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Lewis acid-mediated aqueous glycerol pretreatment of sugarcane bagasse: Pretreatment recycling, one-pot hydrolysis and lignin properties

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  • Zhu, Yuan
  • Qi, Benkun
  • Liang, Xinquan
  • Luo, Jianquan
  • Wan, Yinhua

Abstract

Sugarcane bagasse was pretreated with lewis acid-mediated glycerol, results showed that 98.47% glucan recovery, 95.31% xylan removal and 49.69% delignification were achieved by pretreatment using 80 wt% aqueous glycerol combined with 1.0 wt% AlCl3 at 150 °C for 1 h. Reutilization experiments of acidified glycerol showed that its pretreatment efficiency was relatively well maintained during four consecutive cycles. Enzymatic in situ saccharification of pretreated bagasse led to about 50% glucose yield at 16 wt% glycerol concentration. After pretreatment, the lignin distributed in pretreatment hydrolysate and pretreated solid residue (referred to as organosolv lignin (OL) and cellulolytic enzyme lignin (CEL), respectively) demonstrated contrasting effect on enzymatic hydrolysis with OL slightly increasing while CEL decreasing cellulose conversion, which could be explained by their differences in hydrophobicity and surface charge. Further analysis of the structure and molecular weights of two lignin samples indicated their great potential for valorization into value-added products.

Suggested Citation

  • Zhu, Yuan & Qi, Benkun & Liang, Xinquan & Luo, Jianquan & Wan, Yinhua, 2021. "Lewis acid-mediated aqueous glycerol pretreatment of sugarcane bagasse: Pretreatment recycling, one-pot hydrolysis and lignin properties," Renewable Energy, Elsevier, vol. 178(C), pages 1456-1465.
    • Handle: RePEc:eee:renene:v:178:y:2021:i:c:p:1456-1465
    DOI: 10.1016/j.renene.2021.07.006
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    References listed on IDEAS

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    1. Okoye, P.U. & Abdullah, A.Z. & Hameed, B.H., 2017. "A review on recent developments and progress in the kinetics and deactivation of catalytic acetylation of glycerol—A byproduct of biodiesel," Renewable and Sustainable Energy Reviews, Elsevier, vol. 74(C), pages 387-401.
    2. Kumari, Dolly & Singh, Radhika, 2018. "Pretreatment of lignocellulosic wastes for biofuel production: A critical review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 90(C), pages 877-891.
    3. Saini, Jitendra Kumar & Patel, Anil Kumar & Adsul, Mukund & Singhania, Reeta Rani, 2016. "Cellulase adsorption on lignin: A roadblock for economic hydrolysis of biomass," Renewable Energy, Elsevier, vol. 98(C), pages 29-42.
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    1. Zhao, Man & Wang, Yanan & Zhou, Wenting & Zhou, Wei & Gong, Zhiwei, 2023. "Co-valorization of crude glycerol and low-cost substrates via oleaginous yeasts to micro-biodiesel: Status and outlook," Renewable and Sustainable Energy Reviews, Elsevier, vol. 180(C).
    2. Wang, Peng & Su, Yan & Tang, Wei & Huang, Caoxing & Lai, Chenhuan & Ling, Zhe & Yong, Qiang, 2022. "Revealing enzymatic digestibility of kraft pretreated larch based on a comprehensive analysis of substrate-related factors," Renewable Energy, Elsevier, vol. 199(C), pages 1461-1468.
    3. Fan, Meishan & Lei, Ming & Xie, Jun & Zhang, Hongdan, 2022. "Further insights into the solubilization and surface modification of lignin on enzymatic hydrolysis and ethanol production," Renewable Energy, Elsevier, vol. 186(C), pages 646-655.
    4. Wang, Xin & Fan, Ruichen & Yang, Qiang & Tao, Yehan & Lu, Jie & Du, Jian & Hu, Jinwen & Wang, Haisong, 2024. "Optimal tartaric acid pretreatment of reed for bioethanol production by fed batch semi-synchronous saccharification fermentation," Renewable Energy, Elsevier, vol. 227(C).

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