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Coemissive luminescent nanoparticles combining aggregation-induced emission and quenching dyes prepared in continuous flow

Author

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  • Chong Li

    (Dalian University of Technology
    Dalian University of Technology)

  • Qi Liu

    (Dalian University of Technology)

  • Shengyang Tao

    (Dalian University of Technology
    Dalian University of Technology)

Abstract

Achieving an ideal light-harvesting system at a low cost remains a challenge. Herein, we report the synthesis of a hybrid dye system based on tetraphenylene (TPE) encapsulated organic dyes in a continuous flow microreactor. The composite dye nanoparticles (NPs) are synthesized based on supramolecular self-assembly to achieve the co-emission of aggregation-induced emission dyes and aggregation-caused quenching dyes (CEAA). Numerical simulations and molecular spectroscopy were used to investigate the synthesis mechanism of the CEAA dyes. Nanoparticles of CEAA dyes provide a platform for efficient cascade Förster resonance energy transfer (FRET). Composite dye nanoparticles of TPE and Nile red (NiR) are synthesized for an ideal light-harvesting system using coumarin 6 (C-6) as an energy intermediate. The light-harvesting system has a considerable red-shift distance (~126 nm), high energy-transfer efficiency (ΦET) of 99.37%, and an antenna effect of 26.23. Finally, the versatility of the preparation method and the diversity of CEAA dyes are demonstrated.

Suggested Citation

  • Chong Li & Qi Liu & Shengyang Tao, 2022. "Coemissive luminescent nanoparticles combining aggregation-induced emission and quenching dyes prepared in continuous flow," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    • Handle: RePEc:nat:natcom:v:13:y:2022:i:1:d:10.1038_s41467-022-33857-x
    DOI: 10.1038/s41467-022-33857-x
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    References listed on IDEAS

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    1. Håkan Nilsson & Fabrice Rappaport & Alain Boussac & Johannes Messinger, 2014. "Substrate–water exchange in photosystem II is arrested before dioxygen formation," Nature Communications, Nature, vol. 5(1), pages 1-7, September.
    2. Inès Massiot & Andrea Cattoni & Stéphane Collin, 2020. "Progress and prospects for ultrathin solar cells," Nature Energy, Nature, vol. 5(12), pages 959-972, December.
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    Cited by:

    1. Bin Mu & Xiangnan Hao & Xiao Luo & Zhongke Yang & Huanjun Lu & Wei Tian, 2024. "Bioinspired polymeric supramolecular columns as efficient yet controllable artificial light-harvesting platform," Nature Communications, Nature, vol. 15(1), pages 1-10, December.

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