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Experimental investigation of different factors influencing the replacement efficiency of CO2 for methane hydrate

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  • Chen, Ye
  • Gao, Yonghai
  • Zhao, Yipeng
  • Chen, Litao
  • Dong, Changyin
  • Sun, Baojiang

Abstract

The objective of this research is to study the replacement efficiency of methane hydrate with CO2, which is an important index to describe the use of CO2 for this application and to evaluate its economic benefits. An experimental study was designed to simulate the replacement of methane hydrate with CO2 in a low permeability, porous medium, and analyze the influence of different factors such as injection rate (0.5–1.5 ml/min), total amount (1.8–5.4 L), temperature (275–279 K) and pressure (3–5 MPa) by controlling these variables. The results indicated that the total amount at injection and the temperature had relatively significant impacts on the replacement efficiency. The CO2 injection rate and pressure primarily affected the CH4 production rate, rather than the total amount produced. The injection temperature and pressure should be comprehensively optimized for improved economic benefits. The ultimate replacement efficiency ranged from 22.9% to 44.6%, and the ultimate production ratio ranged from 3.35% to 13%, confirming the necessity of a comprehensive optimization of the influencing factors and implying that most of the large cavities had not yet been occupied by CO2.

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  • Chen, Ye & Gao, Yonghai & Zhao, Yipeng & Chen, Litao & Dong, Changyin & Sun, Baojiang, 2018. "Experimental investigation of different factors influencing the replacement efficiency of CO2 for methane hydrate," Applied Energy, Elsevier, vol. 228(C), pages 309-316.
    • Handle: RePEc:eee:appene:v:228:y:2018:i:c:p:309-316
    DOI: 10.1016/j.apenergy.2018.05.126
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    3. Gajanan, K. & Ranjith, P.G. & Yang, S.Q. & Xu, T., 2024. "Advances in research and developments on natural gas hydrate extraction with gas exchange," Renewable and Sustainable Energy Reviews, Elsevier, vol. 190(PB).
    4. Jyoti Shanker Pandey & Nicolas von Solms, 2019. "Hydrate Stability and Methane Recovery from Gas Hydrate through CH 4 –CO 2 Replacement in Different Mass Transfer Scenarios," Energies, MDPI, vol. 12(12), pages 1-20, June.
    5. Tsypkin, G.G., 2021. "Analytical study of CO2–CH4 exchange in hydrate at high rates of carbon dioxide injection into a reservoir saturated with methane hydrate and gaseous methane," Energy, Elsevier, vol. 233(C).
    6. Wang, Xiaolin & Zhang, Fengyuan & Lipiński, Wojciech, 2020. "Research progress and challenges in hydrate-based carbon dioxide capture applications," Applied Energy, Elsevier, vol. 269(C).
    7. Baicen Lin & Yunsheng Wei & Shusheng Gao & Liyou Ye & Huaxun Liu & Wenqing Zhu & Jianzhong Zhang & Donghuan Han, 2024. "Current Progress and Development Trend of Gas Injection to Enhance Gas Recovery in Gas Reservoirs," Energies, MDPI, vol. 17(7), pages 1-24, March.
    8. Sun, You-Hong & Zhang, Guo-Biao & Carroll, John J. & Li, Sheng-Li & Jiang, Shu-Hui & Guo, Wei, 2018. "Experimental investigation into gas recovery from CH4-C2H6-C3H8 hydrates by CO2 replacement," Applied Energy, Elsevier, vol. 229(C), pages 625-636.
    9. Le, Quang-Du & Rodriguez, Carla T. & Legoix, Ludovic N. & Pirim, Claire & Chazallon, Bertrand, 2020. "Influence of the initial CH4-hydrate system properties on CO2 capture kinetics," Applied Energy, Elsevier, vol. 280(C).
    10. Jyoti Shanker Pandey & Charilaos Karantonidis & Adam Paul Karcz & Nicolas von Solms, 2020. "Enhanced CH 4 -CO 2 Hydrate Swapping in the Presence of Low Dosage Methanol," Energies, MDPI, vol. 13(20), pages 1-30, October.
    11. Li, Yanghui & Wei, Zhaosheng & Wang, Haijun & Wu, Peng & Zhang, Shuheng & You, Zeshao & Liu, Tao & Huang, Lei & Song, Yongchen, 2024. "Impact of hydrate spatial heterogeneity on gas permeability in hydrate-bearing sediments," Energy, Elsevier, vol. 293(C).

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