IDEAS home Printed from https://ideas.repec.org/a/nat/natcom/v13y2022i1d10.1038_s41467-022-32290-4.html
   My bibliography  Save this article

Dynamic magnetic crossover at the origin of the hidden-order in van der Waals antiferromagnet CrSBr

Author

Listed:
  • Sara A. López-Paz

    (University of Geneva
    University of Zurich)

  • Zurab Guguchia

    (Laboratory for Muon Spin Spectroscopy, Paul Scherrer Institut)

  • Vladimir Y. Pomjakushin

    (Laboratory for Neutron Scattering and Imaging, Paul Scherrer Institut)

  • Catherine Witteveen

    (University of Geneva
    University of Zurich)

  • Antonio Cervellino

    (Laboratory for Synchrotron Radiation - Condensed Matter, Paul Scherrer Institut)

  • Hubertus Luetkens

    (Laboratory for Muon Spin Spectroscopy, Paul Scherrer Institut)

  • Nicola Casati

    (Laboratory for Synchrotron Radiation - Condensed Matter, Paul Scherrer Institut)

  • Alberto F. Morpurgo

    (University of Geneva
    University of Geneva)

  • Fabian O. von Rohr

    (University of Geneva)

Abstract

The van-der-Waals material CrSBr stands out as a promising two-dimensional magnet. Here, we report on its detailed magnetic and structural characteristics. We evidence that it undergoes a transition to an A-type antiferromagnetic state below TN ≈ 140 K with a pronounced two-dimensional character, preceded by ferromagnetic correlations within the monolayers. Furthermore, we unravel the low-temperature hidden-order within the long-range magnetically-ordered state. We find that it is associated to a slowing down of the magnetic fluctuations, accompanied by a continuous reorientation of the internal field. These take place upon cooling below Ts ≈ 100 K, until a spin freezing process occurs at T* ≈ 40 K. We argue this complex behavior to reflect a crossover driven by the in-plane uniaxial anisotropy, which is ultimately caused by its mixed-anion character. Our findings reinforce CrSBr as an important candidate for devices in the emergent field of two-dimensional magnetic materials.

Suggested Citation

  • Sara A. López-Paz & Zurab Guguchia & Vladimir Y. Pomjakushin & Catherine Witteveen & Antonio Cervellino & Hubertus Luetkens & Nicola Casati & Alberto F. Morpurgo & Fabian O. von Rohr, 2022. "Dynamic magnetic crossover at the origin of the hidden-order in van der Waals antiferromagnet CrSBr," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
    • Handle: RePEc:nat:natcom:v:13:y:2022:i:1:d:10.1038_s41467-022-32290-4
    DOI: 10.1038/s41467-022-32290-4
    as

    Download full text from publisher

    File URL: https://www.nature.com/articles/s41467-022-32290-4
    File Function: Abstract
    Download Restriction: no
    File URL: https://libkey.io/10.1038/s41467-022-32290-4?utm_source=ideas
    LibKey link: if access is restricted and if your library uses this service, LibKey will redirect you to where you can use your library subscription to access this item
    ---><---

    References listed on IDEAS

    as
    1. Nathan P. Wilson & Wang Yao & Jie Shan & Xiaodong Xu, 2021. "Excitons and emergent quantum phenomena in stacked 2D semiconductors," Nature, Nature, vol. 599(7885), pages 383-392, November.
    2. Bevin Huang & Genevieve Clark & Efrén Navarro-Moratalla & Dahlia R. Klein & Ran Cheng & Kyle L. Seyler & Ding Zhong & Emma Schmidgall & Michael A. McGuire & David H. Cobden & Wang Yao & Di Xiao & Pabl, 2017. "Layer-dependent ferromagnetism in a van der Waals crystal down to the monolayer limit," Nature, Nature, vol. 546(7657), pages 270-273, June.
    3. A. K. Geim & I. V. Grigorieva, 2013. "Van der Waals heterostructures," Nature, Nature, vol. 499(7459), pages 419-425, July.
    4. Kenneth S. Burch & David Mandrus & Je-Geun Park, 2018. "Magnetism in two-dimensional van der Waals materials," Nature, Nature, vol. 563(7729), pages 47-52, November.
    5. Cheng Gong & Lin Li & Zhenglu Li & Huiwen Ji & Alex Stern & Yang Xia & Ting Cao & Wei Bao & Chenzhe Wang & Yuan Wang & Z. Q. Qiu & R. J. Cava & Steven G. Louie & Jing Xia & Xiang Zhang, 2017. "Discovery of intrinsic ferromagnetism in two-dimensional van der Waals crystals," Nature, Nature, vol. 546(7657), pages 265-269, June.
    Full references (including those not matched with items on IDEAS)

    Citations

    Citations are extracted by the CitEc Project, subscribe to its RSS feed for this item.
    as


    Cited by:

    1. Xiaoyu Guo & Wenhao Liu & Jonathan Schwartz & Suk Hyun Sung & Dechen Zhang & Makoto Shimizu & Aswin L. N. Kondusamy & Lu Li & Kai Sun & Hui Deng & Harald O. Jeschke & Igor I. Mazin & Robert Hovden & B, 2024. "Extraordinary phase transition revealed in a van der Waals antiferromagnet," Nature Communications, Nature, vol. 15(1), pages 1-10, December.

    Most related items

    These are the items that most often cite the same works as this one and are cited by the same works as this one.
    1. Guanghui Cheng & Mohammad Mushfiqur Rahman & Zhiping He & Andres Llacsahuanga Allcca & Avinash Rustagi & Kirstine Aggerbeck Stampe & Yanglin Zhu & Shaohua Yan & Shangjie Tian & Zhiqiang Mao & Hechang , 2022. "Emergence of electric-field-tunable interfacial ferromagnetism in 2D antiferromagnet heterostructures," Nature Communications, Nature, vol. 13(1), pages 1-6, December.
    2. Faran Zhou & Kyle Hwangbo & Qi Zhang & Chong Wang & Lingnan Shen & Jiawei Zhang & Qianni Jiang & Alfred Zong & Yifan Su & Marc Zajac & Youngjun Ahn & Donald A. Walko & Richard D. Schaller & Jiun-Haw C, 2022. "Dynamical criticality of spin-shear coupling in van der Waals antiferromagnets," Nature Communications, Nature, vol. 13(1), pages 1-7, December.
    3. Zefang Li & Huai Zhang & Guanqi Li & Jiangteng Guo & Qingping Wang & Ying Deng & Yue Hu & Xuange Hu & Can Liu & Minghui Qin & Xi Shen & Richeng Yu & Xingsen Gao & Zhimin Liao & Junming Liu & Zhipeng H, 2024. "Room-temperature sub-100 nm Néel-type skyrmions in non-stoichiometric van der Waals ferromagnet Fe3-xGaTe2 with ultrafast laser writability," Nature Communications, Nature, vol. 15(1), pages 1-11, December.
    4. Yong Zhong & Cheng Peng & Haili Huang & Dandan Guan & Jinwoong Hwang & Kuan H. Hsu & Yi Hu & Chunjing Jia & Brian Moritz & Donghui Lu & Jun-Sik Lee & Jin-Feng Jia & Thomas P. Devereaux & Sung-Kwan Mo , 2023. "From Stoner to local moment magnetism in atomically thin Cr2Te3," Nature Communications, Nature, vol. 14(1), pages 1-7, December.
    5. Yongxi Ou & Wilson Yanez & Run Xiao & Max Stanley & Supriya Ghosh & Boyang Zheng & Wei Jiang & Yu-Sheng Huang & Timothy Pillsbury & Anthony Richardella & Chaoxing Liu & Tony Low & Vincent H. Crespi & , 2022. "ZrTe2/CrTe2: an epitaxial van der Waals platform for spintronics," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    6. Jun Cui & Emil Viñas Boström & Mykhaylo Ozerov & Fangliang Wu & Qianni Jiang & Jiun-Haw Chu & Changcun Li & Fucai Liu & Xiaodong Xu & Angel Rubio & Qi Zhang, 2023. "Chirality selective magnon-phonon hybridization and magnon-induced chiral phonons in a layered zigzag antiferromagnet," Nature Communications, Nature, vol. 14(1), pages 1-9, December.
    7. Shun Akatsuka & Sebastian Esser & Shun Okumura & Ryota Yambe & Rinsuke Yamada & Moritz M. Hirschmann & Seno Aji & Jonathan S. White & Shang Gao & Yoshichika Onuki & Taka-hisa Arima & Taro Nakajima & M, 2024. "Non-coplanar helimagnetism in the layered van-der-Waals metal DyTe3," Nature Communications, Nature, vol. 15(1), pages 1-10, December.
    8. Jing-Jing Xian & Cong Wang & Jin-Hua Nie & Rui Li & Mengjiao Han & Junhao Lin & Wen-Hao Zhang & Zhen-Yu Liu & Zhi-Mo Zhang & Mao-Peng Miao & Yangfan Yi & Shiwei Wu & Xiaodie Chen & Junbo Han & Zhengca, 2022. "Spin mapping of intralayer antiferromagnetism and field-induced spin reorientation in monolayer CrTe2," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    9. Fengrui Yao & Volodymyr Multian & Zhe Wang & Nicolas Ubrig & Jérémie Teyssier & Fan Wu & Enrico Giannini & Marco Gibertini & Ignacio Gutiérrez-Lezama & Alberto F. Morpurgo, 2023. "Multiple antiferromagnetic phases and magnetic anisotropy in exfoliated CrBr3 multilayers," Nature Communications, Nature, vol. 14(1), pages 1-10, December.
    10. Linfeng Ai & Enze Zhang & Jinshan Yang & Xiaoyi Xie & Yunkun Yang & Zehao Jia & Yuda Zhang & Shanshan Liu & Zihan Li & Pengliang Leng & Xiangyu Cao & Xingdan Sun & Tongyao Zhang & Xufeng Kou & Zheng H, 2021. "Van der Waals ferromagnetic Josephson junctions," Nature Communications, Nature, vol. 12(1), pages 1-9, December.
    11. David Lujan & Jeongheon Choe & Martin Rodriguez-Vega & Zhipeng Ye & Aritz Leonardo & T. Nathan Nunley & Liang-Juan Chang & Shang-Fan Lee & Jiaqiang Yan & Gregory A. Fiete & Rui He & Xiaoqin Li, 2022. "Magnons and magnetic fluctuations in atomically thin MnBi2Te4," Nature Communications, Nature, vol. 13(1), pages 1-7, December.
    12. M. T. Birch & L. Powalla & S. Wintz & O. Hovorka & K. Litzius & J. C. Loudon & L. A. Turnbull & V. Nehruji & K. Son & C. Bubeck & T. G. Rauch & M. Weigand & E. Goering & M. Burghard & G. Schütz, 2022. "History-dependent domain and skyrmion formation in 2D van der Waals magnet Fe3GeTe2," Nature Communications, Nature, vol. 13(1), pages 1-11, December.
    13. P. Padmanabhan & F. L. Buessen & R. Tutchton & K. W. C. Kwock & S. Gilinsky & M. C. Lee & M. A. McGuire & S. R. Singamaneni & D. A. Yarotski & A. Paramekanti & J.-X. Zhu & R. P. Prasankumar, 2022. "Coherent helicity-dependent spin-phonon oscillations in the ferromagnetic van der Waals crystal CrI3," Nature Communications, Nature, vol. 13(1), pages 1-8, December.
    14. Xingzhi Wang & Qishuo Tan & Tie Li & Zhengguang Lu & Jun Cao & Yanan Ge & Lili Zhao & Jing Tang & Hikari Kitadai & Mingda Guo & Yun-Mei Li & Weigao Xu & Ran Cheng & Dmitry Smirnov & Xi Ling, 2024. "Unveiling the spin evolution in van der Waals antiferromagnets via magneto-exciton effects," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    15. Ruiqing Cheng & Lei Yin & Yao Wen & Baoxing Zhai & Yuzheng Guo & Zhaofu Zhang & Weitu Liao & Wenqi Xiong & Hao Wang & Shengjun Yuan & Jian Jiang & Chuansheng Liu & Jun He, 2022. "Ultrathin ferrite nanosheets for room-temperature two-dimensional magnetic semiconductors," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    16. J. Klein & T. Pham & J. D. Thomsen & J. B. Curtis & T. Denneulin & M. Lorke & M. Florian & A. Steinhoff & R. A. Wiscons & J. Luxa & Z. Sofer & F. Jahnke & P. Narang & F. M. Ross, 2022. "Control of structure and spin texture in the van der Waals layered magnet CrSBr," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    17. Senlei Li & Zeliang Sun & Nathan J. McLaughlin & Afsana Sharmin & Nishkarsh Agarwal & Mengqi Huang & Suk Hyun Sung & Hanyi Lu & Shaohua Yan & Hechang Lei & Robert Hovden & Hailong Wang & Hua Chen & Li, 2024. "Observation of stacking engineered magnetic phase transitions within moiré supercells of twisted van der Waals magnets," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    18. Chenhui Zhang & Ze Jiang & Jiawei Jiang & Wa He & Junwei Zhang & Fanrui Hu & Shishun Zhao & Dongsheng Yang & Yakun Liu & Yong Peng & Hongxin Yang & Hyunsoo Yang, 2024. "Above-room-temperature chiral skyrmion lattice and Dzyaloshinskii–Moriya interaction in a van der Waals ferromagnet Fe3−xGaTe2," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    19. Han Wu & Lei Chen & Paul Malinowski & Bo Gyu Jang & Qinwen Deng & Kirsty Scott & Jianwei Huang & Jacob P. C. Ruff & Yu He & Xiang Chen & Chaowei Hu & Ziqin Yue & Ji Seop Oh & Xiaokun Teng & Yucheng Gu, 2024. "Reversible non-volatile electronic switching in a near-room-temperature van der Waals ferromagnet," Nature Communications, Nature, vol. 15(1), pages 1-11, December.
    20. Cheng Gong & Peiyao Zhang & Tenzin Norden & Quanwei Li & Zhen Guo & Apoorva Chaturvedi & Arman Najafi & Shoufeng Lan & Xiaoze Liu & Yuan Wang & Shi-Jing Gong & Hao Zeng & Hua Zhang & Athos Petrou & Xi, 2023. "Ferromagnetism emerged from non-ferromagnetic atomic crystals," Nature Communications, Nature, vol. 14(1), pages 1-7, December.

    More about this item

    Statistics

    Access and download statistics

    Corrections

    All material on this site has been provided by the respective publishers and authors. You can help correct errors and omissions. When requesting a correction, please mention this item's handle: RePEc:nat:natcom:v:13:y:2022:i:1:d:10.1038_s41467-022-32290-4. See general information about how to correct material in RePEc.

    If you have authored this item and are not yet registered with RePEc, we encourage you to do it here. This allows to link your profile to this item. It also allows you to accept potential citations to this item that we are uncertain about.

    If CitEc recognized a bibliographic reference but did not link an item in RePEc to it, you can help with this form .

    If you know of missing items citing this one, you can help us creating those links by adding the relevant references in the same way as above, for each refering item. If you are a registered author of this item, you may also want to check the "citations" tab in your RePEc Author Service profile, as there may be some citations waiting for confirmation.

    For technical questions regarding this item, or to correct its authors, title, abstract, bibliographic or download information, contact: Sonal Shukla or Springer Nature Abstracting and Indexing (email available below). General contact details of provider: http://www.nature.com .

    Please note that corrections may take a couple of weeks to filter through the various RePEc services.

    IDEAS is a RePEc service. RePEc uses bibliographic data supplied by the respective publishers.