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Unveiling the Potential of Cryogenic Post-Combustion Carbon Capture: From Fundamentals to Innovative Processes

Author

Listed:
  • Mauro Luberti

    (Department of Chemical Engineering, School of Engineering, The University of Manchester, Oxford Road, Manchester M13 9PL, UK)

  • Erika Ballini

    (Research Unit of Process Engineering, Department of Science & Technology for Sustainable Development & One Health, University Campus Bio-Medico di Roma, Via Alvaro del Portillo, 21, 00128 Rome, Italy)

  • Mauro Capocelli

    (Research Unit of Process Engineering, Department of Science & Technology for Sustainable Development & One Health, University Campus Bio-Medico di Roma, Via Alvaro del Portillo, 21, 00128 Rome, Italy)

Abstract

Climate change necessitates urgent actions to mitigate carbon dioxide (CO 2 ) emissions from fossil fuel-based energy generation. Among various strategies, the deployment of carbon capture and storage (CCS) solutions is critical for reducing emissions from point sources such as power plants and heavy industries. In this context, cryogenic carbon capture (CCC) via desublimation has emerged as a promising technology. While CCC offers high separation efficiency, minimal downstream compression work, and integration potential with existing industrial processes, challenges such as low operating temperatures and equipment costs persist. Ongoing research aims to address these hurdles in order to optimize the desublimation processes for widespread implementation. This review consolidates diverse works from the literature, providing insights into the strengths and limitations of CCC technology, including the latest pilot plant scale demonstrations. The transformative potential of CCC is first assessed on a theoretical basis, such as thermodynamic aspects and mass transfer phenomena. Then, recent advancements in the proposed process configurations are critically assessed and compared through key performance indicators. Furthermore, future research directions for this technology are clearly highlighted.

Suggested Citation

  • Mauro Luberti & Erika Ballini & Mauro Capocelli, 2024. "Unveiling the Potential of Cryogenic Post-Combustion Carbon Capture: From Fundamentals to Innovative Processes," Energies, MDPI, vol. 17(11), pages 1-24, May.
    • Handle: RePEc:gam:jeners:v:17:y:2024:i:11:p:2673-:d:1406163
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    References listed on IDEAS

    as
    1. David Cann & Carolina Font-Palma, 2023. "Evaluation of Mathematical Models for CO 2 Frost Formation in a Cryogenic Moving Bed," Energies, MDPI, vol. 16(5), pages 1-14, February.
    2. Barbara Koelbl & Machteld Broek & André Faaij & Detlef Vuuren, 2014. "Uncertainty in Carbon Capture and Storage (CCS) deployment projections: a cross-model comparison exercise," Climatic Change, Springer, vol. 123(3), pages 461-476, April.
    3. Hossein Asgharian & Florin Iov & Samuel Simon Araya & Thomas Helmer Pedersen & Mads Pagh Nielsen & Ehsan Baniasadi & Vincenzo Liso, 2023. "A Review on Process Modeling and Simulation of Cryogenic Carbon Capture for Post-Combustion Treatment," Energies, MDPI, vol. 16(4), pages 1-35, February.
    4. Safdarnejad, Seyed Mostafa & Hedengren, John D. & Baxter, Larry L., 2015. "Plant-level dynamic optimization of Cryogenic Carbon Capture with conventional and renewable power sources," Applied Energy, Elsevier, vol. 149(C), pages 354-366.
    5. Mauro Luberti & Alexander Brown & Marco Balsamo & Mauro Capocelli, 2022. "Numerical Analysis of VPSA Technology Retrofitted to Steam Reforming Hydrogen Plants to Capture CO 2 and Produce Blue H 2," Energies, MDPI, vol. 15(3), pages 1-18, February.
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