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Ag-graphene/PEG composite phase change materials for enhancing solar-thermal energy conversion and storage capacity

Author

Listed:
  • Zhang, Yuang
  • Wang, Jiasheng
  • Qiu, Jinjing
  • Jin, Xin
  • Umair, Malik Muhammad
  • Lu, Rongwen
  • Zhang, Shufen
  • Tang, Bingtao

Abstract

In view of the excellent characteristic of thermal energy storage, phase change materials (PCMs) are of great significance for improving the efficiency of solar thermal energy utilization. However, the direct thermal effect of visible-light (40% of solar radiation) is very low. In order to improve the capabilities of visible-light absorption and photothermal conversion, we reported novel and efficient sunlight-driven PCMs based on polyethylene glycol (PEG) supported by Ag nanoparticle-functionalized graphene nanosheets (Ag–GNS). The multi-folded layered structure provides Ag–GNS a large surface area to support PEG for achieving the shape stability before and after phase transition. Meanwhile, based on the local surface plasma resonance effect of Ag, Ag has high visible light selective absorption and infrared reflectance, which can give Ag–GNS enhanced light absorption capacity and reduced thermal radiation. So Ag–GNS/PEG can harvest sunlight and convert light to thermal energy with significantly higher efficiency (η = 88.7–92.0%). Moreover, Ag–GNS/PEG composites exhibit enhanced thermal conductivities (49.5–95.3%), high energy storage densities (>166.1 J/g), high thermal energy storage/release rates and outstanding form-stable properties. Therefore, this novel sunlight-driven composite can be potentially used for clean and efficient utilization of solar energy.

Suggested Citation

  • Zhang, Yuang & Wang, Jiasheng & Qiu, Jinjing & Jin, Xin & Umair, Malik Muhammad & Lu, Rongwen & Zhang, Shufen & Tang, Bingtao, 2019. "Ag-graphene/PEG composite phase change materials for enhancing solar-thermal energy conversion and storage capacity," Applied Energy, Elsevier, vol. 237(C), pages 83-90.
    • Handle: RePEc:eee:appene:v:237:y:2019:i:c:p:83-90
    DOI: 10.1016/j.apenergy.2018.12.075
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    References listed on IDEAS

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    8. Wang, Chengjun & Liang, Weidong & Yang, Yueyue & Liu, Fang & Sun, Hanxue & Zhu, Zhaoqi & Li, An, 2020. "Biomass carbon aerogels based shape-stable phase change composites with high light-to-thermal efficiency for energy storage," Renewable Energy, Elsevier, vol. 153(C), pages 182-192.
    9. Yafang Zhang & Jiebin Tang & Jialin Chen & Yuhai Zhang & Xiangxiang Chen & Meng Ding & Weijia Zhou & Xijin Xu & Hong Liu & Guobin Xue, 2023. "Accelerating the solar-thermal energy storage via inner-light supplying with optical waveguide," Nature Communications, Nature, vol. 14(1), pages 1-10, December.
    10. Li, Chuan & Li, Qi & Cong, Lin & jiang, Feng & Zhao, Yanqi & Liu, Chuanping & Xiong, Yaxuan & Chang, Chun & Ding, Yulong, 2019. "MgO based composite phase change materials for thermal energy storage: The effects of MgO particle density and size on microstructural characteristics as well as thermophysical and mechanical properti," Applied Energy, Elsevier, vol. 250(C), pages 81-91.
    11. Wang, Yabo & Huang, Xinyu & Shu, Gao & Li, Xueqiang & Yang, Xiaohu, 2024. "Influence of microgravity on melting performance of a phase-change heat storage tank," Energy, Elsevier, vol. 289(C).
    12. Cao, Yufeng & Fan, Dongli & Lin, Shaohui & Ng, Flora T.T. & Pan, Qinmin, 2021. "Branched alkylated polynorbornene and 3D flower-like MoS2 nanospheres reinforced phase change composites with high thermal energy storage capacity and photothermal conversion efficiency," Renewable Energy, Elsevier, vol. 179(C), pages 687-695.
    13. Zhang, Hongyun & Wang, Lingling & Xi, Shaobo & Xie, Huaqing & Yu, Wei, 2021. "3D porous copper foam-based shape-stabilized composite phase change materials for high photothermal conversion, thermal conductivity and storage," Renewable Energy, Elsevier, vol. 175(C), pages 307-317.
    14. Jiang, Liang & Lei, Yuan & Liu, Qinfeng & Lei, Jingxin, 2020. "Polyethylene glycol based self-luminous phase change materials for both thermal and light energy storage," Energy, Elsevier, vol. 193(C).
    15. Bing, Naici & Yang, Jie & Gao, Huan & Xie, Huaqing & Yu, Wei, 2021. "Unsaturated polyester resin supported form-stable phase change materials with enhanced thermal conductivity for solar energy storage and conversion," Renewable Energy, Elsevier, vol. 173(C), pages 926-933.

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