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Production of hydrogen through the carbonation–calcination reaction applied to CH4/CO2 mixtures

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  • Barelli, L.
  • Bidini, G.
  • Corradetti, A.
  • Desideri, U.

Abstract

The production of hydrogen combined with carbon capture represents a possible option for reducing CO2 emissions in atmosphere and anthropogenic greenhouse effect. Nowadays the worldwide hydrogen production is based mainly on natural gas reforming, but the attention of the scientific community is focused also on other gas mixtures with significant methane content. In particular mixtures constituted mainly by methane and carbon dioxide are extensively used in energy conversion applications, as they include land-fill gas, digester gas and natural gas. The present paper addresses the development of an innovative system for hydrogen production and CO2 capture starting from these mixtures. The plant is based on steam methane reforming, coupled with the carbonation and calcination reactions for CO2 absorption and desorption, respectively. A thermodynamic approach is proposed to investigate the plant performance in relation to the CH4 content in the feeding gas. The results suggest that, in order to optimize the hydrogen purity and the efficiency, two different methodologies can be adopted involving both the system layout and operating parameters. In particular such methodologies are suitable for a methane content, respectively, higher and lower than 65%.

Suggested Citation

  • Barelli, L. & Bidini, G. & Corradetti, A. & Desideri, U., 2007. "Production of hydrogen through the carbonation–calcination reaction applied to CH4/CO2 mixtures," Energy, Elsevier, vol. 32(5), pages 834-843.
    • Handle: RePEc:eee:energy:v:32:y:2007:i:5:p:834-843
    DOI: 10.1016/j.energy.2006.06.008
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    References listed on IDEAS

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    1. Spiegel, R.J & Preston, J.L, 2003. "Technical assessment of fuel cell operation on landfill gas at the Groton, CT, landfill," Energy, Elsevier, vol. 28(5), pages 397-409.
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    Cited by:

    1. Barelli, L. & Ottaviano, A., 2014. "Solid oxide fuel cell technology coupled with methane dry reforming: A viable option for high efficiency plant with reduced CO2 emissions," Energy, Elsevier, vol. 71(C), pages 118-129.
    2. Barelli, L. & Bidini, G. & Gallorini, F., 2015. "SE-SR with sorbents based on calcium aluminates: Process optimization," Applied Energy, Elsevier, vol. 143(C), pages 110-118.
    3. Kavosh, Masoud & Patchigolla, Kumar & Anthony, Edward J. & Oakey, John E., 2014. "Carbonation performance of lime for cyclic CO2 capture following limestone calcination in steam/CO2 atmosphere," Applied Energy, Elsevier, vol. 131(C), pages 499-507.
    4. Li, Yingjie & Zhao, Changsui & Chen, Huichao & Ren, Qiangqiang & Duan, Lunbo, 2011. "CO2 capture efficiency and energy requirement analysis of power plant using modified calcium-based sorbent looping cycle," Energy, Elsevier, vol. 36(3), pages 1590-1598.
    5. Barelli, L. & Bidini, G. & Gallorini, F. & Servili, S., 2008. "Hydrogen production through sorption-enhanced steam methane reforming and membrane technology: A review," Energy, Elsevier, vol. 33(4), pages 554-570.
    6. Barelli, L. & Bidini, G. & Cinti, G. & Gallorini, F. & Pöniz, M., 2017. "SOFC stack coupled with dry reforming," Applied Energy, Elsevier, vol. 192(C), pages 498-507.

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    More about this item

    Keywords

    Hydrogen; Reforming; CO2 capture; Biogas; Solid acceptor;
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