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Observation of stacking engineered magnetic phase transitions within moiré supercells of twisted van der Waals magnets

Author

Listed:
  • Senlei Li

    (Georgia Institute of Technology)

  • Zeliang Sun

    (the University of Michigan)

  • Nathan J. McLaughlin

    (University of California, San Diego, La Jolla)

  • Afsana Sharmin

    (Colorado State University)

  • Nishkarsh Agarwal

    (University of Michigan)

  • Mengqi Huang

    (Georgia Institute of Technology)

  • Suk Hyun Sung

    (University of Michigan)

  • Hanyi Lu

    (University of California, San Diego, La Jolla)

  • Shaohua Yan

    (Renmin University of China
    Renmin University of China)

  • Hechang Lei

    (Renmin University of China
    Renmin University of China)

  • Robert Hovden

    (University of Michigan)

  • Hailong Wang

    (Georgia Institute of Technology)

  • Hua Chen

    (Colorado State University
    Colorado State University)

  • Liuyan Zhao

    (the University of Michigan)

  • Chunhui Rita Du

    (Georgia Institute of Technology
    University of California, San Diego, La Jolla)

Abstract

Recent demonstrations of moiré magnetism, featuring exotic phases with noncollinear spin order in the twisted van der Waals (vdW) magnet chromium triiodide CrI3, have highlighted the potential of twist engineering of magnetic (vdW) materials. However, the local magnetic interactions, spin dynamics, and magnetic phase transitions within and across individual moiré supercells remain elusive. Taking advantage of a scanning single-spin magnetometry platform, here we report observation of two distinct magnetic phase transitions with separate critical temperatures within a moiré supercell of small-angle twisted double trilayer CrI3. By measuring temperature-dependent spin fluctuations at the coexisting ferromagnetic and antiferromagnetic regions in twisted CrI3, we explicitly show that the Curie temperature of the ferromagnetic state is higher than the Néel temperature of the antiferromagnetic one by ~10 K. Our mean-field calculations attribute such a spatial and thermodynamic phase separation to the stacking order modulated interlayer exchange coupling at the twisted interface of moiré superlattices.

Suggested Citation

  • Senlei Li & Zeliang Sun & Nathan J. McLaughlin & Afsana Sharmin & Nishkarsh Agarwal & Mengqi Huang & Suk Hyun Sung & Hanyi Lu & Shaohua Yan & Hechang Lei & Robert Hovden & Hailong Wang & Hua Chen & Li, 2024. "Observation of stacking engineered magnetic phase transitions within moiré supercells of twisted van der Waals magnets," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    • Handle: RePEc:nat:natcom:v:15:y:2024:i:1:d:10.1038_s41467-024-49942-2
    DOI: 10.1038/s41467-024-49942-2
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