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High energy density supercapacitors with hierarchical nitrogen-doped porous carbon as active material obtained from bio-waste

Author

Listed:
  • Chen, Tingting
  • Luo, Lu
  • Luo, Lingcong
  • Deng, Jianping
  • Wu, Xi
  • Fan, Mizi
  • Du, Guanben
  • Weigang Zhao,

Abstract

Supercapacitors (SCs) is a promising energy storage approach to solve the intermittent problems of most renewable energy sources. N-doped hierarchically activated porous carbon materials (ACBS) for supercapacitor applicaitons are obtained by pre-carbonization and KOH activation of N-rich sword bean shells. ACBS containing 1–2% of N show hierarchical porosity, very high surface area and pore volume (equal to 2917 m2/g and 1.73 cm3/g, respectively). These materials are incorporated into supercapacitors. The device containing ACBS obtained using 700 °C as a post-treatment temperature shows a very high specific capacity (equal to 264 F/g at 1 A/g), which remains high (∼180 F/g) even at 20 A/g current density. Corresponding symmetric coin-cell supercapacitor demonstrats 12.5 Wh/kg energy density at 100 W/kg power density. This cell is capable of maintaining its energy density at the 11.1 Wh/kg level at 5000 W/kg power density and demonstrats almost 100% capacity retention after one thousand 1 A/g charge/discharge cycles. Such superior electrochemical performance of devices fabricated using ACBS as active materials is possible because of synergy between electrical double-layer capacitance and faradaic pseudocapacitance, which strongly depend on the surface area, pore volume and size distribution as well as dopant of heteroatoams.

Suggested Citation

  • Chen, Tingting & Luo, Lu & Luo, Lingcong & Deng, Jianping & Wu, Xi & Fan, Mizi & Du, Guanben & Weigang Zhao,, 2021. "High energy density supercapacitors with hierarchical nitrogen-doped porous carbon as active material obtained from bio-waste," Renewable Energy, Elsevier, vol. 175(C), pages 760-769.
  • Handle: RePEc:eee:renene:v:175:y:2021:i:c:p:760-769
    DOI: 10.1016/j.renene.2021.05.006
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    References listed on IDEAS

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    1. González, Ander & Goikolea, Eider & Barrena, Jon Andoni & Mysyk, Roman, 2016. "Review on supercapacitors: Technologies and materials," Renewable and Sustainable Energy Reviews, Elsevier, vol. 58(C), pages 1189-1206.
    2. Yakaboylu, Gunes A. & Jiang, Changle & Yumak, Tugrul & Zondlo, John W. & Wang, Jingxin & Sabolsky, Edward M., 2021. "Engineered hierarchical porous carbons for supercapacitor applications through chemical pretreatment and activation of biomass precursors," Renewable Energy, Elsevier, vol. 163(C), pages 276-287.
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    2. Zhou, Man & Li, Kai & Hu, Jinguang & Tang, Liping & Li, Mingliu & Su, Lifang & Zhao, Hong & Ko, Frank & Cai, Zaisheng & Zhao, Yaping, 2022. "Sustainable production of oxygen-rich hierarchically porous carbon network from corn straw lignin and silk degumming wastewater for high-performance electrochemical energy storage," Renewable Energy, Elsevier, vol. 191(C), pages 141-150.
    3. Melkiyur, Isacfranklin & Rathinam, Yuvakkumar & Kumar, P. Senthil & Sankaiya, Asaithambi & Pitchaiya, Selvakumar & Ganesan, Ravi & Velauthapillai, Dhayalan, 2023. "A comprehensive review on novel quaternary metal oxide and sulphide electrode materials for supercapacitor: Origin, fundamentals, present perspectives and future aspects," Renewable and Sustainable Energy Reviews, Elsevier, vol. 173(C).
    4. Xu, He & Zhang, Yi & Wang, Liyuan & Chen, Ye & Gao, Shuyan, 2021. "Hierarchical porous biomass-derived carbon framework with ultrahigh surface area for outstanding capacitance supercapacitor," Renewable Energy, Elsevier, vol. 179(C), pages 1826-1835.
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