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Stress-induced ordering evolution of 1D segmented heteronanostructures and their chemical post-transformations

Author

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  • Qing-Xia Chen

    (University of Science and Technology of China)

  • Yu-Yang Lu

    (University of Science and Technology of China)

  • Yang Yang

    (University of Science and Technology of China)

  • Li-Ge Chang

    (University of Science and Technology of China)

  • Yi Li

    (University of Science and Technology of China)

  • Yuan Yang

    (University of Science and Technology of China)

  • Zhen He

    (University of Science and Technology of China)

  • Jian-Wei Liu

    (University of Science and Technology of China)

  • Yong Ni

    (University of Science and Technology of China)

  • Shu-Hong Yu

    (University of Science and Technology of China)

Abstract

Investigations of one-dimensional segmented heteronanostructures (1D-SHs) have recently attracted much attention due to their potentials for applications resulting from their structure and synergistic effects between compositions and interfaces. Unfortunately, developing a simple, versatile and controlled synthetic method to fabricate 1D-SHs is still a challenge. Here we demonstrate a stress-induced axial ordering mechanism to describe the synthesis of 1D-SHs by a general under-stoichiometric reaction strategy. Using the continuum phase-field simulations, we elaborate a three-stage evolution process of the regular segment alternations. This strategy, accompanied by easy chemical post-transformations, enables to synthesize 25 1D-SHs, including 17 nanowire-nanowire and 8 nanowire-nanotube nanostructures with 13 elements (Ag, Te, Cu, Pt, Pb, Cd, Sb, Se, Bi, Rh, Ir, Ru, Zn) involved. This ordering evolution-driven synthesis will help to investigate the ordering reconstruction and potential applications of 1D-SHs.

Suggested Citation

  • Qing-Xia Chen & Yu-Yang Lu & Yang Yang & Li-Ge Chang & Yi Li & Yuan Yang & Zhen He & Jian-Wei Liu & Yong Ni & Shu-Hong Yu, 2024. "Stress-induced ordering evolution of 1D segmented heteronanostructures and their chemical post-transformations," Nature Communications, Nature, vol. 15(1), pages 1-12, December.
    • Handle: RePEc:nat:natcom:v:15:y:2024:i:1:d:10.1038_s41467-024-47446-7
    DOI: 10.1038/s41467-024-47446-7
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