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Facet-selective growth of halide perovskite/2D semiconductor van der Waals heterostructures for improved optical gain and lasing

Author

Listed:
  • Liqiang Zhang

    (Hunan University)

  • Yiliu Wang

    (Hunan University)

  • Anshi Chu

    (Hunan University)

  • Zhengwei Zhang

    (Central South University)

  • Miaomiao Liu

    (Hunan University)

  • Xiaohua Shen

    (Hunan University)

  • Bailing Li

    (Hunan University)

  • Xu Li

    (Hunan University)

  • Chen Yi

    (Hunan University)

  • Rong Song

    (Hunan University)

  • Yingying Liu

    (Hunan University)

  • Xiujuan Zhuang

    (Hunan University)

  • Xidong Duan

    (Hunan University)

Abstract

The tunable properties of halide perovskite/two dimensional (2D) semiconductor mixed-dimensional van der Waals heterostructures offer high flexibility for innovating optoelectronic and photonic devices. However, the general and robust growth of high-quality monocrystalline halide perovskite/2D semiconductor heterostructures with attractive optical properties has remained challenging. Here, we demonstrate a universal van der Waals heteroepitaxy strategy to synthesize a library of facet-specific single-crystalline halide perovskite/2D semiconductor (multi)heterostructures. The obtained heterostructures can be broadly tailored by selecting the coupling layer of interest, and can include perovskites varying from all-inorganic to organic-inorganic hybrid counterparts, individual transition metal dichalcogenides or 2D heterojunctions. The CsPbI2Br/WSe2 heterostructures demonstrate ultrahigh optical gain coefficient, reduced gain threshold and prolonged gain lifetime, which are attributed to the reduced energetic disorder. Accordingly, the self-organized halide perovskite/2D semiconductor heterostructure lasers show highly reproducible single-mode lasing with largely reduced lasing threshold and improved stability. Our findings provide a high-quality and versatile material platform for probing unique optoelectronic and photonic physics and developing further electrically driven on-chip lasers, nanophotonic devices and electronic-photonic integrated systems.

Suggested Citation

  • Liqiang Zhang & Yiliu Wang & Anshi Chu & Zhengwei Zhang & Miaomiao Liu & Xiaohua Shen & Bailing Li & Xu Li & Chen Yi & Rong Song & Yingying Liu & Xiujuan Zhuang & Xidong Duan, 2024. "Facet-selective growth of halide perovskite/2D semiconductor van der Waals heterostructures for improved optical gain and lasing," Nature Communications, Nature, vol. 15(1), pages 1-15, December.
  • Handle: RePEc:nat:natcom:v:15:y:2024:i:1:d:10.1038_s41467-024-49364-0
    DOI: 10.1038/s41467-024-49364-0
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