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Benchmarking the performance of all-solid-state lithium batteries

Author

Listed:
  • Simon Randau

    (Justus-Liebig-University Giessen)

  • Dominik A. Weber

    (Justus-Liebig-University Giessen
    Volkswagen AG, Group Research)

  • Olaf Kötz

    (Justus-Liebig-University Giessen)

  • Raimund Koerver

    (Justus-Liebig-University Giessen
    BMW Group)

  • Philipp Braun

    (Karlsruhe Institute of Technology, Institute for Applied Materials)

  • André Weber

    (Karlsruhe Institute of Technology, Institute for Applied Materials)

  • Ellen Ivers-Tiffée

    (Karlsruhe Institute of Technology, Institute for Applied Materials)

  • Torben Adermann

    (BASF SE)

  • Jörn Kulisch

    (BASF SE)

  • Wolfgang G. Zeier

    (Justus-Liebig-University Giessen)

  • Felix H. Richter

    (Justus-Liebig-University Giessen)

  • Jürgen Janek

    (Justus-Liebig-University Giessen)

Abstract

Increasing the specific energy, energy density, specific power, energy efficiency and energy retention of electrochemical storage devices are major incentives for the development of all-solid-state batteries. However, a general evaluation of all-solid-state battery performance is often difficult to derive from published reports, mostly due to the interdependence of performance measures, but also due to the lack of a basic reference system. Here, we present all-solid-state batteries reduced to the bare minimum of compounds, containing only a lithium metal anode, β-Li3PS4 solid electrolyte and Li(Ni0.6Co0.2Mn0.2)O2 cathode active material. We use this minimalistic system to benchmark the performance of all-solid-state batteries. In a Ragone-type graph, we compare literature data for thiophosphate-, oxide-, phosphate- and polymer-based all-solid-state batteries with our minimalistic cell. Using fundamental equations for key performance parameters, we identify research targets towards high energy, high power and practical all-solid-state batteries.

Suggested Citation

  • Simon Randau & Dominik A. Weber & Olaf Kötz & Raimund Koerver & Philipp Braun & André Weber & Ellen Ivers-Tiffée & Torben Adermann & Jörn Kulisch & Wolfgang G. Zeier & Felix H. Richter & Jürgen Janek, 2020. "Benchmarking the performance of all-solid-state lithium batteries," Nature Energy, Nature, vol. 5(3), pages 259-270, March.
    • Handle: RePEc:nat:natene:v:5:y:2020:i:3:d:10.1038_s41560-020-0565-1
    DOI: 10.1038/s41560-020-0565-1
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    Citations

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    Cited by:

    1. Sung-Kyun Jung & Hyeokjo Gwon & Hyungsub Kim & Gabin Yoon & Dongki Shin & Jihyun Hong & Changhoon Jung & Ju-Sik Kim, 2022. "Unlocking the hidden chemical space in cubic-phase garnet solid electrolyte for efficient quasi-all-solid-state lithium batteries," Nature Communications, Nature, vol. 13(1), pages 1-13, December.
    2. Mouhamad S. Diallo & Tan Shi & Yaqian Zhang & Xinxing Peng & Imtiaz Shozib & Yan Wang & Lincoln J. Miara & Mary C. Scott & Qingsong Howard Tu & Gerbrand Ceder, 2024. "Effect of solid-electrolyte pellet density on failure of solid-state batteries," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    3. Tong-Tong Zuo & Raffael Rueß & Ruijun Pan & Felix Walther & Marcus Rohnke & Satoshi Hori & Ryoji Kanno & Daniel Schröder & Jürgen Janek, 2021. "A mechanistic investigation of the Li10GeP2S12|LiNi1-x-yCoxMnyO2 interface stability in all-solid-state lithium batteries," Nature Communications, Nature, vol. 12(1), pages 1-10, December.
    4. Ghulam E Mustafa Abro & Saiful Azrin B. M. Zulkifli & Kundan Kumar & Najib El Ouanjli & Vijanth Sagayan Asirvadam & Mahmoud A. Mossa, 2023. "Comprehensive Review of Recent Advancements in Battery Technology, Propulsion, Power Interfaces, and Vehicle Network Systems for Intelligent Autonomous and Connected Electric Vehicles," Energies, MDPI, vol. 16(6), pages 1-31, March.
    5. Jiaxuan Wang & Feng Hao, 2023. "Experimental Investigations on the Chemo-Mechanical Coupling in Solid-State Batteries and Electrode Materials," Energies, MDPI, vol. 16(3), pages 1-17, January.
    6. Dewu Zeng & Jingming Yao & Long Zhang & Ruonan Xu & Shaojie Wang & Xinlin Yan & Chuang Yu & Lin Wang, 2022. "Promoting favorable interfacial properties in lithium-based batteries using chlorine-rich sulfide inorganic solid-state electrolytes," Nature Communications, Nature, vol. 13(1), pages 1-13, December.
    7. Daiwei Wang & Li-Ji Jhang & Rong Kou & Meng Liao & Shiyao Zheng & Heng Jiang & Pei Shi & Guo-Xing Li & Kui Meng & Donghai Wang, 2023. "Realizing high-capacity all-solid-state lithium-sulfur batteries using a low-density inorganic solid-state electrolyte," Nature Communications, Nature, vol. 14(1), pages 1-10, December.
    8. Manfred Dollinger & Gerhard Fischerauer, 2023. "Physics-Based Prediction for the Consumption and Emissions of Passenger Vehicles and Light Trucks up to 2050," Energies, MDPI, vol. 16(8), pages 1-29, April.
    9. Yantao Wang & Hongtao Qu & Bowen Liu & Xiaoju Li & Jiangwei Ju & Jiedong Li & Shu Zhang & Jun Ma & Chao Li & Zhiwei Hu & Chung-Kai Chang & Hwo-Shuenn Sheu & Longfei Cui & Feng Jiang & Ernst R. H. Eck , 2023. "Self-organized hetero-nanodomains actuating super Li+ conduction in glass ceramics," Nature Communications, Nature, vol. 14(1), pages 1-11, December.
    10. James T. Frith & Matthew J. Lacey & Ulderico Ulissi, 2023. "A non-academic perspective on the future of lithium-based batteries," Nature Communications, Nature, vol. 14(1), pages 1-17, December.
    11. Jing Li & Jizhen Qi & Feng Jin & Fengrui Zhang & Lei Zheng & Lingfei Tang & Rong Huang & Jingjing Xu & Hongwei Chen & Ming Liu & Yejun Qiu & Andrew I. Cooper & Yanbin Shen & Liwei Chen, 2022. "Room temperature all-solid-state lithium batteries based on a soluble organic cage ionic conductor," Nature Communications, Nature, vol. 13(1), pages 1-11, December.
    12. Yun Su & Xiaohui Rong & Ang Gao & Yuan Liu & Jianwei Li & Minglei Mao & Xingguo Qi & Guoliang Chai & Qinghua Zhang & Liumin Suo & Lin Gu & Hong Li & Xuejie Huang & Liquan Chen & Binyuan Liu & Yong-She, 2022. "Rational design of a topological polymeric solid electrolyte for high-performance all-solid-state alkali metal batteries," Nature Communications, Nature, vol. 13(1), pages 1-15, December.
    13. Burak Aktekin & Luise M. Riegger & Svenja-K. Otto & Till Fuchs & Anja Henss & Jürgen Janek, 2023. "SEI growth on Lithium metal anodes in solid-state batteries quantified with coulometric titration time analysis," Nature Communications, Nature, vol. 14(1), pages 1-14, December.

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