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Multiple-core-hole resonance spectroscopy with ultraintense X-ray pulses

Author

Listed:
  • Aljoscha Rörig

    (European XFEL
    Universität Hamburg)

  • Sang-Kil Son

    (Deutsches Elektronen-Synchrotron DESY)

  • Tommaso Mazza

    (European XFEL)

  • Philipp Schmidt

    (European XFEL)

  • Thomas M. Baumann

    (European XFEL)

  • Benjamin Erk

    (Deutsches Elektronen-Synchrotron DESY)

  • Markus Ilchen

    (European XFEL
    Deutsches Elektronen-Synchrotron DESY
    Universität Kassel)

  • Joakim Laksman

    (European XFEL)

  • Valerija Music

    (European XFEL
    Deutsches Elektronen-Synchrotron DESY
    Universität Kassel)

  • Shashank Pathak

    (Kansas State University)

  • Daniel E. Rivas

    (European XFEL)

  • Daniel Rolles

    (Kansas State University)

  • Svitozar Serkez

    (European XFEL)

  • Sergey Usenko

    (European XFEL)

  • Robin Santra

    (Universität Hamburg
    Deutsches Elektronen-Synchrotron DESY)

  • Michael Meyer

    (European XFEL)

  • Rebecca Boll

    (European XFEL)

Abstract

Understanding the interaction of intense, femtosecond X-ray pulses with heavy atoms is crucial for gaining insights into the structure and dynamics of matter. One key aspect of nonlinear light–matter interaction was, so far, not studied systematically at free-electron lasers—its dependence on the photon energy. Here, we use resonant ion spectroscopy to map out the transient electronic structures occurring during the complex charge-up pathways of xenon. Massively hollow atoms featuring up to six simultaneous core holes determine the spectra at specific photon energies and charge states. We also illustrate how different X-ray pulse parameters, which are usually intertwined, can be partially disentangled. The extraction of resonance spectra is facilitated by the possibility of working with a constant number of photons per X-ray pulse at all photon energies and the fact that the ion yields become independent of the peak fluence beyond a saturation point. Our study lays the groundwork for spectroscopic investigations of transient atomic species in exotic, multiple-core-hole states that have not been explored previously.

Suggested Citation

  • Aljoscha Rörig & Sang-Kil Son & Tommaso Mazza & Philipp Schmidt & Thomas M. Baumann & Benjamin Erk & Markus Ilchen & Joakim Laksman & Valerija Music & Shashank Pathak & Daniel E. Rivas & Daniel Rolles, 2023. "Multiple-core-hole resonance spectroscopy with ultraintense X-ray pulses," Nature Communications, Nature, vol. 14(1), pages 1-10, December.
  • Handle: RePEc:nat:natcom:v:14:y:2023:i:1:d:10.1038_s41467-023-41505-1
    DOI: 10.1038/s41467-023-41505-1
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    References listed on IDEAS

    as
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