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Benchmarking the reproducibility of all-solid-state battery cell performance

Author

Listed:
  • Sebastian Puls

    (Forschungszetrum Jülich)

  • Elina Nazmutdinova

    (University of Münster
    University of Münster)

  • Fariza Kalyk

    (Forschungszetrum Jülich)

  • Henry M. Woolley

    (University of Münster
    Institute of Physical Chemistry)

  • Jesper Frost Thomsen

    (University of Münster
    University of Münster)

  • Zhu Cheng

    (Delft University of Technology)

  • Adrien Fauchier-Magnan

    (LEPMI)

  • Ajay Gautam

    (Delft University of Technology)

  • Michael Gockeln

    (Fraunhofer Institute for Manufacturing and Advanced Materials IFAM)

  • So-Yeon Ham

    (University of California San Diego)

  • Md Toukir Hasan

    (Purdue University)

  • Min-Gi Jeong

    (Department of Mechanical and Aerospace Engineering and the Andlinger Center for Energy and the Environment)

  • Daiki Hiraoka

    (Osaka Metropolitan University)

  • Jong Seok Kim

    (Yonsei University)

  • Tobias Kutsch

    (Technische Universität München
    TUMint·Energy Research GmbH)

  • Barthélémy Lelotte

    (Paul Scherrer Institut)

  • Philip Minnmann

    (Justus Liebig University Giessen)

  • Vanessa Miß

    (Philipps-Universität Marburg)

  • Kota Motohashi

    (Osaka Metropolitan University)

  • Douglas Lars Nelson

    (Georgia Institute of Technology)

  • Frans Ooms

    (Delft University of Technology)

  • Francesco Piccolo

    (Humboldt Universität zu Berlin
    Helmholtz-Zentrum Berlin)

  • Christian Plank

    (University of Bayreuth
    University of Bayreuth)

  • Maria Rosner

    (Fraunhofer Institute for Material and Beam Technology (IWS)
    Technical University Dresden)

  • Stephanie E. Sandoval

    (Georgia Institute of Technology
    Georgia Institute of Technology)

  • Eva Schlautmann

    (University of Münster)

  • Robin Schuster

    (Technische Universität München
    TUMint·Energy Research GmbH)

  • Dominic Spencer-Jolly

    (University of Oxford
    University of Birmingham)

  • Yipeng Sun

    (University of Western Ontario)

  • Bairav S. Vishnugopi

    (Purdue University)

  • Ruizhuo Zhang

    (Karlsruhe Institute of Technology (KIT))

  • Huang Zheng

    (Kyushu University)

  • Philipp Adelhelm

    (Humboldt Universität zu Berlin
    Helmholtz-Zentrum Berlin)

  • Torsten Brezesinski

    (Karlsruhe Institute of Technology (KIT))

  • Peter G. Bruce

    (University of Oxford
    University of Oxford)

  • Michael Danzer

    (University of Bayreuth
    University of Bayreuth)

  • Mario El Kazzi

    (Paul Scherrer Institut)

  • Hubert Gasteiger

    (Technische Universität München)

  • Kelsey B. Hatzell

    (Department of Mechanical and Aerospace Engineering and the Andlinger Center for Energy and the Environment)

  • Akitoshi Hayashi

    (Osaka Metropolitan University)

  • Felix Hippauf

    (Fraunhofer Institute for Material and Beam Technology (IWS))

  • Jürgen Janek

    (Justus Liebig University Giessen)

  • Yoon Seok Jung

    (Yonsei University)

  • Matthew T. McDowell

    (Georgia Institute of Technology
    Georgia Institute of Technology)

  • Ying Shirley Meng

    (University of California San Diego
    University of Chicago)

  • Partha P. Mukherjee

    (Purdue University)

  • Saneyuki Ohno

    (Kyushu University
    Tohoku University)

  • Bernhard Roling

    (Philipps-Universität Marburg)

  • Atsushi Sakuda

    (Osaka Metropolitan University)

  • Julian Schwenzel

    (Fraunhofer Institute for Manufacturing and Advanced Materials IFAM)

  • Xueliang Sun

    (University of Western Ontario)

  • Claire Villevieille

    (LEPMI)

  • Marnix Wagemaker

    (Delft University of Technology)

  • Wolfgang G. Zeier

    (Forschungszetrum Jülich
    University of Münster)

  • Nella M. Vargas-Barbosa

    (Forschungszetrum Jülich
    University of Bayreuth
    University of Bayreuth)

Abstract

The interlaboratory comparability and reproducibility of all-solid-state battery cell cycling performance are poorly understood due to the lack of standardized set-ups and assembly parameters. This study quantifies the extent of this variability by providing commercially sourced battery materials—LiNi0.6Mn0.2Co0.2O2 for the positive electrode, Li6PS5Cl as the solid electrolyte and indium for the negative electrode—to 21 research groups. Each group was asked to use their own cell assembly protocol but follow a specific electrochemical protocol. The results show large variability in assembly and electrochemical performance, including differences in processing pressures, pressing durations and In-to-Li ratios. Despite this, an initial open circuit voltage of 2.5 and 2.7 V vs Li+/Li is a good predictor of successful cycling for cells using these electroactive materials. We suggest a set of parameters for reporting all-solid-state battery cycling results and advocate for reporting data in triplicate.

Suggested Citation

  • Sebastian Puls & Elina Nazmutdinova & Fariza Kalyk & Henry M. Woolley & Jesper Frost Thomsen & Zhu Cheng & Adrien Fauchier-Magnan & Ajay Gautam & Michael Gockeln & So-Yeon Ham & Md Toukir Hasan & Min-, 2024. "Benchmarking the reproducibility of all-solid-state battery cell performance," Nature Energy, Nature, vol. 9(10), pages 1310-1320, October.
    • Handle: RePEc:nat:natene:v:9:y:2024:i:10:d:10.1038_s41560-024-01634-3
    DOI: 10.1038/s41560-024-01634-3
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    References listed on IDEAS

    as
    1. Simon Randau & Dominik A. Weber & Olaf Kötz & Raimund Koerver & Philipp Braun & André Weber & Ellen Ivers-Tiffée & Torben Adermann & Jörn Kulisch & Wolfgang G. Zeier & Felix H. Richter & Jürgen Janek, 2020. "Benchmarking the performance of all-solid-state lithium batteries," Nature Energy, Nature, vol. 5(3), pages 259-270, March.
    2. Richard Van Noorden, 2014. "The rechargeable revolution: A better battery," Nature, Nature, vol. 507(7490), pages 26-28, March.
    Full references (including those not matched with items on IDEAS)

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