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Sustainable production of oxygen-rich hierarchically porous carbon network from corn straw lignin and silk degumming wastewater for high-performance electrochemical energy storage

Author

Listed:
  • Zhou, Man
  • Li, Kai
  • Hu, Jinguang
  • Tang, Liping
  • Li, Mingliu
  • Su, Lifang
  • Zhao, Hong
  • Ko, Frank
  • Cai, Zaisheng
  • Zhao, Yaping

Abstract

Herein, a clean, green, and sustainable strategy is presented to prepare a high-performance energy storage material, the sericin-lignin derived hierarchically porous carbon materials (SLHPCs). Extracted from biomass waste, corn straw lignin and sericin from silk degumming wastewater are endowed with a high added value. Combining the cross-linking reaction between lignin and sericin and the porogen role of sericin, the as-prepared SLHPC-2 possesses an advantageous pore structure, a high BET specific surface area (1948.4 m2 g−1) with a superior mesoporous area (598.6 m2 g−1). The high in-situ oxygen doping (14%) is simultaneously realized. It exhibits remarkable electrochemical properties and displays the universality in either alkali, acid, or neutral electrolytes as supercapacitor (SC) electrodes. The as-assembled symmetrical button-type SLHPC-based SC transmits a high energy density of 17.0 Wh kg−1 at a power density of 500.1 W kg−1 and retains 13.3 Wh kg−1 at 10.0 kW kg−1. The porogen role of sericin can be extended to be a universal fabrication of biomass wastes-based hierarchically porous carbon material. The proposed recycling strategy of biomass waste resources paves the way for new applications in energy storage.

Suggested Citation

  • Zhou, Man & Li, Kai & Hu, Jinguang & Tang, Liping & Li, Mingliu & Su, Lifang & Zhao, Hong & Ko, Frank & Cai, Zaisheng & Zhao, Yaping, 2022. "Sustainable production of oxygen-rich hierarchically porous carbon network from corn straw lignin and silk degumming wastewater for high-performance electrochemical energy storage," Renewable Energy, Elsevier, vol. 191(C), pages 141-150.
    • Handle: RePEc:eee:renene:v:191:y:2022:i:c:p:141-150
    DOI: 10.1016/j.renene.2022.04.037
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    References listed on IDEAS

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    1. Chen, Tingting & Luo, Lu & Luo, Lingcong & Deng, Jianping & Wu, Xi & Fan, Mizi & Du, Guanben & Weigang Zhao,, 2021. "High energy density supercapacitors with hierarchical nitrogen-doped porous carbon as active material obtained from bio-waste," Renewable Energy, Elsevier, vol. 175(C), pages 760-769.
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