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Non-coplanar helimagnetism in the layered van-der-Waals metal DyTe3

Author

Listed:
  • Shun Akatsuka

    (The University of Tokyo)

  • Sebastian Esser

    (The University of Tokyo)

  • Shun Okumura

    (The University of Tokyo)

  • Ryota Yambe

    (The University of Tokyo)

  • Rinsuke Yamada

    (The University of Tokyo)

  • Moritz M. Hirschmann

    (RIKEN Center for Emergent Matter Science (CEMS))

  • Seno Aji

    (The University of Tokyo
    Universitas Indonesia)

  • Jonathan S. White

    (Paul Scherrer Institute (PSI))

  • Shang Gao

    (University of Science and Technology of China)

  • Yoshichika Onuki

    (RIKEN Center for Emergent Matter Science (CEMS))

  • Taka-hisa Arima

    (RIKEN Center for Emergent Matter Science (CEMS)
    The University of Tokyo)

  • Taro Nakajima

    (RIKEN Center for Emergent Matter Science (CEMS)
    The University of Tokyo)

  • Max Hirschberger

    (The University of Tokyo
    RIKEN Center for Emergent Matter Science (CEMS)
    The University of Tokyo)

Abstract

Van-der-Waals magnetic materials can be exfoliated to realize ultrathin sheets or interfaces with highly controllable optical or spintronics responses. In majority, these are collinear ferro-, ferri-, or antiferromagnets, with a particular scarcity of lattice-incommensurate helimagnets of defined left- or right-handed rotation sense, or helicity. Here, we report polarized neutron scattering experiments on DyTe3, whose layered structure has highly metallic tellurium layers separated by double-slabs of dysprosium square nets. We reveal cycloidal (conical) magnetic textures, with coupled commensurate and incommensurate order parameters, and probe the evolution of this ground state in a magnetic field. The observations are well explained by a one-dimensional spin model, with an off-diagonal on-site term that is spatially modulated by DyTe3’s unconventional charge density wave (CDW) order. The CDW-driven term couples to antiferromagnetism, or to the net magnetization in an applied magnetic field, and creates a complex magnetic phase diagram indicative of competing interactions in this easily cleavable van-der-Waals helimagnet.

Suggested Citation

  • Shun Akatsuka & Sebastian Esser & Shun Okumura & Ryota Yambe & Rinsuke Yamada & Moritz M. Hirschmann & Seno Aji & Jonathan S. White & Shang Gao & Yoshichika Onuki & Taka-hisa Arima & Taro Nakajima & M, 2024. "Non-coplanar helimagnetism in the layered van-der-Waals metal DyTe3," Nature Communications, Nature, vol. 15(1), pages 1-10, December.
    • Handle: RePEc:nat:natcom:v:15:y:2024:i:1:d:10.1038_s41467-024-47127-5
    DOI: 10.1038/s41467-024-47127-5
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