IDEAS home Printed from https://ideas.repec.org/a/nat/natcom/v13y2022i1d10.1038_s41467-022-32753-8.html
   My bibliography  Save this article

Atomic partial wave meter by attosecond coincidence metrology

Author

Listed:
  • Wenyu Jiang

    (East China Normal University)

  • Gregory S. J. Armstrong

    (Queen’s University Belfast)

  • Jihong Tong

    (East China Normal University)

  • Yidan Xu

    (East China Normal University)

  • Zitan Zuo

    (East China Normal University)

  • Junjie Qiang

    (East China Normal University)

  • Peifen Lu

    (East China Normal University)

  • Daniel D. A. Clarke

    (School of Physics and CRANN Institute, Trinity College Dublin)

  • Jakub Benda

    (Institute of Theoretical Physics, Faculty of Mathematics and Physics, Charles University)

  • Avner Fleischer

    (Tel Aviv University)

  • Hongcheng Ni

    (East China Normal University
    Shanxi University)

  • Kiyoshi Ueda

    (East China Normal University)

  • Hugo W. Hart

    (Queen’s University Belfast)

  • Andrew C. Brown

    (Queen’s University Belfast)

  • Xiaochun Gong

    (East China Normal University
    Shanxi University)

  • Jian Wu

    (East China Normal University
    Shanxi University
    CAS Center for Excellence in Ultra-intense Laser Science)

Abstract

Attosecond chronoscopy is central to the understanding of ultrafast electron dynamics in matter from gas to the condensed phase with attosecond temporal resolution. It has, however, not yet been possible to determine the timing of individual partial waves, and steering their contribution has been a substantial challenge. Here, we develop a polarization-skewed attosecond chronoscopy serving as a partial wave meter to reveal the role of each partial wave from the angle-resolved photoionization phase shifts in rare gas atoms. We steer the relative ratio between different partial waves and realize a magnetic-sublevel-resolved atomic phase shift measurement. Our experimental observations are well supported by time-dependent R-matrix numerical simulations and analytical soft-photon approximation analysis. The symmetry-resolved, partial-wave analysis identifies the transition rate and phase shift property in the attosecond photoelectron emission dynamics. Our findings provide critical insights into the ubiquitous attosecond optical timer and the underlying attosecond photoionization dynamics.

Suggested Citation

  • Wenyu Jiang & Gregory S. J. Armstrong & Jihong Tong & Yidan Xu & Zitan Zuo & Junjie Qiang & Peifen Lu & Daniel D. A. Clarke & Jakub Benda & Avner Fleischer & Hongcheng Ni & Kiyoshi Ueda & Hugo W. Hart, 2022. "Atomic partial wave meter by attosecond coincidence metrology," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
  • Handle: RePEc:nat:natcom:v:13:y:2022:i:1:d:10.1038_s41467-022-32753-8
    DOI: 10.1038/s41467-022-32753-8
    as

    Download full text from publisher

    File URL: https://www.nature.com/articles/s41467-022-32753-8
    File Function: Abstract
    Download Restriction: no

    File URL: https://libkey.io/10.1038/s41467-022-32753-8?utm_source=ideas
    LibKey link: if access is restricted and if your library uses this service, LibKey will redirect you to where you can use your library subscription to access this item
    ---><---

    References listed on IDEAS

    as
    1. A. L. Cavalieri & N. Müller & Th. Uphues & V. S. Yakovlev & A. Baltuška & B. Horvath & B. Schmidt & L. Blümel & R. Holzwarth & S. Hendel & M. Drescher & U. Kleineberg & P. M. Echenique & R. Kienberger, 2007. "Attosecond spectroscopy in condensed matter," Nature, Nature, vol. 449(7165), pages 1029-1032, October.
    2. Xiaochun Gong & Saijoscha Heck & Denis Jelovina & Conaill Perry & Kristina Zinchenko & Robert Lucchese & Hans Jakob Wörner, 2022. "Attosecond spectroscopy of size-resolved water clusters," Nature, Nature, vol. 609(7927), pages 507-511, September.
    Full references (including those not matched with items on IDEAS)

    Most related items

    These are the items that most often cite the same works as this one and are cited by the same works as this one.
    1. Li Wang & Guangru Bai & Xiaowei Wang & Jing Zhao & Cheng Gao & Jiacan Wang & Fan Xiao & Wenkai Tao & Pan Song & Qianyu Qiu & Jinlei Liu & Zengxiu Zhao, 2024. "Raman time-delay in attosecond transient absorption of strong-field created krypton vacancy," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
    2. Xiaochun Gong & Étienne Plésiat & Alicia Palacios & Saijoscha Heck & Fernando Martín & Hans Jakob Wörner, 2023. "Attosecond delays between dissociative and non-dissociative ionization of polyatomic molecules," Nature Communications, Nature, vol. 14(1), pages 1-8, December.

    More about this item

    Statistics

    Access and download statistics

    Corrections

    All material on this site has been provided by the respective publishers and authors. You can help correct errors and omissions. When requesting a correction, please mention this item's handle: RePEc:nat:natcom:v:13:y:2022:i:1:d:10.1038_s41467-022-32753-8. See general information about how to correct material in RePEc.

    If you have authored this item and are not yet registered with RePEc, we encourage you to do it here. This allows to link your profile to this item. It also allows you to accept potential citations to this item that we are uncertain about.

    If CitEc recognized a bibliographic reference but did not link an item in RePEc to it, you can help with this form .

    If you know of missing items citing this one, you can help us creating those links by adding the relevant references in the same way as above, for each refering item. If you are a registered author of this item, you may also want to check the "citations" tab in your RePEc Author Service profile, as there may be some citations waiting for confirmation.

    For technical questions regarding this item, or to correct its authors, title, abstract, bibliographic or download information, contact: Sonal Shukla or Springer Nature Abstracting and Indexing (email available below). General contact details of provider: http://www.nature.com .

    Please note that corrections may take a couple of weeks to filter through the various RePEc services.

    IDEAS is a RePEc service. RePEc uses bibliographic data supplied by the respective publishers.