IDEAS home Printed from https://ideas.repec.org/a/nat/natcom/v15y2024i1d10.1038_s41467-024-47088-9.html
   My bibliography  Save this article

Raman time-delay in attosecond transient absorption of strong-field created krypton vacancy

Author

Listed:
  • Li Wang

    (National University of Defense Technology
    National University of Defense Technology)

  • Guangru Bai

    (National University of Defense Technology
    National University of Defense Technology)

  • Xiaowei Wang

    (National University of Defense Technology
    National University of Defense Technology)

  • Jing Zhao

    (National University of Defense Technology
    National University of Defense Technology)

  • Cheng Gao

    (National University of Defense Technology
    National University of Defense Technology)

  • Jiacan Wang

    (National University of Defense Technology
    National University of Defense Technology)

  • Fan Xiao

    (National University of Defense Technology
    National University of Defense Technology)

  • Wenkai Tao

    (National University of Defense Technology
    National University of Defense Technology)

  • Pan Song

    (National University of Defense Technology)

  • Qianyu Qiu

    (National University of Defense Technology
    National University of Defense Technology)

  • Jinlei Liu

    (National University of Defense Technology
    National University of Defense Technology)

  • Zengxiu Zhao

    (National University of Defense Technology
    National University of Defense Technology)

Abstract

Strong field ionization injects a transient vacancy in the atom which is entangled to the outgoing photoelectron. When the electron is finally detached, the ion is populated at different excited states with part of coherence information lost. The preserved coherence of matter after interacting with intense short pulses has important consequences on the subsequent nonequilibrium evolution and energy relaxation. Here we employ attosecond transient absorption spectroscopy to measure the time-delay of resonant transitions of krypton vacancy during their creation. We have observed that the absorptions by the two spin-orbit split states are modulated at different paces when varying the time-delay between the near-infrared pumping pulse and the attosecond probing pulse. It is shown that the coupling of the ions with the remaining field leads to a suppression of ionic coherence. Comparison between theory and experiments uncovers that coherent Raman coupling induces time-delay between the resonant absorptions, which provides insight into laser-ion interactions enriching attosecond chronoscopy.

Suggested Citation

  • Li Wang & Guangru Bai & Xiaowei Wang & Jing Zhao & Cheng Gao & Jiacan Wang & Fan Xiao & Wenkai Tao & Pan Song & Qianyu Qiu & Jinlei Liu & Zengxiu Zhao, 2024. "Raman time-delay in attosecond transient absorption of strong-field created krypton vacancy," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
  • Handle: RePEc:nat:natcom:v:15:y:2024:i:1:d:10.1038_s41467-024-47088-9
    DOI: 10.1038/s41467-024-47088-9
    as

    Download full text from publisher

    File URL: https://www.nature.com/articles/s41467-024-47088-9
    File Function: Abstract
    Download Restriction: no

    File URL: https://libkey.io/10.1038/s41467-024-47088-9?utm_source=ideas
    LibKey link: if access is restricted and if your library uses this service, LibKey will redirect you to where you can use your library subscription to access this item
    ---><---

    References listed on IDEAS

    as
    1. M. Uiberacker & Th. Uphues & M. Schultze & A. J. Verhoef & V. Yakovlev & M. F. Kling & J. Rauschenberger & N. M. Kabachnik & H. Schröder & M. Lezius & K. L. Kompa & H.-G. Muller & M. J. J. Vrakking & , 2007. "Attosecond real-time observation of electron tunnelling in atoms," Nature, Nature, vol. 446(7136), pages 627-632, April.
    2. M. Drescher & M. Hentschel & R. Kienberger & M. Uiberacker & V. Yakovlev & A. Scrinzi & Th. Westerwalbesloh & U. Kleineberg & U. Heinzmann & F. Krausz, 2002. "Time-resolved atomic inner-shell spectroscopy," Nature, Nature, vol. 419(6909), pages 803-807, October.
    3. Eleftherios Goulielmakis & Zhi-Heng Loh & Adrian Wirth & Robin Santra & Nina Rohringer & Vladislav S. Yakovlev & Sergey Zherebtsov & Thomas Pfeifer & Abdallah M. Azzeer & Matthias F. Kling & Stephen R, 2010. "Real-time observation of valence electron motion," Nature, Nature, vol. 466(7307), pages 739-743, August.
    4. Hongbin Lei & Jinping Yao & Jing Zhao & Hongqiang Xie & Fangbo Zhang & He Zhang & Ning Zhang & Guihua Li & Qian Zhang & Xiaowei Wang & Yan Yang & Luqi Yuan & Ya Cheng & Zengxiu Zhao, 2022. "Ultraviolet supercontinuum generation driven by ionic coherence in a strong laser field," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    5. Olga Smirnova & Yann Mairesse & Serguei Patchkovskii & Nirit Dudovich & David Villeneuve & Paul Corkum & Misha Yu. Ivanov, 2009. "High harmonic interferometry of multi-electron dynamics in molecules," Nature, Nature, vol. 460(7258), pages 972-977, August.
    6. U. Satya Sainadh & Han Xu & Xiaoshan Wang & A. Atia-Tul-Noor & William C. Wallace & Nicolas Douguet & Alexander Bray & Igor Ivanov & Klaus Bartschat & Anatoli Kheifets & R. T. Sang & I. V. Litvinyuk, 2019. "Author Correction: Attosecond angular streaking and tunnelling time in atomic hydrogen," Nature, Nature, vol. 569(7756), pages 5-5, May.
    7. A. L. Cavalieri & N. Müller & Th. Uphues & V. S. Yakovlev & A. Baltuška & B. Horvath & B. Schmidt & L. Blümel & R. Holzwarth & S. Hendel & M. Drescher & U. Kleineberg & P. M. Echenique & R. Kienberger, 2007. "Attosecond spectroscopy in condensed matter," Nature, Nature, vol. 449(7165), pages 1029-1032, October.
    8. U. Satya Sainadh & Han Xu & Xiaoshan Wang & A. Atia-Tul-Noor & William C. Wallace & Nicolas Douguet & Alexander Bray & Igor Ivanov & Klaus Bartschat & Anatoli Kheifets & R. T. Sang & I. V. Litvinyuk, 2019. "Attosecond angular streaking and tunnelling time in atomic hydrogen," Nature, Nature, vol. 568(7750), pages 75-77, April.
    9. J. Freudenstein & M. Borsch & M. Meierhofer & D. Afanasiev & C. P. Schmid & F. Sandner & M. Liebich & A. Girnghuber & M. Knorr & M. Kira & R. Huber, 2022. "Attosecond clocking of correlations between Bloch electrons," Nature, Nature, vol. 610(7931), pages 290-295, October.
    10. M. Ossiander & J. Riemensberger & S. Neppl & M. Mittermair & M. Schäffer & A. Duensing & M. S. Wagner & R. Heider & M. Wurzer & M. Gerl & M. Schnitzenbaumer & J. V. Barth & F. Libisch & C. Lemell & J., 2018. "Absolute timing of the photoelectric effect," Nature, Nature, vol. 561(7723), pages 374-377, September.
    Full references (including those not matched with items on IDEAS)

    Most related items

    These are the items that most often cite the same works as this one and are cited by the same works as this one.
    1. Lixin He & Siqi Sun & Pengfei Lan & Yanqing He & Bincheng Wang & Pu Wang & Xiaosong Zhu & Liang Li & Wei Cao & Peixiang Lu & C. D. Lin, 2022. "Filming movies of attosecond charge migration in single molecules with high harmonic spectroscopy," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    2. Yudong Yang & Roland E. Mainz & Giulio Maria Rossi & Fabian Scheiba & Miguel A. Silva-Toledo & Phillip D. Keathley & Giovanni Cirmi & Franz X. Kärtner, 2021. "Strong-field coherent control of isolated attosecond pulse generation," Nature Communications, Nature, vol. 12(1), pages 1-8, December.
    3. Álvaro Jiménez-Galán & Chandler Bossaer & Guilmot Ernotte & Andrew M. Parks & Rui E. F. Silva & David M. Villeneuve & André Staudte & Thomas Brabec & Adina Luican-Mayer & Giulio Vampa, 2023. "Orbital perspective on high-harmonic generation from solids," Nature Communications, Nature, vol. 14(1), pages 1-6, December.
    4. Wenyu Jiang & Gregory S. J. Armstrong & Jihong Tong & Yidan Xu & Zitan Zuo & Junjie Qiang & Peifen Lu & Daniel D. A. Clarke & Jakub Benda & Avner Fleischer & Hongcheng Ni & Kiyoshi Ueda & Hugo W. Hart, 2022. "Atomic partial wave meter by attosecond coincidence metrology," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    5. Peipei Ge & Yankun Dou & Meng Han & Yiqi Fang & Yongkai Deng & Chengyin Wu & Qihuang Gong & Yunquan Liu, 2024. "Spatiotemporal imaging and shaping of electron wave functions using novel attoclock interferometry," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    6. Pengcheng Chen & Dingxin Fan & Annabella Selloni & Emily A. Carter & Craig B. Arnold & Yunlong Zhang & Adam S. Gross & James R. Chelikowsky & Nan Yao, 2023. "Observation of electron orbital signatures of single atoms within metal-phthalocyanines using atomic force microscopy," Nature Communications, Nature, vol. 14(1), pages 1-7, December.
    7. Hongbin Lei & Jinping Yao & Jing Zhao & Hongqiang Xie & Fangbo Zhang & He Zhang & Ning Zhang & Guihua Li & Qian Zhang & Xiaowei Wang & Yan Yang & Luqi Yuan & Ya Cheng & Zengxiu Zhao, 2022. "Ultraviolet supercontinuum generation driven by ionic coherence in a strong laser field," Nature Communications, Nature, vol. 13(1), pages 1-9, December.

    More about this item

    Statistics

    Access and download statistics

    Corrections

    All material on this site has been provided by the respective publishers and authors. You can help correct errors and omissions. When requesting a correction, please mention this item's handle: RePEc:nat:natcom:v:15:y:2024:i:1:d:10.1038_s41467-024-47088-9. See general information about how to correct material in RePEc.

    If you have authored this item and are not yet registered with RePEc, we encourage you to do it here. This allows to link your profile to this item. It also allows you to accept potential citations to this item that we are uncertain about.

    If CitEc recognized a bibliographic reference but did not link an item in RePEc to it, you can help with this form .

    If you know of missing items citing this one, you can help us creating those links by adding the relevant references in the same way as above, for each refering item. If you are a registered author of this item, you may also want to check the "citations" tab in your RePEc Author Service profile, as there may be some citations waiting for confirmation.

    For technical questions regarding this item, or to correct its authors, title, abstract, bibliographic or download information, contact: Sonal Shukla or Springer Nature Abstracting and Indexing (email available below). General contact details of provider: http://www.nature.com .

    Please note that corrections may take a couple of weeks to filter through the various RePEc services.

    IDEAS is a RePEc service. RePEc uses bibliographic data supplied by the respective publishers.