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Hydrogen Generation from Wood Chip and Biochar by Combined Continuous Pyrolysis and Hydrothermal Gasification

Author

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  • Bingyao Zeng

    (Graduate School of Agriculture, Hokkaido University, Sapporo 060-8589, Hokkaido, Japan)

  • Naoto Shimizu

    (Field Science Center for Northern Biosphere, Research Faculty of Agriculture, Hokkaido University, Sapporo 060-8589, Hokkaido, Japan)

Abstract

Hydrothermal gasification (HTG) experiments were carried out to extract hydrogen from biomass. Although extensive research has been conducted on hydrogen production with HTG, limited research exists on the use of biochar as a raw material. In this study, woodland residues (wood chip) and biochar from wood-chip pyrolysis were used in HTG treatment to generate hydrogen. This research investigated the effect of temperature (300–425 °C) and biomass/water (0.5–10) ratio on gas composition. A higher temperature promoted hydrogen production because the water–gas shift reaction and steam-reforming reaction were promoted with an increase in temperature. The methane concentration was related positively to temperature because of the methanation and hydrogenation reactions. A lower biomass/water ratio promoted hydrogen production but suppressed carbon-monoxide production. Most reactions that produce hydrogen consume water, but water also affects the water–gas shift reaction balance, which decreases the carbon-monoxide concentration. By focusing on the practical application of HTG, we attempted biochar treatment by pyrolysis (temperature of heating part: 700 °C), and syngas was obtained from hydrothermal treatment above 425 °C.

Suggested Citation

  • Bingyao Zeng & Naoto Shimizu, 2021. "Hydrogen Generation from Wood Chip and Biochar by Combined Continuous Pyrolysis and Hydrothermal Gasification," Energies, MDPI, vol. 14(13), pages 1-11, June.
    • Handle: RePEc:gam:jeners:v:14:y:2021:i:13:p:3793-:d:581221
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    References listed on IDEAS

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    1. Mohammad I. Jahirul & Mohammad G. Rasul & Ashfaque Ahmed Chowdhury & Nanjappa Ashwath, 2012. "Biofuels Production through Biomass Pyrolysis —A Technological Review," Energies, MDPI, vol. 5(12), pages 1-50, November.
    2. Akhtar, Javaid & Amin, Nor Aishah Saidina, 2011. "A review on process conditions for optimum bio-oil yield in hydrothermal liquefaction of biomass," Renewable and Sustainable Energy Reviews, Elsevier, vol. 15(3), pages 1615-1624, April.
    3. Ibrahim Shaba Mohammed & Risu Na & Keisuke Kushima & Naoto Shimizu, 2020. "Investigating the Effect of Processing Parameters on the Products of Hydrothermal Carbonization of Corn Stover," Sustainability, MDPI, vol. 12(12), pages 1-21, June.
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    1. Dmitrii Glushkov & Galina Nyashina & Anatolii Shvets & Amaro Pereira & Anand Ramanathan, 2021. "Current Status of the Pyrolysis and Gasification Mechanism of Biomass," Energies, MDPI, vol. 14(22), pages 1-24, November.
    2. Simone Marzeddu & Andrea Cappelli & Andrea Ambrosio & María Alejandra Décima & Paolo Viotti & Maria Rosaria Boni, 2021. "A Life Cycle Assessment of an Energy-Biochar Chain Involving a Gasification Plant in Italy," Land, MDPI, vol. 10(11), pages 1-29, November.

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