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Carbon based catalysts for the hydrodeoxygenation of lignin and related molecules: A powerful tool for the generation of non-petroleum chemical products including hydrocarbons

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  • Sharma, Vinit
  • Getahun, Tokuma
  • Verma, Minal
  • Villa, Alberto
  • Gupta, Neeraj

Abstract

Lignin has a complex aromatic framework that can be used to generate various aromatic compounds capable to replace chemicals (including hydrocarbon fuels) derived from unrefined oil. However, the selective cleavage of polymeric lignin to simpler molecules is a demanding task due to excessive oxygen content present in it. Hence, reducing the whole oxygen content from lignin by-products is necessary for their effective use. Hydrodeoxygenation is a process capable to reduce the overall oxygen content present in lignin with the support of hydrogen gas. Carbon materials deliver a good opportunity to design catalysts for hydrodeoxygenation by providing chemically inert surface and tunable functional groups to support the metal nanoparticles. The main objective of this work is to give an account on the use of carbon material supported heterogeneous catalysts for the HDO of lignin and related molecules for the synthesis of non-petroleum chemical products including hydrocarbons. Thus, this review presents a variety of carbon catalysts for performing the HDO reaction in lignin or its derivatives. The surface properties of the catalysts and mechanistic insights into the conversion with key active sites are provided, which will help the designing of new and effective catalysts for this biomass conversion.

Suggested Citation

  • Sharma, Vinit & Getahun, Tokuma & Verma, Minal & Villa, Alberto & Gupta, Neeraj, 2020. "Carbon based catalysts for the hydrodeoxygenation of lignin and related molecules: A powerful tool for the generation of non-petroleum chemical products including hydrocarbons," Renewable and Sustainable Energy Reviews, Elsevier, vol. 133(C).
    • Handle: RePEc:eee:rensus:v:133:y:2020:i:c:s1364032120305682
    DOI: 10.1016/j.rser.2020.110280
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    References listed on IDEAS

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    1. Bharathiraja, B. & Sudharsana, T. & Jayamuthunagai, J. & Praveenkumar, R. & Chozhavendhan, S. & Iyyappan, J., 2018. "Biogas production – A review on composition, fuel properties, feed stock and principles of anaerobic digestion," Renewable and Sustainable Energy Reviews, Elsevier, vol. 90(C), pages 570-582.
    2. Zhang, Xinghua & Tang, Wenwu & Zhang, Qi & Wang, Tiejun & Ma, Longlong, 2018. "Hydrodeoxygenation of lignin-derived phenoic compounds to hydrocarbon fuel over supported Ni-based catalysts," Applied Energy, Elsevier, vol. 227(C), pages 73-79.
    3. Joselin Herbert, G.M. & Unni Krishnan, A., 2016. "Quantifying environmental performance of biomass energy," Renewable and Sustainable Energy Reviews, Elsevier, vol. 59(C), pages 292-308.
    4. Li, Xiangping & Chen, Guanyi & Liu, Caixia & Ma, Wenchao & Yan, Beibei & Zhang, Jianguang, 2017. "Hydrodeoxygenation of lignin-derived bio-oil using molecular sieves supported metal catalysts: A critical review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 71(C), pages 296-308.
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    Cited by:

    1. Li, Tong & Li, Hao & Li, Chunli, 2022. "Self-support semi-hollow carbon nanosphere supported palladium catalyst for biomass upgrading," Renewable Energy, Elsevier, vol. 191(C), pages 101-109.
    2. Mingyuan Zhang & Xue Han & Huanang Wang & Yimin Zeng & Chunbao Charles Xu, 2023. "Hydrodeoxygenation of Pyrolysis Oil in Supercritical Ethanol with Formic Acid as an In Situ Hydrogen Source over NiMoW Catalysts Supported on Different Materials," Sustainability, MDPI, vol. 15(10), pages 1-15, May.

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