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Strong bulk photovoltaic effect in engineered edge-embedded van der Waals structures

Author

Listed:
  • Zihan Liang

    (Southern University of Science and Technology)

  • Xin Zhou

    (National University of Singapore)

  • Le Zhang

    (Southern University of Science and Technology)

  • Xiang-Long Yu

    (Southern University of Science and Technology
    International Quantum Academy)

  • Yan Lv

    (Nanjing Tech University (NanjingTech))

  • Xuefen Song

    (Nanjing Tech University (NanjingTech))

  • Yongheng Zhou

    (Southern University of Science and Technology)

  • Han Wang

    (Southern University of Science and Technology)

  • Shuo Wang

    (Nanjing Tech University (NanjingTech))

  • Taihong Wang

    (Southern University of Science and Technology)

  • Perry Ping Shum

    (Southern University of Science and Technology)

  • Qian He

    (National University of Singapore)

  • Yanjun Liu

    (Southern University of Science and Technology)

  • Chao Zhu

    (Southeast University)

  • Lin Wang

    (Nanjing Tech University (NanjingTech))

  • Xiaolong Chen

    (Southern University of Science and Technology)

Abstract

Bulk photovoltaic effect (BPVE), a second-order nonlinear optical effect governed by the quantum geometric properties of materials, offers a promising approach to overcome the Shockley-Quiesser limit of traditional photovoltaic effect and further improve the efficiency of energy harvesting. Here, we propose an effective platform, the nano edges embedded in assembled van der Waals (vdW) homo- or hetero-structures with strong symmetry breaking, low dimensionality and abundant species, for BPVE investigations. The BPVE-induced photocurrents strongly depend on the orientation of edge-embedded structures and polarization of incident light. Reversed photocurrent polarity can be observed at left and right edge-embedded structures. Our work not only visualizes the unique optoelectronic effect in vdW nano edges, but also provides an effective strategy for achieving BPVE in engineered vdW structures.

Suggested Citation

  • Zihan Liang & Xin Zhou & Le Zhang & Xiang-Long Yu & Yan Lv & Xuefen Song & Yongheng Zhou & Han Wang & Shuo Wang & Taihong Wang & Perry Ping Shum & Qian He & Yanjun Liu & Chao Zhu & Lin Wang & Xiaolong, 2023. "Strong bulk photovoltaic effect in engineered edge-embedded van der Waals structures," Nature Communications, Nature, vol. 14(1), pages 1-9, December.
    • Handle: RePEc:nat:natcom:v:14:y:2023:i:1:d:10.1038_s41467-023-39995-0
    DOI: 10.1038/s41467-023-39995-0
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    Cited by:

    1. Yongheng Zhou & Xin Zhou & Xiang-Long Yu & Zihan Liang & Xiaoxu Zhao & Taihong Wang & Jinshui Miao & Xiaolong Chen, 2024. "Giant intrinsic photovoltaic effect in one-dimensional van der Waals grain boundaries," Nature Communications, Nature, vol. 15(1), pages 1-7, December.
    2. Zhouxiaosong Zeng & Zhiqiang Tian & Yufan Wang & Cuihuan Ge & Fabian Strauß & Kai Braun & Patrick Michel & Lanyu Huang & Guixian Liu & Dong Li & Marcus Scheele & Mingxing Chen & Anlian Pan & Xiao Wang, 2024. "Dual polarization-enabled ultrafast bulk photovoltaic response in van der Waals heterostructures," Nature Communications, Nature, vol. 15(1), pages 1-9, December.

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