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General technoeconomic analysis for electrochemical coproduction coupling carbon dioxide reduction with organic oxidation

Author

Listed:
  • Jonggeol Na

    (Korea Institute of Science and Technology (KIST)
    Carnegie Mellon University)

  • Bora Seo

    (Korea Institute of Science and Technology (KIST))

  • Jeongnam Kim

    (Korea Institute of Science and Technology (KIST)
    Seoul National University)

  • Chan Woo Lee

    (Kookmin University)

  • Hyunjoo Lee

    (Korea Institute of Science and Technology (KIST)
    Korea University of Science and Technology (UST))

  • Yun Jeong Hwang

    (Korea Institute of Science and Technology (KIST)
    Korea University of Science and Technology (UST)
    Yonsei University)

  • Byoung Koun Min

    (Korea Institute of Science and Technology (KIST)
    Green School, Korea University)

  • Dong Ki Lee

    (Korea Institute of Science and Technology (KIST))

  • Hyung-Suk Oh

    (Korea Institute of Science and Technology (KIST)
    Korea University of Science and Technology (UST))

  • Ung Lee

    (Korea Institute of Science and Technology (KIST)
    Korea University of Science and Technology (UST)
    Green School, Korea University)

Abstract

Electrochemical processes coupling carbon dioxide reduction reactions with organic oxidation reactions are promising techniques for producing clean chemicals and utilizing renewable energy. However, assessments of the economics of the coupling technology remain questionable due to diverse product combinations and significant process design variability. Here, we report a technoeconomic analysis of electrochemical carbon dioxide reduction reaction–organic oxidation reaction coproduction via conceptual process design and thereby propose potential economic combinations. We first develop a fully automated process synthesis framework to guide process simulations, which are then employed to predict the levelized costs of chemicals. We then identify the global sensitivity of current density, Faraday efficiency, and overpotential across 295 electrochemical coproduction processes to both understand and predict the levelized costs of chemicals at various technology levels. The analysis highlights the promise that coupling the carbon dioxide reduction reaction with the value-added organic oxidation reaction can secure significant economic feasibility.

Suggested Citation

  • Jonggeol Na & Bora Seo & Jeongnam Kim & Chan Woo Lee & Hyunjoo Lee & Yun Jeong Hwang & Byoung Koun Min & Dong Ki Lee & Hyung-Suk Oh & Ung Lee, 2019. "General technoeconomic analysis for electrochemical coproduction coupling carbon dioxide reduction with organic oxidation," Nature Communications, Nature, vol. 10(1), pages 1-13, December.
    • Handle: RePEc:nat:natcom:v:10:y:2019:i:1:d:10.1038_s41467-019-12744-y
    DOI: 10.1038/s41467-019-12744-y
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    Cited by:

    1. Ke Xie & Adnan Ozden & Rui Kai Miao & Yuhang Li & David Sinton & Edward H. Sargent, 2022. "Eliminating the need for anodic gas separation in CO2 electroreduction systems via liquid-to-liquid anodic upgrading," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    2. Jun Qi & Yadong Du & Qi Yang & Na Jiang & Jiachun Li & Yi Ma & Yangjun Ma & Xin Zhao & Jieshan Qiu, 2023. "Energy-saving and product-oriented hydrogen peroxide electrosynthesis enabled by electrochemistry pairing and product engineering," Nature Communications, Nature, vol. 14(1), pages 1-12, December.
    3. Shengqin Liu & Yangxin Jin & Shuquan Huang & Qi Zhu & Shan Shao & Jason Chun-Ho Lam, 2024. "One-pot redox cascade paired electrosynthesis of gamma-butyrolactone from furoic acid," Nature Communications, Nature, vol. 15(1), pages 1-11, December.
    4. Xiaoyi Jiang & Le Ke & Kai Zhao & Xiaoyu Yan & Hongbo Wang & Xiaojuan Cao & Yuchen Liu & Lingjiao Li & Yifei Sun & Zhiping Wang & Dai Dang & Ning Yan, 2024. "Integrating hydrogen utilization in CO2 electrolysis with reduced energy loss," Nature Communications, Nature, vol. 15(1), pages 1-12, December.
    5. Pribyl-Kranewitter, B. & Beard, A. & Gîjiu, C.L. & Dinculescu, D. & Schmidt, T.J., 2022. "Influence of low-temperature electrolyser design on economic and environmental potential of CO and HCOOH production: A techno-economic assessment," Renewable and Sustainable Energy Reviews, Elsevier, vol. 154(C).
    6. Young-Jin Ko & Chulwan Lim & Junyoung Jin & Min Gyu Kim & Ji Yeong Lee & Tae-Yeon Seong & Kwan-Young Lee & Byoung Koun Min & Jae-Young Choi & Taegeun Noh & Gyu Weon Hwang & Woong Hee Lee & Hyung-Suk O, 2024. "Extrinsic hydrophobicity-controlled silver nanoparticles as efficient and stable catalysts for CO2 electrolysis," Nature Communications, Nature, vol. 15(1), pages 1-11, December.
    7. Yuyang Pan & Huiyan Zhang & Bowen Zhang & Feng Gong & Jianyong Feng & Huiting Huang & Srinivas Vanka & Ronglei Fan & Qi Cao & Mingrong Shen & Zhaosheng Li & Zhigang Zou & Rui Xiao & Sheng Chu, 2023. "Renewable formate from sunlight, biomass and carbon dioxide in a photoelectrochemical cell," Nature Communications, Nature, vol. 14(1), pages 1-10, December.
    8. Kezia Megagita Gerby Langie & Kyungjae Tak & Changsoo Kim & Hee Won Lee & Kwangho Park & Dongjin Kim & Wonsang Jung & Chan Woo Lee & Hyung-Suk Oh & Dong Ki Lee & Jai Hyun Koh & Byoung Koun Min & Da Hy, 2022. "Toward economical application of carbon capture and utilization technology with near-zero carbon emission," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
    9. Fenghui Ye & Shishi Zhang & Qingqing Cheng & Yongde Long & Dong Liu & Rajib Paul & Yunming Fang & Yaqiong Su & Liangti Qu & Liming Dai & Chuangang Hu, 2023. "The role of oxygen-vacancy in bifunctional indium oxyhydroxide catalysts for electrochemical coupling of biomass valorization with CO2 conversion," Nature Communications, Nature, vol. 14(1), pages 1-14, December.
    10. Ruiz-López, Estela & Gandara-Loe, Jesús & Baena-Moreno, Francisco & Reina, Tomas Ramirez & Odriozola, José Antonio, 2022. "Electrocatalytic CO2 conversion to C2 products: Catalysts design, market perspectives and techno-economic aspects," Renewable and Sustainable Energy Reviews, Elsevier, vol. 161(C).
    11. Kannangara, Miyuru & Shadbahr, Jalil & Vasudev, Madhav & Yang, Jianjun & Zhang, Lei & Bensebaa, Farid & Lees, Eric & Simpson, Grace & Berlinguette, Curtis & Cai, Jingjing & Nishikawa, Emily & McCoy, S, 2022. "A standardized methodology for economic and carbon footprint assessment of CO2 to transport fuels: Comparison of novel bicarbonate electrolysis with competing pathways," Applied Energy, Elsevier, vol. 325(C).

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