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Catalytic methanation of carbon dioxide captured from ambient air

Author

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  • Veselovskaya, Janna V.
  • Parunin, Pavel D.
  • Netskina, Olga V.
  • Kibis, Lidiya S.
  • Lysikov, Anton I.
  • Okunev, Aleksey G.

Abstract

A novel process, combining direct CO2 capture from ambient air using K2CO3/Al2O3 composite sorbent and CO2 methanation in the presence of 4% Ru/Al2O3 catalyst, has been developed and tested in a cyclic mode. The thermal regeneration of the composite sorbent in these cycles has been carried out in H2 atmosphere at T = 325 °C with the gas flow going straight from the adsorber outlet to the preheated catalytic reactor. Performance of the ruthenium catalyst in CO2 methanation process has improved upon cycling, apparently due to in situ activation of the supported component. Activation of the catalyst has been studied in a gaseous mixture of CO2 and H2 (1:4) at 300 °C. The activation of the catalyst in reductive atmosphere leads to transformation of Ru4+ surface species to Ru0 particles, identified by means of X-ray photoelectron spectroscopy and high-resolution transmission electron microscopy. It has been demonstrated that it is possible to transform the desorbed carbon dioxide to methane with conversion >98% at T = 325–400 °C using the activated Ru/Al2O3 catalyst.

Suggested Citation

  • Veselovskaya, Janna V. & Parunin, Pavel D. & Netskina, Olga V. & Kibis, Lidiya S. & Lysikov, Anton I. & Okunev, Aleksey G., 2018. "Catalytic methanation of carbon dioxide captured from ambient air," Energy, Elsevier, vol. 159(C), pages 766-773.
    • Handle: RePEc:eee:energy:v:159:y:2018:i:c:p:766-773
    DOI: 10.1016/j.energy.2018.06.180
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    References listed on IDEAS

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    1. Suciu, Raluca & Girardin, Luc & Maréchal, François, 2018. "Energy integration of CO2 networks and power to gas for emerging energy autonomous cities in Europe," Energy, Elsevier, vol. 157(C), pages 830-842.
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    3. Yaumi, A.L. & Bakar, M.Z. Abu & Hameed, B.H., 2017. "Recent advances in functionalized composite solid materials for carbon dioxide capture," Energy, Elsevier, vol. 124(C), pages 461-480.
    4. Kirchbacher, Florian & Biegger, Philipp & Miltner, Martin & Lehner, Markus & Harasek, Michael, 2018. "A new methanation and membrane based power-to-gas process for the direct integration of raw biogas – Feasability and comparison," Energy, Elsevier, vol. 146(C), pages 34-46.
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    Cited by:

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    2. Mejía-Botero, Cristian & Echeverri-Uribe, Camilo & Ferrer-Ruiz, Juan E. & Amell, Andrés A., 2023. "Effect of preheat temperature, pressure, and residence time on methanation performance," Energy, Elsevier, vol. 269(C).
    3. Chistyakov, A.V. & Nikolaev, S.A. & Zharova, P.A. & Tsodikov, M.V. & Manenti, F., 2019. "Linear α-alcohols production from supercritical ethanol over Cu/Al2O3 catalyst," Energy, Elsevier, vol. 166(C), pages 569-576.
    4. Ye, Run-Ping & Gong, Weibo & Sun, Zhao & Sheng, Qingtao & Shi, Xiufeng & Wang, Tongtong & Yao, Yi & Razink, Joshua J. & Lin, Ling & Zhou, Zhangfeng & Adidharma, Hertanto & Tang, Jinke & Fan, Maohong &, 2019. "Enhanced stability of Ni/SiO2 catalyst for CO2 methanation: Derived from nickel phyllosilicate with strong metal-support interactions," Energy, Elsevier, vol. 188(C).

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