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Direct nano-imaging of light-matter interactions in nanoscale excitonic emitters

Author

Listed:
  • Kiyoung Jo

    (University of Pennsylvania)

  • Emanuele Marino

    (University of Pennsylvania
    Università degli Studi di Palermo)

  • Jason Lynch

    (University of Pennsylvania)

  • Zhiqiao Jiang

    (University of Pennsylvania
    University of Pennsylvania)

  • Natalie Gogotsi

    (University of Pennsylvania)

  • Thomas P. Darlington

    (Columbia University)

  • Mohammad Soroush

    (Montana State University)

  • P. James Schuck

    (Columbia University)

  • Nicholas J. Borys

    (Montana State University)

  • Christopher B. Murray

    (University of Pennsylvania
    University of Pennsylvania)

  • Deep Jariwala

    (University of Pennsylvania)

Abstract

Strong light-matter interactions in localized nano-emitters placed near metallic mirrors have been widely reported via spectroscopic studies in the optical far-field. Here, we report a near-field nano-spectroscopic study of localized nanoscale emitters on a flat Au substrate. Using quasi 2-dimensional CdSe/CdxZn1-xS nanoplatelets, we observe directional propagation on the Au substrate of surface plasmon polaritons launched from the excitons of the nanoplatelets as wave-like fringe patterns in the near-field photoluminescence maps. These fringe patterns were confirmed via extensive electromagnetic wave simulations to be standing-waves formed between the tip and the edge-up assembled nano-emitters on the substrate plane. We further report that both light confinement and in-plane emission can be engineered by tuning the surrounding dielectric environment of the nanoplatelets. Our results lead to renewed understanding of in-plane, near-field electromagnetic signal transduction from the localized nano-emitters with profound implications in nano and quantum photonics as well as resonant optoelectronics.

Suggested Citation

  • Kiyoung Jo & Emanuele Marino & Jason Lynch & Zhiqiao Jiang & Natalie Gogotsi & Thomas P. Darlington & Mohammad Soroush & P. James Schuck & Nicholas J. Borys & Christopher B. Murray & Deep Jariwala, 2023. "Direct nano-imaging of light-matter interactions in nanoscale excitonic emitters," Nature Communications, Nature, vol. 14(1), pages 1-10, December.
    • Handle: RePEc:nat:natcom:v:14:y:2023:i:1:d:10.1038_s41467-023-38189-y
    DOI: 10.1038/s41467-023-38189-y
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