IDEAS home Printed from https://ideas.repec.org/a/gam/jeners/v15y2022i19p7433-d937900.html
   My bibliography  Save this article

On the Possibility of Cleaning Producer Gas Laden with Large Quantities of Tars through Using a Simple Fixed-Bed Activated Carbon Adsorption Process

Author

Listed:
  • Mateusz Kochel

    (Institute for Energy and Fuel Processing Technology (ITPE), Zamkowa 1, 41-803 Zabrze, Poland)

  • Mateusz Szul

    (Institute for Energy and Fuel Processing Technology (ITPE), Zamkowa 1, 41-803 Zabrze, Poland)

  • Tomasz Iluk

    (Institute for Energy and Fuel Processing Technology (ITPE), Zamkowa 1, 41-803 Zabrze, Poland)

  • Jan Najser

    (ENET Centre, VSB-Technical University of Ostrava, 17. listopadu 2172/15, 708 00 Ostrava, Czech Republic)

Abstract

The study presents the results of research on using fixed-bed, activated carbon (AC) adsorbers in the cleaning of heavily tar-laden producer gas from the gasification of biomass. The efficiency of removal of organic compounds as well as the remaining adsorption capacity of the bed were determined using a spectrum of commonly applied diagnostic methods, including qualitative and quantitative analyses of the adsorbed compounds and changes in the pore volume of the bed material (IN, MN). The authors compare these lab quantifications with a simple technique which is based on the analysis of the changes in the position of temperature front in the bed. The main benefit of the latter is the possibility of performing the diagnostics of the bed “online” and using low-cost temperature measurements. The test was performed using a commercially available AC Desotec AIRPEL 10-3 and real producer gas obtained through the gasification of alder chips. For tar, VOC and C 2 –C 5 compounds, the removal efficiencies reached respectively 74.5%-wt., 52.8%-wt., and 85.5%-wt. Obtained results indicate that depending on the final application of the gas, the use of dry adsorption systems is an interesting alternative to the well-established but complicated, cumbersome, and costly wet scrubbers. Moreover, a concept for in situ regeneration of the adsorbent, coupled with direct reforming of the tars, is presented and discussed.

Suggested Citation

  • Mateusz Kochel & Mateusz Szul & Tomasz Iluk & Jan Najser, 2022. "On the Possibility of Cleaning Producer Gas Laden with Large Quantities of Tars through Using a Simple Fixed-Bed Activated Carbon Adsorption Process," Energies, MDPI, vol. 15(19), pages 1-19, October.
  • Handle: RePEc:gam:jeners:v:15:y:2022:i:19:p:7433-:d:937900
    as

    Download full text from publisher

    File URL: https://www.mdpi.com/1996-1073/15/19/7433/pdf
    Download Restriction: no

    File URL: https://www.mdpi.com/1996-1073/15/19/7433/
    Download Restriction: no
    ---><---

    References listed on IDEAS

    as
    1. Bai, Zhang & Liu, Qibin & Gong, Liang & Lei, Jing, 2019. "Investigation of a solar-biomass gasification system with the production of methanol and electricity: Thermodynamic, economic and off-design operation," Applied Energy, Elsevier, vol. 243(C), pages 91-101.
    2. Liu, Yigang & Li, Guoxuan & Chen, Zhengrun & Shen, Yuanyuan & Zhang, Hongru & Wang, Shuai & Qi, Jianguang & Zhu, Zhaoyou & Wang, Yinglong & Gao, Jun, 2020. "Comprehensive analysis of environmental impacts and energy consumption of biomass-to-methanol and coal-to-methanol via life cycle assessment," Energy, Elsevier, vol. 204(C).
    3. Clausen, Lasse R. & Butera, Giacomo & Jensen, Søren Højgaard, 2019. "High efficiency SNG production from biomass and electricity by integrating gasification with pressurized solid oxide electrolysis cells," Energy, Elsevier, vol. 172(C), pages 1117-1131.
    4. Nakamura, Shunsuke & Kitano, Shigeru & Yoshikawa, Kunio, 2016. "Biomass gasification process with the tar removal technologies utilizing bio-oil scrubber and char bed," Applied Energy, Elsevier, vol. 170(C), pages 186-192.
    5. Kotowicz, Janusz & Sobolewski, Aleksander & Iluk, Tomasz, 2013. "Energetic analysis of a system integrated with biomass gasification," Energy, Elsevier, vol. 52(C), pages 265-278.
    6. Harris, Kylee & Grim, R. Gary & Huang, Zhe & Tao, Ling, 2021. "A comparative techno-economic analysis of renewable methanol synthesis from biomass and CO2: Opportunities and barriers to commercialization," Applied Energy, Elsevier, vol. 303(C).
    7. Giulio Allesina & Simone Pedrazzi, 2021. "Barriers to Success: A Technical Review on the Limits and Possible Future Roles of Small Scale Gasifiers," Energies, MDPI, vol. 14(20), pages 1-23, October.
    8. Shahbeik, Hossein & Peng, Wanxi & Kazemi Shariat Panahi, Hamed & Dehhaghi, Mona & Guillemin, Gilles J. & Fallahi, Alireza & Amiri, Hamid & Rehan, Mohammad & Raikwar, Deepak & Latine, Hannes & Pandalon, 2022. "Synthesis of liquid biofuels from biomass by hydrothermal gasification: A critical review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 167(C).
    9. Marchese, Marco & Chesta, Simone & Santarelli, Massimo & Lanzini, Andrea, 2021. "Techno-economic feasibility of a biomass-to-X plant: Fischer-Tropsch wax synthesis from digestate gasification," Energy, Elsevier, vol. 228(C).
    10. Mateusz Szul & Tomasz Iluk & Aleksander Sobolewski, 2020. "High-Temperature, Dry Scrubbing of Syngas with Use of Mineral Sorbents and Ceramic Rigid Filters," Energies, MDPI, vol. 13(6), pages 1-22, March.
    Full references (including those not matched with items on IDEAS)

    Most related items

    These are the items that most often cite the same works as this one and are cited by the same works as this one.
    1. Li, Jiaxuan & Zhu, Xun & Djilali, Ned & Yang, Yang & Ye, Dingding & Chen, Rong & Liao, Qiang, 2022. "Comparative well-to-pump assessment of fueling pathways for zero-carbon transportation in China: Hydrogen economy or methanol economy?," Renewable and Sustainable Energy Reviews, Elsevier, vol. 169(C).
    2. Mateusz Szul & Tomasz Iluk & Aleksander Sobolewski, 2020. "High-Temperature, Dry Scrubbing of Syngas with Use of Mineral Sorbents and Ceramic Rigid Filters," Energies, MDPI, vol. 13(6), pages 1-22, March.
    3. Chengjiang Li & Tingwen Jia & Shiyuan Wang & Xiaolin Wang & Michael Negnevitsky & Honglei Wang & Yujie Hu & Weibin Xu & Na Zhou & Gang Zhao, 2023. "Methanol Vehicles in China: A Review from a Policy Perspective," Sustainability, MDPI, vol. 15(12), pages 1-22, June.
    4. Tabibian, Seyed Shayan & Sharifzadeh, Mahdi, 2023. "Statistical and analytical investigation of methanol applications, production technologies, value-chain and economy with a special focus on renewable methanol," Renewable and Sustainable Energy Reviews, Elsevier, vol. 179(C).
    5. Zhou, Xin & Yan, Hao & Sun, Zongzhuang & Feng, Xiang & Zhao, Hui & Liu, Yibin & Chen, Xiaobo & Yang, Chaohe, 2021. "Opportunities for utilizing waste cooking oil in crude to petrochemical process: Novel process design, optimal strategy, techno-economic analysis and life cycle society-environment assessment," Energy, Elsevier, vol. 237(C).
    6. Chu, Genyun & Fan, Yingjie & Zhang, Dawei & Gao, Minglin & Yu, Jianhua & Xie, Jianhui & Yang, Qingchun, 2022. "A highly efficient and environmentally friendly approach for in-situ utilization of CO2 from coal to ethylene glycol plant," Energy, Elsevier, vol. 256(C).
    7. Adnan, Muflih A. & Hossain, Mohammad M. & Kibria, Md Golam, 2020. "Biomass upgrading to high-value chemicals via gasification and electrolysis: A thermodynamic analysis," Renewable Energy, Elsevier, vol. 162(C), pages 1367-1379.
    8. Robert Wejkowski & Sylwester Kalisz & Mateusz Tymoszuk & Szymon Ciukaj & Izabella Maj, 2021. "Full-Scale Investigation of Dry Sorbent Injection for NO x Emission Control and Mercury Retention," Energies, MDPI, vol. 14(22), pages 1-13, November.
    9. Janusz-Szymańska, Katarzyna & Dryjańska, Aleksandra, 2015. "Possibilities for improving the thermodynamic and economic characteristics of an oxy-type power plant with a cryogenic air separation unit," Energy, Elsevier, vol. 85(C), pages 45-61.
    10. Bai, Zhang & Gu, Yucheng & Wang, Shuoshuo & Jiang, Tieliu & Kong, Debin & Li, Qi, 2023. "Applying the solar solid particles as heat carrier to enhance the solar-driven biomass gasification with dynamic operation power generation performance analysis," Applied Energy, Elsevier, vol. 351(C).
    11. Zhang, Hanfei & Wang, Ligang & Van herle, Jan & Maréchal, François & Desideri, Umberto, 2020. "Techno-economic evaluation of biomass-to-fuels with solid-oxide electrolyzer," Applied Energy, Elsevier, vol. 270(C).
    12. Gabriele Calì & Paolo Deiana & Claudia Bassano & Simone Meloni & Enrico Maggio & Michele Mascia & Alberto Pettinau, 2020. "Syngas Production, Clean-Up and Wastewater Management in a Demo-Scale Fixed-Bed Updraft Biomass Gasification Unit," Energies, MDPI, vol. 13(10), pages 1-15, May.
    13. Rajat Kumar Sharma & Mohammad Ali Nazari & Juma Haydary & Triveni Prasad Singh & Sandip Mandal, 2023. "A Review on Advanced Processes of Biohydrogen Generation from Lignocellulosic Biomass with Special Emphasis on Thermochemical Conversion," Energies, MDPI, vol. 16(17), pages 1-27, September.
    14. Bartela, Łukasz & Kotowicz, Janusz & Dubiel-Jurgaś, Klaudia, 2018. "Investment risk for biomass integrated gasification combined heat and power unit with an internal combustion engine and a Stirling engine," Energy, Elsevier, vol. 150(C), pages 601-616.
    15. Janusz Kotowicz & Sebastian Michalski & Mateusz Brzęczek, 2019. "The Characteristics of a Modern Oxy-Fuel Power Plant," Energies, MDPI, vol. 12(17), pages 1-34, September.
    16. Bai, Zhang & Liu, Qibin & Gong, Liang & Lei, Jing, 2019. "Application of a mid-/low-temperature solar thermochemical technology in the distributed energy system with cooling, heating and power production," Applied Energy, Elsevier, vol. 253(C), pages 1-1.
    17. Kobori, Takahiro & Yoshikawa, Kunio & Ismail, Tamer M. & Yasser, T.M. & García, Abraham Castro & Kanazawa, Kiryu & Takahashi, Fumitake, 2022. "Effect of electron injection on oxidative pyrolysis of cellulose and polypropylene," Applied Energy, Elsevier, vol. 326(C).
    18. AlNouss, Ahmed & Parthasarathy, Prakash & Shahbaz, Muhammad & Al-Ansari, Tareq & Mackey, Hamish & McKay, Gordon, 2020. "Techno-economic and sensitivity analysis of coconut coir pith-biomass gasification using ASPEN PLUS," Applied Energy, Elsevier, vol. 261(C).
    19. Hervy, Maxime & Weiss-Hortala, Elsa & Pham Minh, Doan & Dib, Hadi & Villot, Audrey & Gérente, Claire & Berhanu, Sarah & Chesnaud, Anthony & Thorel, Alain & Le Coq, Laurence & Nzihou, Ange, 2019. "Reactivity and deactivation mechanisms of pyrolysis chars from bio-waste during catalytic cracking of tar," Applied Energy, Elsevier, vol. 237(C), pages 487-499.
    20. Xin, Yu & Xing, Xueli & Li, Xiang & Hong, Hui, 2024. "A biomass–solar hybrid gasification system by solar pyrolysis and PV– Solid oxide electrolysis cell for sustainable fuel production," Applied Energy, Elsevier, vol. 356(C).

    Corrections

    All material on this site has been provided by the respective publishers and authors. You can help correct errors and omissions. When requesting a correction, please mention this item's handle: RePEc:gam:jeners:v:15:y:2022:i:19:p:7433-:d:937900. See general information about how to correct material in RePEc.

    If you have authored this item and are not yet registered with RePEc, we encourage you to do it here. This allows to link your profile to this item. It also allows you to accept potential citations to this item that we are uncertain about.

    If CitEc recognized a bibliographic reference but did not link an item in RePEc to it, you can help with this form .

    If you know of missing items citing this one, you can help us creating those links by adding the relevant references in the same way as above, for each refering item. If you are a registered author of this item, you may also want to check the "citations" tab in your RePEc Author Service profile, as there may be some citations waiting for confirmation.

    For technical questions regarding this item, or to correct its authors, title, abstract, bibliographic or download information, contact: MDPI Indexing Manager (email available below). General contact details of provider: https://www.mdpi.com .

    Please note that corrections may take a couple of weeks to filter through the various RePEc services.

    IDEAS is a RePEc service. RePEc uses bibliographic data supplied by the respective publishers.