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Study on susceptibility of CO2-assisted pyrolysis of various biomass to CO2

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  • Lee, Jechan
  • Oh, Jeong-Ik
  • Ok, Yong Sik
  • Kwon, Eilhann E.

Abstract

This study systematically investigates simultaneous genuine roles of CO2 in pyrolysis process by comparing the susceptibility of pyrolysis of various biomass feedstocks (spent coffee ground, oak wood, corn stover, macroalgae, microalgae, cellulose, hemicellulose, and lignin) to CO2: 1) the enhanced thermal cracking of volatile organic carbons (VOCs) evolved from the thermal decomposition of biomass and 2) the direct reaction between VOCs and CO2. The identified roles of CO2 led to the enhanced generation of CO and the subsequent reduction of condensable tar. Even though the influence of CO2 on pyrolysis of various biomass and coal was universal, it exhibited a different magnitude due to the different susceptibility to CO2. This study also reports that the susceptibility to CO2 was contingent on the lignin content in biomass.

Suggested Citation

  • Lee, Jechan & Oh, Jeong-Ik & Ok, Yong Sik & Kwon, Eilhann E., 2017. "Study on susceptibility of CO2-assisted pyrolysis of various biomass to CO2," Energy, Elsevier, vol. 137(C), pages 510-517.
    • Handle: RePEc:eee:energy:v:137:y:2017:i:c:p:510-517
    DOI: 10.1016/j.energy.2017.01.155
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    References listed on IDEAS

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    7. Lee, Jechan & Yang, Xiao & Cho, Seong-Heon & Kim, Jae-Kon & Lee, Sang Soo & Tsang, Daniel C.W. & Ok, Yong Sik & Kwon, Eilhann E., 2017. "Pyrolysis process of agricultural waste using CO2 for waste management, energy recovery, and biochar fabrication," Applied Energy, Elsevier, vol. 185(P1), pages 214-222.
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    4. Jung, Sungyup & Jung, Jong-Min & Tsang, Yiu Fai & Bhatnagar, Amit & Chen, Wei-Hsin & Lin, Kun-Yi Andrew & Kwon, Eilhann E., 2022. "Biodiesel production from black soldier fly larvae derived from food waste by non-catalytic transesterification," Energy, Elsevier, vol. 238(PA).
    5. Jung, Jong-Min & Kim, Sok & Lee, Jechan & Oh, Jeong Ik & Choi, Yoon-E. & Kwon, Eilhann E., 2019. "Tailoring pyrogenic products from pyrolysis of defatted Euglena gracilis using CO2 as reactive gas medium," Energy, Elsevier, vol. 174(C), pages 184-190.
    6. Kwon, Dohee & Kim, Youngju & Choi, Dongho & Jung, Sungyup & Tsang, Yiu Fai & Kwon, Eilhann E., 2024. "Enhanced thermochemical valorization of coconut husk through carbon dioxide integration: A sustainable approach to agricultural residue utilization," Applied Energy, Elsevier, vol. 369(C).
    7. Jung, Sungyup & Kwon, Dohee & Park, Young-Kwon & Lee, Kyun Ho & Kwon, Eilhann E., 2020. "Power generation using rice husk derived fuels from CO2-assisted catalytic pyrolysis over Co/Al2O3," Energy, Elsevier, vol. 206(C).
    8. Park, Jonghyun & Yim, Jun Ho & Cho, Seong-Heon & Jung, Sungyup & Tsang, Yiu Fai & Chen, Wei-Hsin & Jeon, Young Jae & Kwon, Eilhann E., 2024. "A virtuous cycle for thermal treatment of polyvinyl chloride and fermentation of lignocellulosic biomass," Applied Energy, Elsevier, vol. 362(C).

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