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Comparative study of alkaline water electrolysis, proton exchange membrane water electrolysis and solid oxide electrolysis through multiphysics modeling

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  • Hu, Kewei
  • Fang, Jiakun
  • Ai, Xiaomeng
  • Huang, Danji
  • Zhong, Zhiyao
  • Yang, Xiaobo
  • Wang, Lei

Abstract

This paper provides a comparative study of alkaline water electrolysis (AE), proton exchange membrane water electrolysis (PEM) and solid oxide electrolysis cells (SOEC) through multiphysics modeling. A unified multiphysics model for the three types of electrolyzers, considering current density distribution, single-phase and diphasic flow, mass transfer and temperature dependence in the electrolyzers, is derived to make a thorough interpretation of their differences in terms of I-V characteristics, cell efficiency and part-load performances. Besides, various definitions of electrolysis efficiency from different researches on PtH are compared and evaluated from thermodynamics to unify the definitions of efficiency. Main drawbacks of the cell performances are then reviewed respectively to explain the parametric gap among three types of water electrolysis.

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  • Hu, Kewei & Fang, Jiakun & Ai, Xiaomeng & Huang, Danji & Zhong, Zhiyao & Yang, Xiaobo & Wang, Lei, 2022. "Comparative study of alkaline water electrolysis, proton exchange membrane water electrolysis and solid oxide electrolysis through multiphysics modeling," Applied Energy, Elsevier, vol. 312(C).
    • Handle: RePEc:eee:appene:v:312:y:2022:i:c:s0306261922002367
    DOI: 10.1016/j.apenergy.2022.118788
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    1. Takaya Ogawa & Mizutomo Takeuchi & Yuya Kajikawa, 2018. "Analysis of Trends and Emerging Technologies in Water Electrolysis Research Based on a Computational Method: A Comparison with Fuel Cell Research," Sustainability, MDPI, vol. 10(2), pages 1-24, February.
    2. Buttler, Alexander & Spliethoff, Hartmut, 2018. "Current status of water electrolysis for energy storage, grid balancing and sector coupling via power-to-gas and power-to-liquids: A review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 82(P3), pages 2440-2454.
    3. Götz, Manuel & Lefebvre, Jonathan & Mörs, Friedemann & McDaniel Koch, Amy & Graf, Frank & Bajohr, Siegfried & Reimert, Rainer & Kolb, Thomas, 2016. "Renewable Power-to-Gas: A technological and economic review," Renewable Energy, Elsevier, vol. 85(C), pages 1371-1390.
    4. Srikanth, S. & Heddrich, M.P. & Gupta, S. & Friedrich, K.A., 2018. "Transient reversible solid oxide cell reactor operation – Experimentally validated modeling and analysis," Applied Energy, Elsevier, vol. 232(C), pages 473-488.
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    2. Li, Yuxuan & Li, Hongkun & Liu, Weiqun & Zhu, Qiao, 2024. "Optimization of membrane thickness for proton exchange membrane electrolyzer considering hydrogen production efficiency and hydrogen permeation phenomenon," Applied Energy, Elsevier, vol. 355(C).
    3. Karthikeyan, B. & Praveen Kumar, G. & Narayanan, Ramadas & R, Saravanan & Coronas, Alberto, 2024. "Thermo-economic optimization of hybrid solar-biomass driven organic rankine cycle integrated heat pump and PEM electrolyser for combined power, heating, and green hydrogen applications," Energy, Elsevier, vol. 299(C).
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    5. del Pozo Gonzalez, Hector & Bernadet, Lucile & Torrell, Marc & Bianchi, Fernando D. & Tarancón, Albert & Gomis-Bellmunt, Oriol & Dominguez-Garcia, Jose Luis, 2023. "Power transition cycles of reversible solid oxide cells and its impacts on microgrids," Applied Energy, Elsevier, vol. 352(C).
    6. Wang, Jianxiao & An, Qi & Zhao, Yue & Pan, Guangsheng & Song, Jie & Hu, Qinran & Tan, Chin-Woo, 2023. "Role of electrolytic hydrogen in smart city decarbonization in China," Applied Energy, Elsevier, vol. 336(C).
    7. Xu, Chenyang & Wang, Jian & Wang, Jianzhong & Yang, Kun & Li, Guangzhong & Gao, Wenbin & Wang, Hao & Zhao, Shaoyang, 2024. "Structural optimization study on porous transport layers of sintered titanium for polymer electrolyte membrane electrolyzers," Applied Energy, Elsevier, vol. 357(C).
    8. Kumar, S. Shiva & Ni, Aleksey & Himabindu, V. & Lim, Hankwon, 2023. "Experimental and simulation of PEM water electrolyser with Pd/PN-CNPs electrodes for hydrogen evolution reaction: Performance assessment and validation," Applied Energy, Elsevier, vol. 348(C).
    9. Huang, Danji & Xiong, Binyu & Fang, Jiakun & Hu, Kewei & Zhong, Zhiyao & Ying, Yuheng & Ai, Xiaomeng & Chen, Zhe, 2022. "A multiphysics model of the compactly-assembled industrial alkaline water electrolysis cell," Applied Energy, Elsevier, vol. 314(C).
    10. Hu, Song & Guo, Bin & Ding, Shunliang & Yang, Fuyuan & Dang, Jian & Liu, Biao & Gu, Junjie & Ma, Jugang & Ouyang, Minggao, 2022. "A comprehensive review of alkaline water electrolysis mathematical modeling," Applied Energy, Elsevier, vol. 327(C).
    11. Dong, Tianshu & Duan, Xiudong & Huang, Yuanyuan & Huang, Danji & Luo, Yingdong & Liu, Ziyu & Ai, Xiaomeng & Fang, Jiakun & Song, Chaolong, 2024. "Enhancement of hydrogen production via optimizing micro-structures of electrolyzer on a microfluidic platform," Applied Energy, Elsevier, vol. 356(C).
    12. Mohsen Fallah Vostakola & Hasan Ozcan & Rami S. El-Emam & Bahman Amini Horri, 2023. "Recent Advances in High-Temperature Steam Electrolysis with Solid Oxide Electrolysers for Green Hydrogen Production," Energies, MDPI, vol. 16(8), pages 1-50, April.

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