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Optimization of catalyst preparation conditions for direct sodium borohydride fuel cell using response surface methodology

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  • Okur, Osman
  • Alper, Erdogan
  • Almansoori, Ali

Abstract

The aim of this work is to determine the optimum operating conditions for the process of preparing anode electrocatalysts for direct sodium borohydride fuel cell (DSBHFC). Pt–Au/C electrocatalysts were studied as the anode catalysts while Pt/C were chosen as a cathode catalyst. Anode electrocatalysts were produced by the precipitation method. In this work, pH, temperature, drying time and Pt/Au ratio were selected as independent process parameters and their effects on dependent parameters, such as power density and hydrogen production rate, were investigated using response surface methodology (RSM). Based on this methodology, it was found that the maximum power density and the minimum hydrogen production rate were 354.4mWcm−2 and 30 mlmin−1 respectively. These findings were obtained at 90 °C, 9.27 pH, 61.07 h of drying time, and 93.54% Au ratio to total metal ratio.

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  • Okur, Osman & Alper, Erdogan & Almansoori, Ali, 2014. "Optimization of catalyst preparation conditions for direct sodium borohydride fuel cell using response surface methodology," Energy, Elsevier, vol. 67(C), pages 97-105.
    • Handle: RePEc:eee:energy:v:67:y:2014:i:c:p:97-105
    DOI: 10.1016/j.energy.2014.01.089
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    References listed on IDEAS

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    1. Carton, J.G. & Olabi, A.G., 2010. "Design of experiment study of the parameters that affect performance of three flow plate configurations of a proton exchange membrane fuel cell," Energy, Elsevier, vol. 35(7), pages 2796-2806.
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    2. Li, Li & Zheng, Keqing & Ni, Meng & Leung, Michael K.H. & Xuan, Jin, 2015. "Partial modification of flow-through porous electrodes in microfluidic fuel cell," Energy, Elsevier, vol. 88(C), pages 563-571.
    3. Tafaoli-Masoule, M. & Bahrami, A. & Elsayed, E.M., 2014. "Optimum design parameters and operating condition for maximum power of a direct methanol fuel cell using analytical model and genetic algorithm," Energy, Elsevier, vol. 70(C), pages 643-652.
    4. Chaisubanan, Napapat & Maniwan, Witchaya & Hunsom, Mali, 2017. "Effect of heat-treatment on the performance of PtM/C (M = Cr, Pd, Co) catalysts towards the oxygen reduction reaction in PEM fuel cell," Energy, Elsevier, vol. 127(C), pages 454-461.
    5. Zohdi-Fasaei, Hossein & Atashi, Hossein & Farshchi Tabrizi, Farshad & Mirzaei, Ali Akbar, 2017. "Modeling and optimization of Fischer-Tropsch synthesis over Co-Mn-Ce/SiO2 catalyst using hybrid RSM/LHHW approaches," Energy, Elsevier, vol. 128(C), pages 496-508.
    6. Najafi, Gholamhassan & Ghobadian, Barat & Yusaf, Talal & Safieddin Ardebili, Seyed Mohammad & Mamat, Rizalman, 2015. "Optimization of performance and exhaust emission parameters of a SI (spark ignition) engine with gasoline–ethanol blended fuels using response surface methodology," Energy, Elsevier, vol. 90(P2), pages 1815-1829.

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