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Enhancement of CO2 capture at Ca-looping conditions by high-intensity acoustic fields

Author

Listed:
  • Valverde, J.M.
  • Raganati, F.
  • Quintanilla, M.A.S.
  • Ebri, J.M.P.
  • Ammendola, P.
  • Chirone, R.

Abstract

The Ca-Looping (CaL) technology, based on a dual gas-fluidized bed system of CaO/CaCO3 particles operated at high temperature, is a viable technological process for highly efficient pre-combustion and post-combustion CO2 capture. In this paper we show a lab-scale experimental study on the carbonation/decarbonation of a fluidized bed of CaO particles at CaL conditions as affected by the application of a high-intensity acoustic field. The results obtained demonstrate that both carbonation and decarbonation are remarkably enhanced for sound intensity levels above 140dB and frequencies of about 100Hz. Fine particles (of size smaller than dp∼100μm) are entrained in the oscillating gas flow induced by an acoustic field of such low frequency, which yields a strong agitation of the bed and improves the gas–solid contact efficiency. On the other hand, an intense convection of gas flow (acoustic streaming) is generated on the surface of larger particles unmovable by the sound wave, which promotes the heat/mass transfer at the gas–solid boundary in this case. Either of these mechanisms, whose relative importance will depend on the average particle size and sound frequency, will contribute to increase the carbonation and decarbonation rates of CaO fluidized beds in the CaL technology.

Suggested Citation

  • Valverde, J.M. & Raganati, F. & Quintanilla, M.A.S. & Ebri, J.M.P. & Ammendola, P. & Chirone, R., 2013. "Enhancement of CO2 capture at Ca-looping conditions by high-intensity acoustic fields," Applied Energy, Elsevier, vol. 111(C), pages 538-549.
    • Handle: RePEc:eee:appene:v:111:y:2013:i:c:p:538-549
    DOI: 10.1016/j.apenergy.2013.05.012
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    1. Lisbona, Pilar & Martínez, Ana & Romeo, Luis M., 2013. "Hydrodynamical model and experimental results of a calcium looping cycle for CO2 capture," Applied Energy, Elsevier, vol. 101(C), pages 317-322.
    2. Siefert, Nicholas S. & Litster, Shawn, 2013. "Exergy and economic analyses of advanced IGCC–CCS and IGFC–CCS power plants," Applied Energy, Elsevier, vol. 107(C), pages 315-328.
    3. Chen, Shiyi & Xiang, Wenguo & Wang, Dong & Xue, Zhipeng, 2012. "Incorporating IGCC and CaO sorption-enhanced process for power generation with CO2 capture," Applied Energy, Elsevier, vol. 95(C), pages 285-294.
    4. Valverde, Jose M. & Sanchez-Jimenez, Pedro E. & Perejon, Antonio & Perez-Maqueda, Luis A., 2013. "Constant rate thermal analysis for enhancing the long-term CO2 capture of CaO at Ca-looping conditions," Applied Energy, Elsevier, vol. 108(C), pages 108-120.
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    4. Ma, Xiaotong & Li, Yingjie & Shi, Lei & He, Zirui & Wang, Zeyan, 2016. "Fabrication and CO2 capture performance of magnesia-stabilized carbide slag by by-product of biodiesel during calcium looping process," Applied Energy, Elsevier, vol. 168(C), pages 85-95.
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    6. Valverde, J.M. & Sanchez-Jimenez, P.E. & Perez-Maqueda, L.A., 2014. "Calcium-looping for post-combustion CO2 capture. On the adverse effect of sorbent regeneration under CO2," Applied Energy, Elsevier, vol. 126(C), pages 161-171.
    7. Ammendola, Paola & Raganati, Federica & Miccio, Francesco & Murri, Annalisa Natali & Landi, Elena, 2020. "Insights into utilization of strontium carbonate for thermochemical energy storage," Renewable Energy, Elsevier, vol. 157(C), pages 769-781.
    8. Theo, Wai Lip & Lim, Jeng Shiun & Hashim, Haslenda & Mustaffa, Azizul Azri & Ho, Wai Shin, 2016. "Review of pre-combustion capture and ionic liquid in carbon capture and storage," Applied Energy, Elsevier, vol. 183(C), pages 1633-1663.
    9. Li, Yingjie & Su, Mengying & Xie, Xin & Wu, Shuimu & Liu, Changtian, 2015. "CO2 capture performance of synthetic sorbent prepared from carbide slag and aluminum nitrate hydrate by combustion synthesis," Applied Energy, Elsevier, vol. 145(C), pages 60-68.
    10. Raganati, F. & Ammendola, P. & Chirone, R., 2014. "CO2 adsorption on fine activated carbon in a sound assisted fluidized bed: Effect of sound intensity and frequency, CO2 partial pressure and fluidization velocity," Applied Energy, Elsevier, vol. 113(C), pages 1269-1282.

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    Keywords

    CO2 capture; Ca-looping; Fluidized bed; Sound; Sonoprocessing;
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