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Cotreatment of MSWI Fly Ash and Granulated Lead Smelting Slag Using a Geopolymer System

Author

Listed:
  • De-Gang Liu

    (Institute of Environmental Science and Engineering, School of Metallurgy and Environment, Central South University, Changsha 410083, Hunan, China)

  • Yong Ke

    (Institute of Environmental Science and Engineering, School of Metallurgy and Environment, Central South University, Changsha 410083, Hunan, China
    Chinese National Engineering Research Center for Control and Treatment of Heavy Metal Pollution, Changsha 410083, Hunan, China)

  • Xiao-Bo Min

    (Institute of Environmental Science and Engineering, School of Metallurgy and Environment, Central South University, Changsha 410083, Hunan, China
    Chinese National Engineering Research Center for Control and Treatment of Heavy Metal Pollution, Changsha 410083, Hunan, China)

  • Yan-Jie Liang

    (Institute of Environmental Science and Engineering, School of Metallurgy and Environment, Central South University, Changsha 410083, Hunan, China
    Chinese National Engineering Research Center for Control and Treatment of Heavy Metal Pollution, Changsha 410083, Hunan, China)

  • Zhong-Bing Wang

    (Institute of Environmental Science and Engineering, School of Metallurgy and Environment, Central South University, Changsha 410083, Hunan, China)

  • Yuan-Cheng Li

    (Institute of Environmental Science and Engineering, School of Metallurgy and Environment, Central South University, Changsha 410083, Hunan, China)

  • Jiang-Chi Fei

    (Institute of Environmental Science and Engineering, School of Metallurgy and Environment, Central South University, Changsha 410083, Hunan, China)

  • Li-Wei Yao

    (Institute of Environmental Science and Engineering, School of Metallurgy and Environment, Central South University, Changsha 410083, Hunan, China)

  • Hui Xu

    (Institute of Environmental Science and Engineering, School of Metallurgy and Environment, Central South University, Changsha 410083, Hunan, China)

  • Guang-Hua Jiang

    (Institute of Environmental Science and Engineering, School of Metallurgy and Environment, Central South University, Changsha 410083, Hunan, China)

Abstract

Municipal solid waste incineration fly ash (MSWI FA) and granulated lead smelting slag (GLSS) are toxic industrial wastes. In the present study, granulated lead smelting slag (GLSS) was pretreated as a geopolymer precursor through the high-energy ball milling activation process, which could be used as a geopolymeric solidification/stabilization (S/S) reagent for MSWI FA. The S/S process has been estimated through the physical properties and heavy metals leachability of the S/S matrices. The results show that the compressive strength of the geopolymer matrix reaches 15.32 MPa after curing for 28 days under the best parameters, and the physical properties meet the requirement of MU10 grade fly ash brick. In addition, the toxicity characteristic leaching procedure (TCLP) test results show that arsenic and heavy metals are immobilized effectively in the geopolymer matrix, and their concentrations in the leachate are far below the US EPA TCLP limits. The hydration products of the geopolymer binder are characterized by X-ray diffraction and Fourier transform infrared methods. The results show that the geopolymer gel and Friedel’s salt are the main hydration products. The S/S mechanism of the arsenic and heavy metals in the geopolymer matrix mainly involves physical encapsulation of the geopolymer gel, geopolymer adsorption and ion exchange of Friedel’s salt.

Suggested Citation

  • De-Gang Liu & Yong Ke & Xiao-Bo Min & Yan-Jie Liang & Zhong-Bing Wang & Yuan-Cheng Li & Jiang-Chi Fei & Li-Wei Yao & Hui Xu & Guang-Hua Jiang, 2019. "Cotreatment of MSWI Fly Ash and Granulated Lead Smelting Slag Using a Geopolymer System," IJERPH, MDPI, vol. 16(1), pages 1-12, January.
    • Handle: RePEc:gam:jijerp:v:16:y:2019:i:1:p:156-:d:195739
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    References listed on IDEAS

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    1. Liwei Yao & Xiaobo Min & Hui Xu & Yong Ke & Yanjie Liang & Kang Yang, 2018. "Hydrothermal Treatment of Arsenic Sulfide Residues from Arsenic-Bearing Acid Wastewater," IJERPH, MDPI, vol. 15(9), pages 1-15, August.
    2. Charles H. K. Lam & Alvin W. M. Ip & John Patrick Barford & Gordon McKay, 2010. "Use of Incineration MSW Ash: A Review," Sustainability, MDPI, vol. 2(7), pages 1-26, July.
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    Cited by:

    1. Le Song & Feng Zhao & Haiyang Cui & Jingmin Wan & Hui Li, 2023. "Biofuel Ash Aging in Acidic Environment and Its Influence on Cd Immobilization," IJERPH, MDPI, vol. 20(5), pages 1-16, March.
    2. Liwei Yao & Degang Liu & Yong Ke & Yuancheng Li & Zhongbing Wang & Jiangchi Fei & Hui Xu & Xiaobo Min, 2020. "Synthesis and Hydration Characteristic of Geopolymer Based on Lead Smelting Slag," IJERPH, MDPI, vol. 17(8), pages 1-12, April.
    3. Marija Štulović & Dragana Radovanović & Željko Kamberović & Marija Korać & Zoran Anđić, 2019. "Assessment of Leaching Characteristics of Solidified Products Containing Secondary Alkaline Lead Slag," IJERPH, MDPI, vol. 16(11), pages 1-16, June.

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