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Enhanced electrocatalytic CO2 reduction via field-induced reagent concentration

Author

Listed:
  • Min Liu

    (University of Toronto)

  • Yuanjie Pang

    (University of Toronto)

  • Bo Zhang

    (University of Toronto
    East China University of Science and Technology)

  • Phil De Luna

    (University of Toronto)

  • Oleksandr Voznyy

    (University of Toronto)

  • Jixian Xu

    (University of Toronto)

  • Xueli Zheng

    (University of Toronto
    Tianjin Key Laboratory of Composite and Functional Materials, School of Materials Science and Engineering, Tianjin University)

  • Cao Thang Dinh

    (University of Toronto)

  • Fengjia Fan

    (University of Toronto)

  • Changhong Cao

    (University of Toronto)

  • F. Pelayo García de Arquer

    (University of Toronto)

  • Tina Saberi Safaei

    (University of Toronto)

  • Adam Mepham

    (Institute of Biomaterials and Biomedical Engineering, University of Toronto)

  • Anna Klinkova

    (University of Toronto)

  • Eugenia Kumacheva

    (University of Toronto)

  • Tobin Filleter

    (University of Toronto)

  • David Sinton

    (University of Toronto)

  • Shana O. Kelley

    (Institute of Biomaterials and Biomedical Engineering, University of Toronto
    Leslie Dan Faculty of Pharmacy, University of Toronto
    University of Toronto)

  • Edward H. Sargent

    (University of Toronto)

Abstract

Gold and palladium nanoneedle electrocatalysts benefit from field-induced reagent concentration to improve the efficiency of carbon dioxide reduction in the synthesis of carbon-based fuels using renewable electricity.

Suggested Citation

  • Min Liu & Yuanjie Pang & Bo Zhang & Phil De Luna & Oleksandr Voznyy & Jixian Xu & Xueli Zheng & Cao Thang Dinh & Fengjia Fan & Changhong Cao & F. Pelayo García de Arquer & Tina Saberi Safaei & Adam Me, 2016. "Enhanced electrocatalytic CO2 reduction via field-induced reagent concentration," Nature, Nature, vol. 537(7620), pages 382-386, September.
    • Handle: RePEc:nat:nature:v:537:y:2016:i:7620:d:10.1038_nature19060
    DOI: 10.1038/nature19060
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    Citations

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    Cited by:

    1. Xiaozhi Su & Zhuoli Jiang & Jing Zhou & Hengjie Liu & Danni Zhou & Huishan Shang & Xingming Ni & Zheng Peng & Fan Yang & Wenxing Chen & Zeming Qi & Dingsheng Wang & Yu Wang, 2022. "Complementary Operando Spectroscopy identification of in-situ generated metastable charge-asymmetry Cu2-CuN3 clusters for CO2 reduction to ethanol," Nature Communications, Nature, vol. 13(1), pages 1-11, December.
    2. Ye Tian & Botao Huang & Yizhi Song & Yirui Zhang & Dong Guan & Jiani Hong & Duanyun Cao & Enge Wang & Limei Xu & Yang Shao-Horn & Ying Jiang, 2024. "Effect of ion-specific water structures at metal surfaces on hydrogen production," Nature Communications, Nature, vol. 15(1), pages 1-10, December.
    3. Qiyou Wang & Kang Liu & Kangman Hu & Chao Cai & Huangjingwei Li & Hongmei Li & Matias Herran & Ying-Rui Lu & Ting-Shan Chan & Chao Ma & Junwei Fu & Shiguo Zhang & Ying Liang & Emiliano Cortés & Min Li, 2022. "Attenuating metal-substrate conjugation in atomically dispersed nickel catalysts for electroreduction of CO2 to CO," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
    4. Bingqing Wang & Meng Wang & Ziting Fan & Chao Ma & Shibo Xi & Lo‐Yueh Chang & Mingsheng Zhang & Ning Ling & Ziyu Mi & Shenghua Chen & Wan Ru Leow & Jia Zhang & Dingsheng Wang & Yanwei Lum, 2024. "Nanocurvature-induced field effects enable control over the activity of single-atom electrocatalysts," Nature Communications, Nature, vol. 15(1), pages 1-12, December.
    5. Xiaowei Shi & Chao Dai & Xin Wang & Jiayue Hu & Junying Zhang & Lingxia Zheng & Liang Mao & Huajun Zheng & Mingshan Zhu, 2022. "Protruding Pt single-sites on hexagonal ZnIn2S4 to accelerate photocatalytic hydrogen evolution," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
    6. Chia-Shuo Hsu & Jiali Wang & You-Chiuan Chu & Jui-Hsien Chen & Chia-Ying Chien & Kuo-Hsin Lin & Li Duan Tsai & Hsiao-Chien Chen & Yen-Fa Liao & Nozomu Hiraoka & Yuan-Chung Cheng & Hao Ming Chen, 2023. "Activating dynamic atomic-configuration for single-site electrocatalyst in electrochemical CO2 reduction," Nature Communications, Nature, vol. 14(1), pages 1-14, December.
    7. Jie Xu & Xiong-Xiong Xue & Gonglei Shao & Changfei Jing & Sheng Dai & Kun He & Peipei Jia & Shun Wang & Yifei Yuan & Jun Luo & Jun Lu, 2023. "Atomic-level polarization in electric fields of defects for electrocatalysis," Nature Communications, Nature, vol. 14(1), pages 1-9, December.
    8. Tongtong Li & Boran Wang & Yu Cao & Zhexuan Liu & Shaogang Wang & Qi Zhang & Jie Sun & Guangmin Zhou, 2024. "Energy-saving hydrogen production by seawater electrolysis coupling tip-enhanced electric field promoted electrocatalytic sulfion oxidation," Nature Communications, Nature, vol. 15(1), pages 1-12, December.
    9. Zesong Ma & Zhilong Yang & Wenchuan Lai & Qiyou Wang & Yan Qiao & Haolan Tao & Cheng Lian & Min Liu & Chao Ma & Anlian Pan & Hongwen Huang, 2022. "CO2 electroreduction to multicarbon products in strongly acidic electrolyte via synergistically modulating the local microenvironment," Nature Communications, Nature, vol. 13(1), pages 1-11, December.
    10. Ruixin Yang & Yanming Cai & Yongbing Qi & Zhuodong Tang & Jun-Jie Zhu & Jinxiang Li & Wenlei Zhu & Zixuan Chen, 2024. "How local electric field regulates C–C coupling at a single nanocavity in electrocatalytic CO2 reduction," Nature Communications, Nature, vol. 15(1), pages 1-11, December.
    11. Liu, Sijie & Geng, Yong & Gao, Ziyan & Li, Jinze & Xiao, Shijiang, 2023. "Uncovering the key features of gold flows and stocks in China," Resources Policy, Elsevier, vol. 82(C).
    12. Linjie Zhang & Haihui Hu & Chen Sun & Dongdong Xiao & Hsiao-Tsu Wang & Yi Xiao & Shuwen Zhao & Kuan Hung Chen & Wei-Xuan Lin & Yu-Cheng Shao & Xiuyun Wang & Chih-Wen Pao & Lili Han, 2024. "Bimetallic nanoalloys planted on super-hydrophilic carbon nanocages featuring tip-intensified hydrogen evolution electrocatalysis," Nature Communications, Nature, vol. 15(1), pages 1-12, December.
    13. Pengcheng Ye & Keqing Fang & Haiyan Wang & Yahao Wang & Hao Huang & Chenbin Mo & Jiqiang Ning & Yong Hu, 2024. "Lattice oxygen activation and local electric field enhancement by co-doping Fe and F in CoO nanoneedle arrays for industrial electrocatalytic water oxidation," Nature Communications, Nature, vol. 15(1), pages 1-12, December.
    14. Shoujie Li & Wei Chen & Xiao Dong & Chang Zhu & Aohui Chen & Yanfang Song & Guihua Li & Wei Wei & Yuhan Sun, 2022. "Hierarchical micro/nanostructured silver hollow fiber boosts electroreduction of carbon dioxide," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    15. Yicui Kang & Simão M. João & Rui Lin & Kang Liu & Li Zhu & Junwei Fu & Weng-Chon (Max) Cheong & Seunghoon Lee & Kilian Frank & Bert Nickel & Min Liu & Johannes Lischner & Emiliano Cortés, 2024. "Effect of crystal facets in plasmonic catalysis," Nature Communications, Nature, vol. 15(1), pages 1-13, December.
    16. Meng He & Rui Li & Chuanqi Cheng & Cuibo Liu & Bin Zhang, 2024. "Microenvironment regulation breaks the Faradaic efficiency-current density trade-off for electrocatalytic deuteration using D2O," Nature Communications, Nature, vol. 15(1), pages 1-10, December.
    17. Kejian Kong & An-Zhen Li & Ye Wang & Qiujin Shi & Jing Li & Kaiyue Ji & Haohong Duan, 2023. "Electrochemical carbon–carbon coupling with enhanced activity and racemate stereoselectivity by microenvironment regulation," Nature Communications, Nature, vol. 14(1), pages 1-12, December.
    18. Ji Wei Sun & Xuefeng Wu & Peng Fei Liu & Jiacheng Chen & Yuanwei Liu & Zhen Xin Lou & Jia Yue Zhao & Hai Yang Yuan & Aiping Chen & Xue Lu Wang & Minghui Zhu & Sheng Dai & Hua Gui Yang, 2023. "Scalable synthesis of coordinatively unsaturated metal-nitrogen sites for large-scale CO2 electrolysis," Nature Communications, Nature, vol. 14(1), pages 1-13, December.
    19. Hai Liu & Xinxi Huang & Yang Wang & Baian Kuang & Wanbin Li, 2024. "Nanowire-assisted electrochemical perforation of graphene oxide nanosheets for molecular separation," Nature Communications, Nature, vol. 15(1), pages 1-11, December.

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