elsevier, vol. 151(C).
    17. Ozen, Dilek Nur & Timurkutluk, Bora & Altinisik, Kemal, 2016. "Effects of operation temperature and reactant gas humidity levels on performance of PEM fuel cells," Renewable and Sustainable Energy Reviews, Elsevier, vol. 59(C), pages 1298-1306.
    18. Sadiq T. Bunyan & Hayder A. Dhahad & Dhamyaa S. Khudhur & Talal Yusaf, 2023. "The Effect of Flow Field Design Parameters on the Performance of PEMFC: A Review," Sustainability, MDPI, vol. 15(13), pages 1-62, June.
    19. Barzegari, Mohammad M. & Dardel, Morteza & Alizadeh, Ebrahim & Ramiar, Abas, 2016. "Reduced-order model of cascade-type PEM fuel cell stack with integrated humidifiers and water separators," Energy, Elsevier, vol. 113(C), pages 683-692.
    20. Afra, Mehran & Nazari, Mohsen & Kayhani, Mohammad Hasan & Sharifpur, M. & Meyer, J.P., 2019. "3D experimental visualization of water flooding in proton exchange membrane fuel cells," Energy, Elsevier, vol. 175(C), pages 967-977.

    Corrections

    All material on this site has been provided by the respective publishers and authors. You can help correct errors and omissions. When requesting a correction, please mention this item's handle: RePEc:eee:energy:v:161:y:2018:i:c:p:104-117. See general information about how to correct material in RePEc.

    If you have authored this item and are not yet registered with RePEc, we encourage you to do it here. This allows to link your profile to this item. It also allows you to accept potential citations to this item that we are uncertain about.

    If CitEc recognized a bibliographic reference but did not link an item in RePEc to it, you can help with this form .

    If you know of missing items citing this one, you can help us creating those links by adding the relevant references in the same way as above, for each refering item. If you are a registered author of this item, you may also want to check the "citations" tab in your RePEc Author Service profile, as there may be some citations waiting for confirmation.

    For technical questions regarding this item, or to correct its authors, title, abstract, bibliographic or download information, contact: Catherine Liu (email available below). General contact details of provider: http://www.journals.elsevier.com/energy .

    Please note that corrections may take a couple of weeks to filter through the various RePEc services.

    IDEAS is a RePEc service. RePEc uses bibliographic data supplied by the respective publishers.