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Catalytic conversion of waste cooking oil to fuel oil: Catalyst design and effect of solvent

Author

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  • Li, Zhixia
  • Huang, Zhentao
  • Ding, Shilei
  • Li, Fuwei
  • Wang, Zhaohe
  • Lin, Hongfei
  • Chen, Congjin

Abstract

Waste cooking oil (WCO) is dispersed in tetralin or dodecane and hydrotreated in a batch reactor over a fabricated NiMo/γ-Al2O3-β-zeolite catalyst. The properties of catalysts are controlled by adjusting the mass fraction of β-zeolite in support (x), the mass fraction of NiO and MoO3 (m) and Ni/(Ni + Mo) mol fraction (y) in catalysts. The effects of the catalytic properties, solvents and reaction conditions on the hydrodeoxygenation of WCO are investigated. The results showed that increasing m and y promoted WCO conversion and the formation of alkane hydrocarbons; the addition of Ni into Mo helped to promote the reducing ability of catalysts and enhanced deoxygenation via decarboxylation/decarbonylation pathway. An increase in β-zeolite was unfavourable for WCO conversion. A complete conversion of WCO to hydrocarbons was achieved at 350 °C under H2 at 5 MPa for 3 h with dodecane as solvent. The isomerized compounds accounted for less than 10 wt%. A low H2 pressure is suitable for tetralin exerting hydrogen-donating effect.

Suggested Citation

  • Li, Zhixia & Huang, Zhentao & Ding, Shilei & Li, Fuwei & Wang, Zhaohe & Lin, Hongfei & Chen, Congjin, 2018. "Catalytic conversion of waste cooking oil to fuel oil: Catalyst design and effect of solvent," Energy, Elsevier, vol. 157(C), pages 270-277.
    • Handle: RePEc:eee:energy:v:157:y:2018:i:c:p:270-277
    DOI: 10.1016/j.energy.2018.05.156
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