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Giant piezoresistivity in a van der Waals material induced by intralayer atomic motions

Author

Listed:
  • Lingyun Tang

    (South China University of Technology, Guangzhou)

  • Zhongquan Mao

    (South China University of Technology, Guangzhou)

  • Chutian Wang

    (Monash University)

  • Qi Fu

    (Westlake University)

  • Chen Wang

    (Westlake University)

  • Yichi Zhang

    (Westlake University)

  • Jingyi Shen

    (Westlake University)

  • Yuefeng Yin

    (Monash University)

  • Bin Shen

    (Zhejiang University)

  • Dayong Tan

    (Chinese Academy of Sciences)

  • Qian Li

    (Liaocheng University)

  • Yonggang Wang

    (Center for High Pressure Science and Technology Advanced Research (HPSTAR))

  • Nikhil V. Medhekar

    (Monash University)

  • Jie Wu

    (Westlake University)

  • Huiqiu Yuan

    (Zhejiang University)

  • Yanchun Li

    (Chinese Academy of Sciences)

  • Michael S. Fuhrer

    (Monash University)

  • Changxi Zheng

    (Westlake University)

Abstract

The presence of the van der Waals gap in layered materials creates a wealth of intriguing phenomena different to their counterparts in conventional materials. For example, pressurization can generate a large anisotropic lattice shrinkage along the stacking orientation and/or a significant interlayer sliding, and many of the exotic pressure-dependent properties derive from these mechanisms. Here we report a giant piezoresistivity in pressurized β′-In2Se3. Upon compression, a six-orders-of-magnitude drop of electrical resistivity is obtained below 1.2 GPa in β′-In2Se3 flakes, yielding a giant piezoresistive gauge πp of −5.33 GPa−1. Simultaneously, the sample undergoes a semiconductor-to-semimetal transition without a structural phase transition. Surprisingly, linear dichroism study and theoretical first principles modelling show that these phenomena arise not due to shrinkage or sliding at the van der Waals gap, but rather are dominated by the layer-dependent atomic motions inside the quintuple layer, mainly from the shifting of middle Se atoms to their high-symmetric location. The atomic motions link to both the band structure modulation and the in-plane ferroelectric dipoles. Our work not only provides a prominent piezoresistive material but also points out the importance of intralayer atomic motions beyond van der Waals gap.

Suggested Citation

  • Lingyun Tang & Zhongquan Mao & Chutian Wang & Qi Fu & Chen Wang & Yichi Zhang & Jingyi Shen & Yuefeng Yin & Bin Shen & Dayong Tan & Qian Li & Yonggang Wang & Nikhil V. Medhekar & Jie Wu & Huiqiu Yuan , 2023. "Giant piezoresistivity in a van der Waals material induced by intralayer atomic motions," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
  • Handle: RePEc:nat:natcom:v:14:y:2023:i:1:d:10.1038_s41467-023-37239-9
    DOI: 10.1038/s41467-023-37239-9
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    1. Yuan Cao & Valla Fatemi & Shiang Fang & Kenji Watanabe & Takashi Taniguchi & Efthimios Kaxiras & Pablo Jarillo-Herrero, 2018. "Unconventional superconductivity in magic-angle graphene superlattices," Nature, Nature, vol. 556(7699), pages 43-50, April.
    2. Zefang Wang & Daniel A. Rhodes & Kenji Watanabe & Takashi Taniguchi & James C. Hone & Jie Shan & Kin Fai Mak, 2019. "Evidence of high-temperature exciton condensation in two-dimensional atomic double layers," Nature, Nature, vol. 574(7776), pages 76-80, October.
    3. Yanpeng Qi & Pavel G. Naumov & Mazhar N. Ali & Catherine R. Rajamathi & Walter Schnelle & Oleg Barkalov & Michael Hanfland & Shu-Chun Wu & Chandra Shekhar & Yan Sun & Vicky Süß & Marcus Schmidt & Ulri, 2016. "Superconductivity in Weyl semimetal candidate MoTe2," Nature Communications, Nature, vol. 7(1), pages 1-7, April.
    4. Chen Wang & Qiyuan He & Udayabagya Halim & Yuanyue Liu & Enbo Zhu & Zhaoyang Lin & Hai Xiao & Xidong Duan & Ziying Feng & Rui Cheng & Nathan O. Weiss & Guojun Ye & Yun-Chiao Huang & Hao Wu & Hung-Chie, 2018. "Monolayer atomic crystal molecular superlattices," Nature, Nature, vol. 555(7695), pages 231-236, March.
    5. Defen Kang & Yazhou Zhou & Wei Yi & Chongli Yang & Jing Guo & Youguo Shi & Shan Zhang & Zhe Wang & Chao Zhang & Sheng Jiang & Aiguo Li & Ke Yang & Qi Wu & Guangming Zhang & Liling Sun & Zhongxian Zhao, 2015. "Superconductivity emerging from a suppressed large magnetoresistant state in tungsten ditelluride," Nature Communications, Nature, vol. 6(1), pages 1-6, November.
    6. Zhao Zhao & Haijun Zhang & Hongtao Yuan & Shibing Wang & Yu Lin & Qiaoshi Zeng & Gang Xu & Zhenxian Liu & G. K. Solanki & K. D. Patel & Yi Cui & Harold Y. Hwang & Wendy L. Mao, 2015. "Pressure induced metallization with absence of structural transition in layered molybdenum diselenide," Nature Communications, Nature, vol. 6(1), pages 1-8, November.
    7. Chao Xu & Jianfeng Mao & Xuyun Guo & Shanru Yan & Yancong Chen & Tsz Wing Lo & Changsheng Chen & Dangyuan Lei & Xin Luo & Jianhua Hao & Changxi Zheng & Ye Zhu, 2021. "Two-dimensional ferroelasticity in van der Waals β’-In2Se3," Nature Communications, Nature, vol. 12(1), pages 1-9, December.
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