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Plastic/rubber waste-templated carbide slag pellets for regenerable CO2 capture at elevated temperature

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  • Sun, Jian
  • Sun, Yu
  • Yang, Yuandong
  • Tong, Xianliang
  • Liu, Wenqiang

Abstract

Plastic/rubber waste-templated carbide slag pellets were prepared via an extrusion-spheronization method for high-temperature CO2 capture. Four types of common plastic and rubber wastes (i.e. waste plastic bottle composed of polyethylene terephthalate, disposable plastic cup composed of polypropylene, waste plastic pipe composed of polyvinyl chloride and scrap tire composed of rubber, sulfur and carbon black) were selected as the templating materials. It is found that the addition of waste plastic pipe can cause inferior CO2 capture performance for carbide slag pellets (merely 0.123 g CO2/g sorbent after 25 cycles). It is mainly attributed to the deactivation of carbide slag pellets as a result of the interaction between CaO and the chlorine released from waste plastic pipe. The other chlorine-free plastic and rubber wastes are effective to improve the cyclic CO2 capture performance of carbide slag pellets via altering their porosities. Particularly, the carbide slag pellets doped with 5 wt% of waste plastic bottle exhibit the highest CO2 capture capacity of 0.277 g CO2/g sorbent after 25 cycles, compared to 0.218 g CO2/g sorbent for carbide slag pellets. Moreover, the pre-calcination atmosphere plays an important role on the cyclic CO2 uptake of plastic/rubber waste-templated pellets. The CO2 capture capability of plastic/rubber waste-templated pellets pre-calcined in air is inferior to that pre-calcined in N2. It is mainly due to the heat released from the combustion of plastic or rubber wastes in air accelerates severe sintering for the plastic/rubber waste-templated carbide slag pellets.

Suggested Citation

  • Sun, Jian & Sun, Yu & Yang, Yuandong & Tong, Xianliang & Liu, Wenqiang, 2019. "Plastic/rubber waste-templated carbide slag pellets for regenerable CO2 capture at elevated temperature," Applied Energy, Elsevier, vol. 242(C), pages 919-930.
    • Handle: RePEc:eee:appene:v:242:y:2019:i:c:p:919-930
    DOI: 10.1016/j.apenergy.2019.03.165
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    References listed on IDEAS

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    1. Su, Chenglin & Duan, Lunbo & Donat, Felix & Anthony, Edward John, 2018. "From waste to high value utilization of spent bleaching clay in synthesizing high-performance calcium-based sorbent for CO2 capture," Applied Energy, Elsevier, vol. 210(C), pages 117-126.
    2. Ma, Xiaotong & Li, Yingjie & Duan, Lunbo & Anthony, Edward & Liu, Hantao, 2018. "CO2 capture performance of calcium-based synthetic sorbent with hollow core-shell structure under calcium looping conditions," Applied Energy, Elsevier, vol. 225(C), pages 402-412.
    3. Erans, María & Manovic, Vasilije & Anthony, Edward J., 2016. "Calcium looping sorbents for CO2 capture," Applied Energy, Elsevier, vol. 180(C), pages 722-742.
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    1. Ying Yang & Yingjie Li & Xianyao Yan & Jianli Zhao & Chunxiao Zhang, 2021. "Development of Thermochemical Heat Storage Based on CaO/CaCO 3 Cycles: A Review," Energies, MDPI, vol. 14(20), pages 1-26, October.
    2. Chaoying Sun & Xianyao Yan & Yingjie Li & Jianli Zhao & Zeyan Wang & Tao Wang, 2020. "Coupled CO2 capture and thermochemical heat storage of CaO derived from calcium acetate," Greenhouse Gases: Science and Technology, Blackwell Publishing, vol. 10(5), pages 1027-1038, October.
    3. Sun, Hao & Li, Yingjie & Yan, Xianyao & Zhao, Jianli & Wang, Zeyan, 2020. "Thermochemical energy storage performance of Al2O3/CeO2 co-doped CaO-based material under high carbonation pressure," Applied Energy, Elsevier, vol. 263(C).
    4. Gong, Xuzhong & Zhang, Tong & Zhang, Junqiang & Wang, Zhi & Liu, Junhao & Cao, Jianwei & Wang, Chuan, 2022. "Recycling and utilization of calcium carbide slag - current status and new opportunities," Renewable and Sustainable Energy Reviews, Elsevier, vol. 159(C).

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