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Effects of carbon corrosion on proton exchange membrane fuel cell performance using two durability evaluation methods

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  • Sim, Jaebong
  • Kang, Minsoo
  • Min, Kyoungdoug
  • Lee, Eunsook
  • Jyoung, Jy-Young

Abstract

A gas diffusion layer (GDL) is a major component that facilitates the discharge of generated water and the diffusion of reactant gases in the proton-exchange-membrane fuel cell (PEMFC). However, the GDL is composed of carbon materials, and therefore, it is vulnerable to carbon corrosion. When the PEMFC is at start-up or shutdown, a reduction reaction is induced where a temporary hydrogen shortage phenomenon occurs in the anode region caused by the air flowing into the gaps of the fuel cell stacks from the outside and from the oxygen crossover through the membrane. This phenomenon induces the reaction of carbon and water at the cathode, and eventually, carbon materials are corroded by an oxidation reaction. In this study, two durability evaluation methods for inducing carbon corrosion are applied to investigate the carbon corrosion phenomenon and performance degradation systematically. The effects of the corroded GDL and corroded membrane electrode assembly on the PEMFC performance are independently identified, and the causes of performance degradation of the corroded GDL are quantitatively investigated.

Suggested Citation

  • Sim, Jaebong & Kang, Minsoo & Min, Kyoungdoug & Lee, Eunsook & Jyoung, Jy-Young, 2022. "Effects of carbon corrosion on proton exchange membrane fuel cell performance using two durability evaluation methods," Renewable Energy, Elsevier, vol. 190(C), pages 959-970.
    • Handle: RePEc:eee:renene:v:190:y:2022:i:c:p:959-970
    DOI: 10.1016/j.renene.2022.04.015
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    References listed on IDEAS

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    1. Cho, Junhyun & Park, Jaeman & Oh, Hwanyeong & Min, Kyoungdoug & Lee, Eunsook & Jyoung, Jy-Young, 2013. "Analysis of the transient response and durability characteristics of a proton exchange membrane fuel cell with different micro-porous layer penetration thicknesses," Applied Energy, Elsevier, vol. 111(C), pages 300-309.
    2. Chen, Ben & Wang, Jun & Yang, Tianqi & Cai, Yonghua & Zhang, Caizhi & Chan, Siew Hwa & Yu, Yi & Tu, Zhengkai, 2016. "Carbon corrosion and performance degradation mechanism in a proton exchange membrane fuel cell with dead-ended anode and cathode," Energy, Elsevier, vol. 106(C), pages 54-62.
    3. Chun, Jeong Hwan & Jo, Dong Hyun & Kim, Sang Gon & Park, Sun Hee & Lee, Chang Hoon & Kim, Sung Hyun, 2012. "Improvement of the mechanical durability of micro porous layer in a proton exchange membrane fuel cell by elimination of surface cracks," Renewable Energy, Elsevier, vol. 48(C), pages 35-41.
    4. Bolahaga Randrianarizafy & Pascal Schott & Mathias Gerard & Yann Bultel, 2020. "Modelling Carbon Corrosion during a PEMFC Startup: Simulation of Mitigation Strategies," Energies, MDPI, vol. 13(9), pages 1-17, May.
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    1. Sim, Jaebong & Kang, Minsoo & Kim, Jiwoong & Min, Kyoungdoug, 2022. "Effects of operating conditions, various properties of the gas diffusion layer, and shape of endplate on the open-cathode proton exchange membrane fuel cell performance," Renewable Energy, Elsevier, vol. 196(C), pages 40-51.
    2. Sim, Jaebong & Kang, Minsoo & Oh, Hwanyeong & Lee, Eunsook & Jyoung, Jy-Young & Min, Kyoungdoug, 2022. "The effect of gas diffusion layer on electrochemical effective reaction area of catalyst layer and water discharge capability," Renewable Energy, Elsevier, vol. 197(C), pages 932-942.
    3. Shi, Ting & Peng, Xueyuan & Feng, Jianmei & Guo, Yi & Wang, Bingsheng, 2024. "Study on the startup-shutdown performance of gas foil bearings-rotor system in proton exchange membrane fuel cells," Renewable Energy, Elsevier, vol. 226(C).

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