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Visible-light-driven methane formation from CO2 with a molecular iron catalyst

Author

Listed:
  • Heng Rao

    (Université Paris Diderot, Sorbonne Paris Cité, Laboratoire d’Electrochimie Moléculaire, UMR 7591 CNRS)

  • Luciana C. Schmidt

    (Université Paris Diderot, Sorbonne Paris Cité, Laboratoire d’Electrochimie Moléculaire, UMR 7591 CNRS
    INFIQC-CONICET, Facultad de Ciencias Químicas, Universidad Nacional de Córdoba)

  • Julien Bonin

    (Université Paris Diderot, Sorbonne Paris Cité, Laboratoire d’Electrochimie Moléculaire, UMR 7591 CNRS)

  • Marc Robert

    (Université Paris Diderot, Sorbonne Paris Cité, Laboratoire d’Electrochimie Moléculaire, UMR 7591 CNRS)

Abstract

An iron tetraphenylporphyrin complex is shown to catalyse the reduction of carbon dioxide to methane upon visible light irradiation at ambient temperature and pressure.

Suggested Citation

  • Heng Rao & Luciana C. Schmidt & Julien Bonin & Marc Robert, 2017. "Visible-light-driven methane formation from CO2 with a molecular iron catalyst," Nature, Nature, vol. 548(7665), pages 74-77, August.
    • Handle: RePEc:nat:nature:v:548:y:2017:i:7665:d:10.1038_nature23016
    DOI: 10.1038/nature23016
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    Cited by:

    1. Xiaodong Li & Li Li & Xingyuan Chu & Xiaohui Liu & Guangbo Chen & Quanquan Guo & Zhen Zhang & Mingchao Wang & Shuming Wang & Alexander Tahn & Yongfu Sun & Xinliang Feng, 2024. "Photothermal CO2 conversion to ethanol through photothermal heterojunction-nanosheet arrays," Nature Communications, Nature, vol. 15(1), pages 1-12, December.
    2. Shengyao Wang & Bo Jiang & Joel Henzie & Feiyan Xu & Chengyuan Liu & Xianguang Meng & Sirong Zou & Hui Song & Yang Pan & Hexing Li & Jiaguo Yu & Hao Chen & Jinhua Ye, 2023. "Designing reliable and accurate isotope-tracer experiments for CO2 photoreduction," Nature Communications, Nature, vol. 14(1), pages 1-12, December.
    3. Bonenkamp, T.B. & Middelburg, L.M. & Hosli, M.O. & Wolffenbuttel, R.F., 2020. "From bioethanol containing fuels towards a fuel economy that includes methanol derived from renewable sources and the impact on European Union decision-making on transition pathways," Renewable and Sustainable Energy Reviews, Elsevier, vol. 120(C).
    4. Qinqin Lei & Huiqing Yuan & Jiehao Du & Mei Ming & Shuang Yang & Ya Chen & Jingxiang Lei & Zhiji Han, 2023. "Photocatalytic CO2 reduction with aminoanthraquinone organic dyes," Nature Communications, Nature, vol. 14(1), pages 1-10, December.
    5. Shuang Yang & Huiqing Yuan & Kai Guo & Zuting Wei & Mei Ming & Jinzhi Yi & Long Jiang & Zhiji Han, 2024. "Fluorinated chlorin chromophores for red-light-driven CO2 reduction," Nature Communications, Nature, vol. 15(1), pages 1-10, December.
    6. Yan Shen & Chunjin Ren & Lirong Zheng & Xiaoyong Xu & Ran Long & Wenqing Zhang & Yong Yang & Yongcai Zhang & Yingfang Yao & Haoqiang Chi & Jinlan Wang & Qing Shen & Yujie Xiong & Zhigang Zou & Yong Zh, 2023. "Room-temperature photosynthesis of propane from CO2 with Cu single atoms on vacancy-rich TiO2," Nature Communications, Nature, vol. 14(1), pages 1-9, December.
    7. Shou-Heng Liu & Jun-Sheng Lu & Yi-Chiun Chen, 2018. "Sustainable Recovery of CO 2 by Using Visible-Light-Responsive Crystal Cuprous Oxide/Reduced Graphene Oxide," Sustainability, MDPI, vol. 10(11), pages 1-13, November.
    8. Ya Wang & Jian-Xin Wei & Hong-Liang Tang & Lu-Hua Shao & Long-Zhang Dong & Xiao-Yu Chu & Yan-Xia Jiang & Gui-Ling Zhang & Feng-Ming Zhang & Ya-Qian Lan, 2024. "Artificial photosynthetic system for diluted CO2 reduction in gas-solid phase," Nature Communications, Nature, vol. 15(1), pages 1-13, December.
    9. Yongqiang Zhang & Dongmin Fu & Ziyang Chen & Rongqi Cui & Wenlong He & Hongyao Wang & Jiajin Chen & Yufei Chen & Shi-Jun Li & Yu Lan & Chunying Duan & Yunhe Jin, 2024. "Bifunctional iron-catalyzed alkyne Z-selective hydroalkylation and tandem Z-E inversion via radical molding and flipping," Nature Communications, Nature, vol. 15(1), pages 1-13, December.
    10. Zhengwei Yang & Zhen-Yu Wu & Zhexing Lin & Tianji Liu & Liping Ding & Wenbo Zhai & Zipeng Chen & Yi Jiang & Jinlei Li & Siyun Ren & Zhenhui Lin & Wangxi Liu & Jianyong Feng & Xing Zhang & Wei Li & Yi , 2024. "Optically selective catalyst design with minimized thermal emission for facilitating photothermal catalysis," Nature Communications, Nature, vol. 15(1), pages 1-10, December.
    11. Hidalgo, D. & Martín-Marroquín, J.M., 2020. "Power-to-methane, coupling CO2 capture with fuel production: An overview," Renewable and Sustainable Energy Reviews, Elsevier, vol. 132(C).
    12. Shuaishuai Wang & Tingrui Li & Chengyihan Gu & Jie Han & Chuan-Gang Zhao & Chengjian Zhu & Hairen Tan & Jin Xie, 2022. "Decarboxylative tandem C-N coupling with nitroarenes via SH2 mechanism," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
    13. Sanchita Karmakar & Soumitra Barman & Faruk Ahamed Rahimi & Darsi Rambabu & Sukhendu Nath & Tapas Kumar Maji, 2023. "Confining charge-transfer complex in a metal-organic framework for photocatalytic CO2 reduction in water," Nature Communications, Nature, vol. 14(1), pages 1-13, December.

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