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Evaluation of novel hydrogen integration options in bio-oils introduction to petrochemical refineries

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  • Bampaou, M.
  • Panopoulos, K.D.
  • Seferlis, P.
  • Voutetakis, S.

Abstract

Biomass integration into refineries allows to utilize existing infrastructures without deviating from established production routes and partially substitute fossil-with renewable-carbon. In particular, biomass after being converted by pyrolysis into bio-oil and then upgraded in the hydrotreatment section, it is inserted into existing refinery operations. Hydrogen is a key component during hydroprocessing since it is renewable and used in high excess. Reusing that unreacted hydrogen could prove beneficial for the economic viability of this scheme. An alternative hydrogen recovery technology is electrochemical compression that has the ability to recover and simultaneously compress hydrogen. The proposed biorefinery concept consists of the following subsystems: pyrolysis, hydrotreatment, gas cleaning, electrochemical hydrogen compression and PEM electrolysis. This work investigates the proposed scheme through flowsheet simulations and by determining crucial operating parameters that affect the overall economic and energetic performance. Results showed that recycling using an electrochemical compressor has significant economic and energetic benefits. Substantial cost reductions can also be attained from the economies-of-scale and by utilizing inexpensive electricity and biomass feedstocks. Overall, although the renewable hydrogen production cost surpasses that of the fossil-based, progress in the hydrogen processing techniques can further lower the expenses, transforming renewable hydrogen into a vital component for existing technologies.

Suggested Citation

  • Bampaou, M. & Panopoulos, K.D. & Seferlis, P. & Voutetakis, S., 2022. "Evaluation of novel hydrogen integration options in bio-oils introduction to petrochemical refineries," Energy, Elsevier, vol. 254(PB).
    • Handle: RePEc:eee:energy:v:254:y:2022:i:pb:s0360544222012567
    DOI: 10.1016/j.energy.2022.124353
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    References listed on IDEAS

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    1. Mohammad I. Jahirul & Mohammad G. Rasul & Ashfaque Ahmed Chowdhury & Nanjappa Ashwath, 2012. "Biofuels Production through Biomass Pyrolysis —A Technological Review," Energies, MDPI, vol. 5(12), pages 1-50, November.
    2. Sdanghi, G. & Maranzana, G. & Celzard, A. & Fierro, V., 2019. "Review of the current technologies and performances of hydrogen compression for stationary and automotive applications," Renewable and Sustainable Energy Reviews, Elsevier, vol. 102(C), pages 150-170.
    3. Zorana Božić & Dušan Dobromirov & Jovana Arsić & Mladen Radišić & Beata Ślusarczyk, 2020. "Power Exchange Prices: Comparison of Volatility in European Markets," Energies, MDPI, vol. 13(21), pages 1-15, October.
    4. Braimakis, Konstantinos & Atsonios, Konstantinos & Panopoulos, Kyriakos D. & Karellas, Sotirios & Kakaras, Emmanuel, 2014. "Economic evaluation of decentralized pyrolysis for the production of bio-oil as an energy carrier for improved logistics towards a large centralized gasification plant," Renewable and Sustainable Energy Reviews, Elsevier, vol. 35(C), pages 57-72.
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    1. Erwan Hermawan & Adiarso Adiarso & Sigit Setiadi & Dudi Hidayat, 2023. "Strategy for the implementation of sustainable green fuels in Indonesia," ECONOMICS AND POLICY OF ENERGY AND THE ENVIRONMENT, FrancoAngeli Editore, vol. 2023(1), pages 103-139.

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