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The Crystal Structures in Hydrogen Absorption Reactions of REMgNi 4 -Based Alloys (RE: Rare-Earth Metals)

Author

Listed:
  • Toyoto Sato

    (Department of Engineering Science and Mechanics, College of Engineering, Shibaura Institute of Technology, Tokyo 135-8548, Japan)

  • Shin-ichi Orimo

    (Advanced Institute for Materials Research (WPI-AIMR), Tohoku University, Sendai 980-8577, Japan
    Institute for Materials Research, Tohoku University, Sendai 980-8577, Japan)

Abstract

REMgNi 4 -based alloys, RE (2−x) Mg x Ni 4 (RE: rare-earth metals; 0 < x < 2), with a AuBe 5 -type crystal structure, exhibit reversible hydrogen absorption and desorption reactions, which are known as hydrogen storage properties. These reactions involve formation of three hydride phases. The hydride formation pressures and hydrogen storage capacities are related to the radii of the RE (2−x) Mg x Ni 4 , which in turn are dependent on the radii and compositional ratios of the RE and Mg atoms. The crystal structures formed during hydrogen absorption reactions are the key to understanding the hydrogen storage properties of RE (2−x) Mg x Ni 4 . Therefore, in this review, we provide an overview of the crystal structures in the hydrogen absorption reactions focusing on RE (2−x) Mg x Ni 4 .

Suggested Citation

  • Toyoto Sato & Shin-ichi Orimo, 2021. "The Crystal Structures in Hydrogen Absorption Reactions of REMgNi 4 -Based Alloys (RE: Rare-Earth Metals)," Energies, MDPI, vol. 14(23), pages 1-10, December.
    • Handle: RePEc:gam:jeners:v:14:y:2021:i:23:p:8163-:d:695705
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    References listed on IDEAS

    as
    1. Louis Schlapbach & Andreas Züttel, 2001. "Hydrogen-storage materials for mobile applications," Nature, Nature, vol. 414(6861), pages 353-358, November.
    2. Sangryun Kim & Hiroyuki Oguchi & Naoki Toyama & Toyoto Sato & Shigeyuki Takagi & Toshiya Otomo & Dorai Arunkumar & Naoaki Kuwata & Junichi Kawamura & Shin-ichi Orimo, 2019. "A complex hydride lithium superionic conductor for high-energy-density all-solid-state lithium metal batteries," Nature Communications, Nature, vol. 10(1), pages 1-9, December.
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