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Automatic operation of decoupled water electrolysis based on bipolar electrode

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  • Zhao, Meng-Jie
  • He, Qian
  • Xiang, Ting
  • Ya, Hua-Qin
  • Luo, Hao
  • Wan, Shanhong
  • Ding, Jun
  • He, Jian-Bo

Abstract

Electrolytic hydrogen production faces a technological issue of gas crossover through the ion-membrane between hydrogen and oxygen chambers, especially under renewable energy low power driving conditions. As a solution, decoupled water electrolysis was proposed and has made important progress in laboratory research but faces the problem of how to implement it in industry. The present work develops a decoupled alkaline water electrolysis system without the need to change the filter press structure of industrial electrolyzers. A wireless bipolar electrode was designed and prepared from a redox pair (NiOOH/Ni(OH)2), which functions as a substitute for conventional ion-membrane but enables complete blocking of the gas crossover (and ion transfer also) between the hydrogen and oxygen chambers. A matching control scheme was designed and implemented for continuous water electrolysis. The high purity hydrogen production achieved a coulombic efficiency of 99.2% and a specific electricity consumption of 57.5 kWh kg−1 H2 at a current density of 50 mA cm−2. This bipolar decoupling scheme of automatic operation makes an important step towards industrial implementation of decoupled water electrolysis technology.

Suggested Citation

  • Zhao, Meng-Jie & He, Qian & Xiang, Ting & Ya, Hua-Qin & Luo, Hao & Wan, Shanhong & Ding, Jun & He, Jian-Bo, 2023. "Automatic operation of decoupled water electrolysis based on bipolar electrode," Renewable Energy, Elsevier, vol. 203(C), pages 583-591.
    • Handle: RePEc:eee:renene:v:203:y:2023:i:c:p:583-591
    DOI: 10.1016/j.renene.2022.12.083
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    References listed on IDEAS

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    1. Hen Dotan & Avigail Landman & Stafford W. Sheehan & Kirtiman Deo Malviya & Gennady E. Shter & Daniel A. Grave & Ziv Arzi & Nachshon Yehudai & Manar Halabi & Netta Gal & Noam Hadari & Coral Cohen & Avn, 2019. "Decoupled hydrogen and oxygen evolution by a two-step electrochemical–chemical cycle for efficient overall water splitting," Nature Energy, Nature, vol. 4(9), pages 786-795, September.
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    5. Long Chen & Xiaoli Dong & Yonggang Wang & Yongyao Xia, 2016. "Separating hydrogen and oxygen evolution in alkaline water electrolysis using nickel hydroxide," Nature Communications, Nature, vol. 7(1), pages 1-8, September.
    6. Chen, Nannan & Du, Xiaoqiang & Zhang, Xiaoshuang, 2022. "Controlled synthesis of MnS/ZnS hybrid material with different morphology as efficient water and urea electrolysis catalyst," Renewable Energy, Elsevier, vol. 193(C), pages 715-724.
    7. Zhao, Meng-Jie & Li, Er-Mei & Deng, Ning & Hu, Yingjie & Li, Chao-Xiong & Li, Bing & Li, Fang & Guo, Zhen-Guo & He, Jian-Bo, 2022. "Indirect electrodeposition of a NiMo@Ni(OH)2MoOx composite catalyst for superior hydrogen production in acidic and alkaline electrolytes," Renewable Energy, Elsevier, vol. 191(C), pages 370-379.
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    1. Iesalnieks, Mairis & Vanags, Mārtiņš & Alsiņa, Linda Laima & Šutka, Andris, 2024. "Increasing the capacity of pseudocapacitive WO3 auxiliary electrode for enhanced two-step decoupled acid water electrolysis," Renewable Energy, Elsevier, vol. 228(C).

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