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Inducing and tuning Kondo screening in a narrow-electronic-band system

Author

Listed:
  • Shiwei Shen

    (ShanghaiTech University)

  • Chenhaoping Wen

    (ShanghaiTech University)

  • Pengfei Kong

    (ShanghaiTech University)

  • Jingjing Gao

    (Institute of Solid State Physics, HFIPS, Chinese Academy of Sciences
    University of Science and Technology of China)

  • Jianguo Si

    (Institute of Solid State Physics, HFIPS, Chinese Academy of Sciences)

  • Xuan Luo

    (Institute of Solid State Physics, HFIPS, Chinese Academy of Sciences)

  • Wenjian Lu

    (Institute of Solid State Physics, HFIPS, Chinese Academy of Sciences)

  • Yuping Sun

    (Institute of Solid State Physics, HFIPS, Chinese Academy of Sciences
    High Magnetic Field Laboratory, HFIPS, Chinese Academy of Sciences
    Nanjing University)

  • Gang Chen

    (The University of Hong Kong)

  • Shichao Yan

    (ShanghaiTech University
    ShanghaiTech University)

Abstract

Although the single-impurity Kondo physics has already been well understood, the understanding of the Kondo lattice where a dense array of local moments couples to the conduction electrons is still far from complete. The ability of creating and tuning the Kondo lattice in non-f-electron systems will be great helpful for further understanding the Kondo lattice behavior. Here we show that the Pb intercalation in the charge-density-wave-driven narrow-electronic-band system 1T-TaS2 induces a transition from the insulating gap to a sharp Kondo resonance in the scanning tunneling microscopy measurements. It results from the Kondo screening of the localized moments in the 13-site Star-of-David clusters of 1T-TaS2. As increasing the Pb concentration, the narrow electronic band derived from the localized electrons shifts away from the Fermi level and the Kondo resonance peak is gradually suppressed. Our results pave the way for creating and tuning many-body electronic states in layered narrow-electronic-band materials.

Suggested Citation

  • Shiwei Shen & Chenhaoping Wen & Pengfei Kong & Jingjing Gao & Jianguo Si & Xuan Luo & Wenjian Lu & Yuping Sun & Gang Chen & Shichao Yan, 2022. "Inducing and tuning Kondo screening in a narrow-electronic-band system," Nature Communications, Nature, vol. 13(1), pages 1-7, December.
  • Handle: RePEc:nat:natcom:v:13:y:2022:i:1:d:10.1038_s41467-022-29891-4
    DOI: 10.1038/s41467-022-29891-4
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    1. Y. D. Wang & W. L. Yao & Z. M. Xin & T. T. Han & Z. G. Wang & L. Chen & C. Cai & Yuan Li & Y. Zhang, 2020. "Band insulator to Mott insulator transition in 1T-TaS2," Nature Communications, Nature, vol. 11(1), pages 1-7, December.
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    2. W. Simeth & Z. Wang & E. A. Ghioldi & D. M. Fobes & A. Podlesnyak & N. H. Sung & E. D. Bauer & J. Lass & S. Flury & J. Vonka & D. G. Mazzone & C. Niedermayer & Yusuke Nomura & Ryotaro Arita & C. D. Ba, 2023. "A microscopic Kondo lattice model for the heavy fermion antiferromagnet CeIn3," Nature Communications, Nature, vol. 14(1), pages 1-10, December.
    3. Quanzhen Zhang & Wen-Yu He & Yu Zhang & Yaoyao Chen & Liangguang Jia & Yanhui Hou & Hongyan Ji & Huixia Yang & Teng Zhang & Liwei Liu & Hong-Jun Gao & Thomas A. Jung & Yeliang Wang, 2024. "Quantum spin liquid signatures in monolayer 1T-NbSe2," Nature Communications, Nature, vol. 15(1), pages 1-10, December.
    4. Wen Wan & Rishav Harsh & Antonella Meninno & Paul Dreher & Sandra Sajan & Haojie Guo & Ion Errea & Fernando Juan & Miguel M. Ugeda, 2023. "Evidence for ground state coherence in a two-dimensional Kondo lattice," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    5. Zhen-Yu Liu & Heng Jin & Yao Zhang & Kai Fan & Ting-Fei Guo & Hao-Jun Qin & Lan-Fang Zhu & Lian-Zhi Yang & Wen-Hao Zhang & Bing Huang & Ying-Shuang Fu, 2024. "Charge-density wave mediated quasi-one-dimensional Kondo lattice in stripe-phase monolayer 1T-NbSe2," Nature Communications, Nature, vol. 15(1), pages 1-8, December.

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